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81.
Katsumi Matsumoto 《Journal of Oceanography》2006,62(6):887-902
Iron fertilization of nutrient-rich surface waters of the ocean is one possible way to help slow the rising levels of atmospheric
CO2 by sequestering it in the oceans via biological carbon export. Here, I use an ocean general circulation model to simulate
a patch of nutrient depletion in the subpolar northwest Pacific under various scenarios. Model results confirm that surface
fertilization is an inefficient way to sequester carbon from the atmosphere (Gnanadesikan et al., 2003), since only about 20% of the exported carbon comes initially from the atmosphere. Fertilization reduces future production
and thus CO2 uptake by utilizing nutrients that would otherwise be available later. Effectively, this can be considered as leakage when
compared to a control run. This “effective” leakage and the actual leakage of sequestered CO2 cause a significant, rapid decrease in carbon retention (only 30–45% retained after 10 years and less than 20% after 50 years).
This contrasts markedly with the almost 100% retention efficiency for the same duration using the same model, when carbon
is disposed directly into the northwest Pacific (Matsumoto and Mignone, 2005). As a consequence, the economic effectiveness
of patch fertilization is poor in two limiting cases of the future price path of carbon. Sequestered carbon in patch fertilization
is lost to the atmosphere at increasingly remote places as time passes, which would make monitoring exceedingly difficult.
If all organic carbon from one-time fertilization reached the ocean bottom and remineralized there, acidification would be
about −0.05 pH unit with O2 depletion about −20 μmol kg−1. These anomalies are probably too small to seriously threaten deep sea biota, but they are underestimated in the model because
of its large grid size. The results from this study offer little to advocate purposeful surface fertilization as a serious
means to address the anthropogenic carbon problem. 相似文献
82.
83.
气相色谱指纹法在海上油污染源鉴别中的应用 总被引:4,自引:0,他引:4
通过一个具体案例,探讨了气相色谱指纹法在海上油污染源鉴别中的应用。该鉴别方法基于样品的正构烷烃气相色谱指纹分析,选择既能表征油种固有特性,又受风化影响较小的正十七烷(n-C17)、正十八烷(n-C18)、姥鲛烷(phy)、植烷(phy)和正二十烷(n-C20)等特征烷烃作为判据,可信度大,而且整个操作流程短(一般不超过半天),较简便易行。 相似文献
84.
渤海、黄海、东海沉积物中矿物组合的研究 总被引:12,自引:2,他引:12
本文对黄海、渤海、东海以及长江、黄河、辽河表层沉积物中的轻、重矿物进行了研究。分析资料表明,调查区内共有三种类型的矿物:陆源矿物、自生矿物和海底火山喷发形成的火山型矿物。根据轻、重矿物组合的差异,可把调查区分成8个矿物区。其物质来源主要为黄河与长江。黄河物质主要沉积在黄海、渤海;长江物质沉积在东海陆架区,而冲绳海槽则发现有海底火山喷发物质与浊流沉积。 相似文献
85.
秋茄和榕树叶片中正构烷烃分布和单体化合物δ13C值及其光合作用 总被引:1,自引:0,他引:1
对深圳福田、阳江、海南新竹红树林秋茄Kandelia candel及海口榕树Ficusm icrocarpa叶中类脂物进行萃取,分离出正构烷烃,通过气相色谱(GC)及色谱-质谱(GC MS)分析,测出了正构烷烃的碳数分布和相对含量.气相色谱-稳定同位素比质谱仪(GC-IRMS)测定了正构烷烃单体化合物的稳定同位素组成δ13C.秋茄叶和榕树叶正构烷烃的碳数分布均为C17C33,主要集中在C23-C31(>90%).化合物含量最高为C27的有深圳福田秋茄、海南新竹秋茄、海口榕树,而阳江秋茄为C25.单体化合物的稳定同位素δ13C深圳福田秋茄为-31.42‰-34.48‰,阳江秋茄为-31.69‰-33.62‰,海南新竹秋茄为-30.30‰-33.04‰,海口榕树为-29.92‰33.56‰;平均值分别为-32.95‰、32.67‰、31.67‰、-31.74‰.结果表明,秋茄和陆地植物榕树的光合作用都是通过C3途径,是典型C3植物. 相似文献
86.
分析了赤道东北太平洋海域沉积物中Ba、Ti、Al和有机碳(Corg)的含量。研究表明,研究区沉积物中钡为0.198%~0.792%;采用标准陆源物质扣除法获得的生物钡(Babio)的含量为0.162%~0.764%,占沉积物中总钡含量的81.6%~96.5%,平均为88.7%,其在沉积物中的分布表现为上部一致,下部变化较大;有机碳(Corg)的含量为0.18%~0.58%,并表现为随沉积物深度的增加而降低。沉积物中Babio/Ti的比值表现为东区高于西区,且向高纬度降低的特点,而沉积物中Corg/Ti和Babio/Ti则表现为负相关关系,表明研究区沉积物中钡可能和上层海洋生产力的相关性不明显。 相似文献
87.
