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41.
Curtis M. Oldenburg 《Environmental Geology》2008,54(8):1687-1694
A screening and ranking framework (SRF) has been developed to evaluate potential geologic carbon dioxide (CO2) storage sites on the basis of health, safety, and environmental (HSE) risk arising from CO2 leakage. The approach is based on the assumption that CO2 leakage risk is dependent on three basic characteristics of a geologic CO2 storage site: (1) the potential for primary containment by the target formation; (2) the potential for secondary containment
if the primary formation leaks; and (3) the potential for attenuation and dispersion of leaking CO2 if the primary formation leaks and secondary containment fails. The framework is implemented in a spreadsheet in which users
enter numerical scores representing expert opinions or published information along with estimates of uncertainty. Applications
to three sites in California demonstrate the approach. Refinements and extensions are possible through the use of more detailed
data or model results in place of property proxies. 相似文献
42.
Laura Chiaramonte Mark D. Zoback Julio Friedmann Vicki Stamp 《Environmental Geology》2008,54(8):1667-1675
This paper reports a preliminary investigation of CO2 sequestration and seal integrity at Teapot Dome oil field, Wyoming, USA, with the objective of predicting the potential risk
of CO2 leakage along reservoir-bounding faults. CO2 injection into reservoirs creates anomalously high pore pressure at the top of the reservoir that could potentially hydraulically
fracture the caprock or trigger slip on reservoir-bounding faults. The Tensleep Formation, a Pennsylvanian age eolian sandstone
is evaluated as the target horizon for a pilot CO2 EOR-carbon storage experiment, in a three-way closure trap against a bounding fault, termed the S1 fault. A preliminary geomechanical
model of the Tensleep Formation has been developed to evaluate the potential for CO2 injection inducing slip on the S1 fault and thus threatening seal integrity. Uncertainties in the stress tensor and fault
geometry have been incorporated into the analysis using Monte Carlo simulation. The authors find that even the most pessimistic
risk scenario would require ∼10 MPa of excess pressure to cause the S1 fault to reactivate and provide a potential leakage
pathway. This would correspond to a CO2 column height of ∼1,500 m, whereas the structural closure of the Tensleep Formation in the pilot injection area does not exceed
100 m. It is therefore apparent that CO2 injection is not likely to compromise the S1 fault stability. Better constraint of the least principal stress is needed to
establish a more reliable estimate of the maximum reservoir pressure required to hydrofracture the caprock. 相似文献
43.
This paper presents an example of application of the double solid reactant method (DSRM) of Accornero and Marini (Environmental
Geology, 2007a), an effective way for modeling the fate of several dissolved trace elements during water–rock interaction. The EQ3/6 software
package was used for simulating the irreversible water–rock mass transfer accompanying the generation of the groundwaters
of the Porto Plain shallow aquifer, starting from a degassed diluted crateric steam condensate. Reaction path modeling was
performed in reaction progress mode and under closed-system conditions. The simulations assumed: (1) bulk dissolution (i.e.,
without any constraint on the kinetics of dissolution/precipitation reactions) of a single solid phase, a leucite-latitic
glass, and (2) precipitation of amorphous silica, barite, alunite, jarosite, anhydrite, kaolinite, a solid mixture of smectites,
fluorite, a solid mixture of hydroxides, illite-K, a solid mixture of saponites, a solid mixture of trigonal carbonates and
a solid mixture of orthorhombic carbonates. Analytical concentrations of major chemical elements and several trace elements
(Cr, Mn, Fe, Ni, Cu, Zn, As, Sr and Ba) in groundwaters were satisfactorily reproduced. In addition to these simulations,
similar runs for a rhyolite, a latite and a trachyte permitted to calculate major oxide contents for the authigenic paragenesis
which are comparable, to a first approximation, with the corresponding data measured for local altered rocks belonging to
the silicic, advanced argillic and intermediate argillic alteration facies. The important role played by both the solid mixture
of trigonal carbonates as sequestrator of Mn, Zn, Cu and Ni and the solid mixture of orthorhombic carbonates as scavenger
of Sr and Ba is emphasized.
