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81.
通过对自配标准样品(正构烷烃)进行5à分子筛吸附试验,测定了用5分子筛吸附法分离前后正构烷烃、异构烷烃和环烷烃碳同位素值,探讨试验前后碳同位素值的变化。尽管实验过程中样品经过85℃长时间加热回流及吸附样品的5à分子筛用氢氟酸酸化处理,但实验结果经仪器检测,证明该方法对正构烷烃碳同位素值影响因素不大。本文还介绍了原油和煤可溶有机质中饱和烃络合前后的单体烃碳同位素分析方法。并在前人工作的基础上,改进采用微型索氏抽提加热回流实验装置,既提高了样品的回收率,也减少了样品中轻组分的损失。 相似文献
82.
原油在储层介质中的加水裂解生气模拟实验 总被引:5,自引:2,他引:5
采用高温高压热模拟实验方法,开展了原油在砂岩和火成岩储层介质中的加水裂解生气模拟实验研究.结果表明,原油开始大量裂解的温度是400℃,随模拟温度增加,甲烷相对含量增大,乙烷以上重烃气尤其是丙烷相对含量减小.其中砂岩的油水混合物裂解生气主要发生在450~500℃之间,生气窗范围小,对应的烃气产率高,火成岩的油水混合物裂解生气主要发生在450~600℃之间,生气窗范围大,对应的烃气产率小.模拟烃气的组分碳同位素分馏显著,随模拟温度增加呈变重趋势.在裂解生气过程中,水解加氢和催化作用对烃气的组成、产率和碳同位素分布有重要影响。 相似文献
83.
Constraints on the application of carbon isotope thermometry in high- to ultrahigh-temperature metamorphic terranes 总被引:7,自引:0,他引:7
Nine marble horizons from the granulite facies terrane of southern India were examined in detail for stable carbon and oxygen isotopes in calcite and carbon isotopes in graphite. The marbles in Trivandrum Block show coupled lowering of δ13C and δ18O values in calcite and heterogeneous single crystal δ13C values (? 1 to ? 10‰) for graphite indicating varying carbon isotope fractionation between calcite and graphite, despite the granulite facies regional metamorphic conditions. The stable isotope patterns suggest alteration of δ13C and δ18O values in marbles by infiltration of low δ13C–δ18O‐bearing fluids, the extent of alteration being a direct function of the fluid‐rock ratio. The carbon isotope zonation preserved in graphite suggests that the graphite crystals precipitated/recrystallized in the presence of an externally derived CO2‐rich fluid, and that the infiltration had occurred under high temperature and low fO2 conditions during metamorphism. The onset of graphite precipitation resulted in a depletion of the carbon isotope values of the remaining fluid+calcite carbon reservoir, following a Rayleigh‐type distillation process within fluid‐rich pockets/pathways in marbles resulting in the observed zonation. The results suggest that calcite–graphite thermometry cannot be applied in marbles that are affected by external carbonic fluid infiltration. However, marble horizons in the Madurai Block, where the effect of fluid infiltration is not detected, record clear imprints of ultrahigh temperature metamorphism (800–1000 °C), with fractionations reaching <2‰. Zonation studies on graphite show a nominal rimward lowering δ13C on the order of 1 to 2‰. The zonation carries the imprint of fluid deficient/absent UHT metamorphism. Commonly, calculated core temperatures are > 1000 °C and would be consistent with UHT metamorphism. 相似文献
84.
As a legacy of the centrally planned economy, the economies in transition of Central and Eastern Europe (CEE) have a unique
potential to reduce their greenhouse gas emissions through the improvement in their high energy intensities. Since much of
this `low-hanging fruit' in energy-efficiency improvements can be highly cost-effective, many developed countries facing difficulties
in meeting their greenhouse gas (GHG) emission targets domestically are eager to find such opportunities in the CEE region.
Therefore, studies analysing the potentials and costs of carbon dioxide reduction through technology improvement in the region
have come into the limelight. While there are a few excellent studies in the region aimed at analysing climate change abatement
potentials, they all embark on different assumptions, methodologies and boundary conditions. It is hence difficult, if not
impossible, to compare and analyse the results of these studies across different authors, countries or time horizons. Consequently,
the purpose of this paper is to place four leading studies on GHG mitigation through technology improvement from the CEE region
into an internationally comparable framework. Four studies were selected from three countries, Poland, Hungary and Estonia,
which are all the results of major national and international efforts to assess costs and potentials of GHG reduction. The
paper places their assumptions, methods and final results into a framework which enables policy-makers and project designers
to compare these across geographical and technological boundaries. Since other studies from around the globe have been analysed
in this framework in the literature, this paper provides a vehicle for the findings of these four studies to be compared to
others worldwide. In addition, the paper highlights a few areas where similar studies to be completed in the future in the
region may be enhanced by incorporating features used in GHG mitigation research in other parts of the world.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
85.