台湾海峡表层沉积物中重矿物特征及其物质来源 总被引:15,自引:0,他引:15
台湾海峡重矿物平均分布0.95%,其分布由西岸向东岸递减;由北部经台湾浅滩朝粤东方向缓慢递减。碎屑矿物46种,以角闪石、绿帘石、磁铁矿、钛铁矿、褐铁矿和片状矿物为主,它们占重矿物含量的67%。据主要重矿物含量将海峡分成8个矿物组合区。碎屑矿物来自海峡两岸基岩,通过河流搬运入海,有部分片状矿物为海峡以北的物质随浙闽沿岸流进入海峡而沉积。其海绿石是台湾西岸、澎湖岛第三系或第四系含海绿石岩层剥蚀后搬运入海沉积而成的。台湾浅滩的残留沉积物为晚更新世低海面时期的河口滨海相沉积物。由于处在开放的海洋环境,至今没有接受现代沉积。残留沉积物中的磁铁矿、钛铁矿、锆石等重矿物相对富集,含量高于近源海域,有可能赋存浅海砂矿。 相似文献
88.
R. E. Kirk K. Robertson R. B. Whitmarsh P. R. Miles 《Marine Geophysical Researches》1991,13(2):153-160
A technique has been devised for firing arrays of bottom shots on the ocean bed in depths upto 4000 m or more. Ten kilogram explosive charges are dropped from the surface while the shooting ship is navigated acoustically. They are detonated at preset times by an electronic timer which initiates an electrical detonator, detonating cord and cast PETN/TNT explosive. Ranges to ocean bottom seismographs, and the shot instants, can be calculated from the arrival-time differences of the direct and surface-reflected water waves. The accuracy, which is dependent on water-depth and range, was better than 22 m in range and 14 msec in shot instant for our experiments. 相似文献
89.
The common assumption that the ratio between particulate organic carbon (POC) and particulate 234Th obtained from shallow sediment traps and filterable particles are representative of the ratio in the total particle settling flux should be treated with caution in view of well-known biases associated with tethered shallow sediment traps and the decoupling between size and settling velocity of many natural particle regimes. To make progress toward reliably constraining the POC / 234Th ratio on truly settling particles, we have tested here a settling collection technique designed to remove any hydrodynamic bias; split flow-thin cell fractionation (SPLITT). These first results from a North Sea fjord and an open Baltic Sea time-series station indicates that the POC / 234Th ratio on the more complete particle-settling spectrum, isolated with SPLITT, was higher than the POC / 234Th ratio obtained simultaneously from tethered shallow sediment traps in seven out of seven parallel deployments with an average factor of 210%. The POC / 234Th ratio from the SPLITT was either in the same range or higher than that obtained on filtered “bulk” particles. To explain this novel data we hypothesize that the slowest settling fraction is organic-matter rich and does not strongly complex 234Th (i.e., high POC / 234Th). We suggest that this ultra-slow sinking fraction is better collected by SPLITT than with tethered sediment traps because of minimized hydrodynamic bias.This was tested using the ratio of POC / Al as a tracer of detrital mineral-ballast influenced settling velocity. The higher POC / Al ratios in SPLITT samples relative to in traps is consistent with the hypothesis that SPLITT is better suited for collecting also the slow-settling component of sinking particles. This important slow-settling component appears to here consist primarily of non-APS/TEP components of plankton exudates or other less-strongly 234Th-complexing organic matter. Further applications of the SPLITT technique are likely to return increasingly new insights on the composition (including “truly settling” POC / 234Th) of the total spectrum of particles settling out of the upper ocean. 相似文献
90.
The physical and chemical variability of the water column at subtidal station of an estuary in the Seto Inland Sea, Japan,
was studied over a 24-hour period during a spring tide (tidal range ca. 2 m) in May 1995. Surface water and several depths through the water column were monitored every one and two hours, respectively.
At each occasion, water temperature, salinity and dissolved oxygen concentration were measured and water samples were collected
for the determination of nutrients and suspended particulate matter (SPM). Disruptive changes in the physical and chemical
characteristics of the water was produced by the tidal cycle and the mixing of water masses of different origin. These changes
were highly significant both spatially and temporally, yet with varying effects on physical parameters, nutrients and the
different components of SPM. Significant differences in nutrient concentrations were also observed when the data-set was divided
into ebb and flood components, irrespective of the depth. Nitrate and nitrite rose to 1.8 times higher during the flood. Spatial
differences of SPM were less marked than those of nutrients, only particulate organic carbon (POC) being significantly higher
at the surface than in the intermediate and the lower layer. Both POC and pheopigment concentrations increased markedly through
the water column, being highest shortly before the lower low tide. In contrast, suspended solid (SS) content increased sharply
after the lower low tide (>40 mg l−1) and this coincided with a marked decrease of the C/SS content (<20 mg g−1). The lagtime between POC and SS tidal transport was caused by particle resuspension from the exposed intertidal sediments
as the tidal level rose, and particle transport selection in relation to the tidal state.
This revised version was published online in August 2006 with corrections to the Cover Date. 相似文献