相似文献
Luigi Marini (Corresponding author)Email: |
44.
Wenjun Yong E. Dachs A. C. Withers E. J. Essene 《Contributions to Mineralogy and Petrology》2008,155(2):137-146
The low-temperature heat capacity (C
p) of Si-wadeite (K2Si4O9) synthesized with a piston cylinder device was measured over the range of 5–303 K using the heat capacity option of a physical
properties measurement system. The entropy of Si-wadeite at standard temperature and pressure calculated from the measured
heat capacity data is 253.8 ± 0.6 J mol−1 K−1, which is considerably larger than some of the previous estimated values. The calculated phase transition boundaries in the
system K2O–Al2O3–SiO2 are generally consistent with previous experimental results. Together with our calculated phase boundaries, seven multi-anvil
experiments at 1,400 K and 6.0–7.7 GPa suggest that no equilibrium stability field of kalsilite + coesite intervenes between
the stability field of sanidine and that of coesite + kyanite + Si-wadeite, in contrast to previous predictions. First-order
approximations were undertaken to calculate the phase diagram in the system K2Si4O9 at lower pressure and temperature. Large discrepancies were shown between the calculated diagram compared with previously
published versions, suggesting that further experimental or/and calorimetric work is needed to better constrain the low-pressure
phase relations of the K2Si4O9 polymorphs.
Electronic supplementary material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
45.
H2O-undersaturated melting experiments of synthesized basalt (SiO2 = 50.7 wt.%, MgO = 8.3 wt.%, Mg# = 60) were conducted at fO2 corresponding to NNO+1 and NNO−1 to clarify the effects of pressure (2–7 kbar) and H2O on fractional crystallization in island arcs. H2O content was ranged from nominally anhydrous to 4.4 wt.%. Differentiation trends, namely the liquid lines of descent, change
sensitively according to pressure-H2O relations. Tholeiitic differentiation trends are reproduced with H2O ≤ ∼2 wt.% in primary magma. With such quantities of H2O, fractional crystallization is controlled by olivine + plagioclase at 2 kbar. Increasing the pressure from 2 to ≥4 kbar
induces early crystallization of orthopyroxene instead of olivine and therefore SiO2 enrichment in the residual melts is suppressed. Increasing H2O (≥ ∼2 wt.% in primary magma) stabilizes clinopyroxene relative to orthopyroxene and/or magnetite. Although the phase relations
and proportions strongly depend on fO2 and H2O content, differentiation trends are always calc-alkaline. 相似文献
46.
Complexity theory has received considerable attention over the past decade from a wide variety of disciplines. Some who write on this topic suggest that complexity theory will lead to a unifying understanding of complex phenomena; others dismiss it as a passing and disruptive fad. We suggest that for the analysis of coupled natural/human systems, the truth emerges from the middle ground. As an approach focused as much on the connections among system elements as the elements themselves, we argue that complexity theory provides a useful conceptual framework for the study of coupled natural/human systems. It is, if nothing else, a framework that leads us to ask interesting questions about, for example, sustainability, resilience, threshold events, and predictability.In this paper we attempt to demystify the ongoing discussions on complexity theory by linking its evocative and overloaded terminology to real-world processes. We illustrate how a shift in focus from system elements to connections among elements can lead to meaningful insight into human-environment interactions that might otherwise be overlooked. We ground our discussion in ongoing interdisciplinary research surrounding Yellowstone National Park’s northern elk winter range; a tightly coupled natural/human system that has been the center of debate, conflict, and compromise for more than 135 years. 相似文献
47.