空树河组是滇西腾冲地块北部的石碳-二叠纪冈瓦纳相沉积。菱铁矿结核见于该组顶部的黑色泥岩中。将一个结核通过中心切开,在切面上由中心向边缘用牙钻等间隔提取10个样品。同位素测试结果显示,δ^13C自中心向边缘逐渐由-8.09%减为-16.12%,最外一个样例外(-15.39‰),而δ^18O自中心向边缘逐渐由-10.64‰增加为0‰左右。δ^13C的变化情况表明,菱铁矿结核可能形成于硫酸盐还原带。在解释δ^18o的变化情况时,推测在结核开始生长时可能有δ^18O亏损的大气降水掺入,随着埋藏深度的逐渐加大,孔隙水的O同位素逐渐趋近正常海水的值(0‰)。 相似文献
86.
The Hongzuisi Section in Lanzhou area is used to infer the paleoclimate since the late glacial epoch. Through combined analysis of organic carbon isotope and CaCO3 content, paleoenvironment evolution of Hongzuisi Section since the late glacial epoch is discussed. There were changes in both drymoist and warm-cold. Especially the climate changes can be compared with synchronous sections of other areas, which provides useful information for our future forecast. 相似文献
87.
近20年海南岛森林生态系统碳储量变化 总被引:49,自引:2,他引:49
热带森林在碳循环研究中有重要作用。根据目前森林碳储量的计算方法和海南森林资源二类调查数据 ,估算了不同时段的碳储量 ,并分析其动态变化特点。结果表明 :海南森林碳储量从 1979年的 30 4 5TgC增加到 1998年的 37 74TgC ,年均增加 0 36 4 5TgC ,增长率为1 19% ,是全国平均增长率的 2 5倍 ;海南森林在碳循环中起不断增强的碳汇作用 ;森林碳密度呈加速减少趋势 ,储碳潜力将很大 ;随着海南全面禁止采伐和封育等林业措施的实施 ,森林面积扩大 ,林龄结构改善 ,储碳能力将进一步提高 ,海南森林在全国或全球碳循环中的作用和社会价值与意义将日渐突出。通过对碳储量计算不确定性的分析和讨论 ,提出应加强对森林群落各层次生物量的实测与实地监测研究 ,统一计算方法 ,以提高碳储量计算的精度 相似文献
88.
Rebecca J. Kent 《The Geographical journal》2002,168(1):48-56
The soil conservation campaigns that have been a prominent feature of Jamaican agricultural policy since the 1950s are frequently presented as having failed to ameliorate the problem of soil erosion in hillside agriculture. A case study of a small farming community in the Blue Mountains explores the development of the soil conservation practices currently employed by farmers. The use of trash barriers in carrot farming is described and the origins of this technology and its subsequent adaptation are considered. The study concludes that extension interventions and government policy have influenced the development of current soil conservation practices; practices which have their roots in indigenous techniques. Other factors such as the adaptation of trash barriers to suit local conditions and their importance in soil fertility management also play a role in their widespread use in the study area. The study demonstrates that to understand the process of technical change in farming communities, it is necessary to consider a range of factors, external and internal, technical and social, that have over time influenced farmers' decision making. 相似文献
89.
Floodplains are ecotones that form a transition between aquatic and terrestrial environments. These important ecosystems can be described as dynamic spatial mosaics in which water plays an important role in connecting various patches on the floodplain surface. Hydrological connections facilitate the exchange of carbon and nutrients between the river channel and the floodplain and therefore influence the productivity of the entire river system. This paper examines the influence of hydrological connections on the potential exchange of dissolved organic carbon between a large Australian floodplain to a river channel, and the effects of land and water developments on these exchanges. The paper proposes that an understanding of floodplain ecosystems requires an interdisciplinary approach—a recognition of the importance of the three disciplines hydrology, geomorphology and ecology. Large-scale water-resources and floodplain development has significantly altered the spatial and temporal patterns of hydrological characteristics in the Lower Balonne floodplain, Australia. The magnitude, frequency and duration of flooding events have all been reduced. The construction of levees and water storages has also reduced the reactive floodplain surface area. The presented data show the impacts of these changes on the potential supply of dissolved organic carbon from the floodplain surface during periods of inundation. Annual reductions of up to 1293 tonnes of dissolved organic carbon supply were noted and reductions were especially significant for floods with an average recurrence interval of 2 years or less. Some small flood events no longer facilitate the potential supply of dissolved organic carbon from the floodplain to the river channel because of water-resources and floodplain developments. 相似文献
90.
油气化探中甲烷碳同位素应用、存在问题与对策研究 总被引:5,自引:2,他引:5
阐述了在地表油气化探实践当中甲烷碳同位素对地表土壤烃气成因判别的有效性,但有时也会遇到判断错误的情况。通过对应用实例的分析,指出因忽略了土壤中异常甲烷是一种混合成因甲烷,从而导致判断失误。为全面解决这一问题,提出了同时选送数量相当的背景土壤样品和异常样品进行甲烷同位素测定,然后通过教学方法计算出真实反映来源于油气藏中的甲烷的碳同位素值的对策方案。 相似文献