Klauea historical summit lavas have a wide range in matrix 18OVSMOWvalues (4·9–5·6) with lower values in rockserupted following a major summit collapse or eruptive hiatus.In contrast, 18O values for olivines in most of these lavasare nearly constant (5·1 ± 0·1). The disequilibriumbetween matrix and olivine 18O values in many samples indicatesthat the lower matrix values were acquired by the magma afterolivine growth, probably just before or during eruption. BothMauna Loa and Klauea basement rocks are the likely sources ofthe contamination, based on O, Pb and Sr isotope data. However,the extent of crustal contamination of Klauea historical magmasis probably minor (< 12%, depending on the assumed contaminant)and it is superimposed on a longer-term, cyclic geochemicalvariation that reflects source heterogeneity. Klauea's heterogeneoussource, which is well represented by the historical summit lavas,probably has magma 18O values within the normal mid-ocean ridgebasalt mantle range (5·4–5·8) based on thenew olivine 18O values. KEY WORDS: Hawaii; Klauea; basalt; oxygen isotopes; crustal contamination 相似文献
48.
Serena C. Tarantino Michele Zema Tiziana Boffa Ballaran Paolo Ghigna 《Physics and Chemistry of Minerals》2008,35(2):71-76
High-pressure single-crystal X-ray diffraction measurements of lattice parameters of the compound Li2VOSiO4, which crystallises with a natisite-type structure, has been carried out to a pressure of 8.54(5) GPa at room temperature.
Unit-cell volume data were fitted with a second-order Birch-Murnaghan EoS (BM-EoS), simultaneously refining V
0 and K
0 using the data weighted by the uncertainties in V. The bulk modulus is K
0 = 99(1) GPa, with K′ fixed to 4. Refinements of third order equations-of-state yielded values of K′ that did not differ significantly from 4. The compressibility of the unit-cell is strongly anisotropic with the c axis (K
0(c) = 49.7 ± 0.5 GPa) approximately four times more compressible than the a axis (K
0(a) = 195 ± 3 GPa). 相似文献
49.
CO2地质埋存渗漏风险及补救对策 总被引:7,自引:1,他引:6
目前,将CO2埋存于地下深部地质构造(如油气藏、煤层、地下含水层及岩溶盐腔)的减排方案能有效地减缓温室效应而备受关注。无论什么储集体,我们都希望CO2在地下埋存的时间越长越好。然而,对于一项具体工程的实施,必然存在一些客观和主观因素造成CO2渗漏,比如废弃井的不完善或不合理处理、地层断裂系统和水动力系统以及地震所造成的渗漏等等。存在渗漏就可能会对周围人和生态环境造成危害。因此,进行CO2地质埋存的风险评估是相当有必要的,是我们能长期有效安全地进行该项减排方案必不可少的基础和保证。本文即想从建立一套完整的风险评估、管理和监测体系的角度并以加拿大Weyburn油田为例,深入分析CO2地质埋存中可能存在的渗漏风险和途径,建立CO2渗漏风险评估机制,并针对具体的渗漏可能性提出相应的补救对策,为全球范围内,尤其对我国刚刚开展CO2地质埋存研究工作提供一些有益的思路。 相似文献
50.
位于辽东湾西部低凸起北端的JZ20-2超压凝析气田,离供烃中心较远,压力系数却达到1.56~1.7,这在我国东部裂谷盆地比较少见。经过综合分析,作者认为JZ20-2凝析气田异常高压的形成与其所处的特殊地质背景紧密相关,辽中凹陷沙河街组三段超压凝析油气沿不整合面、砂体输导通道向辽东湾西部低凸起的运移、充注和能量的侧向传递是JZ20-2凝析气田异常高压形成的根本原因,而上覆东营组二段下亚段-东营组三段巨厚的强超压泥岩封盖和辽西3号边界断层侧向遮挡共同构成的优越封闭环境是超压保存的必要条件。本文分析了该气田超压特征及其远距离超压侧向传递的成因机制,不仅有助于揭示辽东湾西部低凸起超压流体运移聚集的规律和成藏作用,而且可能提供了一个超压远距离侧向传递的典型实例。 相似文献