Negative-emissions technology portfolios to meet the 1.5 °C target     

《Global Environmental Change》2021

Our carbon-intensive economy has led to an average temperature rise of 1 °C since pre-industrial times. As a consequence, the world has seen increasing droughts, significant shrinking of the polar ice caps, and steady sea-level rise. To stall these issues’ worsening further, we must limit global warming to 1.5 °C. In addition to the economy’s decarbonization, this endeavour requires the use of negative-emissions technologies (NETs) that remove the main greenhouse gas, carbon dioxide, from the atmosphere. While techno-economic feasibility alone has driven the definition of negative-emissions solutions, NETs’ diverse, far-reaching implications demand a more holistic assessment. Here, we present a comprehensive framework, integrating NETs’ critical performance aspects of feasibility, effectiveness, and side impacts, to define the optimal technology mix within realistic outlooks. The resulting technology portfolios provide a useful new benchmark to compare carbon avoidance and removal measures and deliberately choose the best path to solve the climate emergency.  相似文献   

微/纳结构的弗雷德盐对铜的絮凝-吸附研究     

周丽芸  章兴华  雷平  陆洋  龚国洪  朱守平 《矿物学报》2012,32(4):548-554

以含钙聚合铝(PACCa)作为导向剂与铝源,在常温常压下合成了微/纳结构(微米/纳米尺度)的弗雷德盐。当水溶液中的ρ(Cu2+)为4.406 mg/L时,每升含铜溶液投入0.45 g弗雷德盐对Cu2+的去除率为99.02%。背散射(BEI)与二次电子(SEI)的SEM研究表明:微/纳结构的弗雷德盐在水处理中经历了溶解-结晶过程,XRD鉴定证实弗雷德盐分解后形成方解石晶体与无定形氧化铝。微/纳结构的弗雷德盐去除Cu2+的絮凝沉淀机理与吸附反应模式有所不同,弗雷德盐在絮凝过程中与水中CO2作用转变成方解石与无定形氧化铝,同时Cu2+在碱性环境下生成氢氧化物,新生成的无定型氢氧化铝迅速吸附铜的氢氧化物并裹挟方解石沉淀。  相似文献   

基于波形切除反褶积的探地雷达信号处理效果     

石刚  田养军  杨晓华 《物探与化探》2012,36(6):981-984

探地雷达接收天线通常采用超宽频带进行记录,接收信号中含有多种干扰.为了消除探地雷达记录中的多次波干扰,提高信噪比,提出了将波形切除反褶积应用于探地雷达信号后处理的方法,提高了记录的纵向分辨率.阐述了该方法的原理和实现过程,分析了适用范围和应用条件.模型试验的结果表明雷达信号的多次干扰和随机干扰明显得到压制,图像效果明显得到改善.  相似文献   

基于不同小波变换与同态滤波结合的CBERS-02B卫星CCD图像的薄云去除     

韩念龙  刘闯  庄立  张巍 《吉林大学学报(地球科学版)》2012,42(1):275-279,288

卫星CCD图像的去云处理对遥感信息的增强与提取有重要的意义,尤其是在云覆盖严重的低纬度地区。为去除CBERS-02B卫星CCD图像中薄云的影响,分别使用Mallat和à trous 2种小波变换对图像进行分解;利用同态滤波对2种小波分解图像的低频系数进行处理,衰减其低频信息;将处理后的小波低频系数与分解的高频系数进行小波重构,从而达到去云的目的。定量分析基于Mallat和à trous小波变换结合同态滤波法的去云结果表明,经à trous小波变换结合同态滤波法的去云影像所包含信息量大,细节信息丰富,去云效果较好。  相似文献   

Water-removed spectra increase the retrieval accuracy when estimating savanna grass nitrogen and phosphorus concentrations   总被引：2，自引：0，他引：2  

Abel Ramoelo  Andrew K. SkidmoreMartin Schlerf  Renaud MathieuIgnas M.A. Heitkönig 《ISPRS Journal of Photogrammetry and Remote Sensing》2011,66(4):408-417

Information about the distribution of grass foliar nitrogen (N) and phosphorus (P) is important for understanding rangeland vitality and for facilitating the effective management of wildlife and livestock. Water absorption effects in the near-infrared (NIR) and shortwave-infrared (SWIR) regions pose a challenge for nutrient estimation using remote sensing. The aim of this study was to test the utility of water-removed (WR) spectra in combination with partial least-squares regression (PLSR) and stepwise multiple linear regression (SMLR) to estimate foliar N and P, compared to spectral transformation techniques such as first derivative, continuum removal and log-transformed (Log(1/R)) spectra. The study was based on a greenhouse experiment with a savanna grass species (Digitaria eriantha). Spectral measurements were made using a spectrometer. The D. eriantha was cut, dried and chemically analyzed for foliar N and P concentrations. WR spectra were determined by calculating the residual from the modelled leaf water spectra using a nonlinear spectral matching technique and observed leaf spectra. Results indicated that the WR spectra yielded a higher N retrieval accuracy than a traditional first derivative transformation (R²=0.84, RMSE = 0.28) compared to R²=0.59, RMSE = 0.45 for PLSR. Similar trends were observed for SMLR. The highest P retrieval accuracy was derived from WR spectra using SMLR (R²=0.64, RMSE = 0.067), while the traditional first derivative and continuum removal resulted in lower accuracy. Only when using PLSR did the first derivative result in a higher P retrieval accuracy (R²=0.47, RMSE = 0.07) than the WR spectra (R²=0.43, RMSE = 0.070). It was concluded that the water removal technique is a promising technique to minimize the perturbing effect of foliar water content when estimating grass nutrient concentrations.  相似文献   

A buoyant plume adjacent to a headland—Observations of the Elwha River plume     

Jonathan A. Warrick  Andrew W. Stevens 《Continental Shelf Research》2011,31(2):85-97

Small rivers commonly discharge into coastal settings with topographic complexities - such as headlands and islands - but these settings are underrepresented in river plume studies compared to more simplified, straight coasts. The Elwha River provides a unique opportunity to study the effects of coastal topography on a buoyant plume, because it discharges into the Strait of Juan de Fuca on the western side of its deltaic headland. Here we show that this headland induces flow separation and transient eddies in the tidally dominated currents (O(100 cm/s)), consistent with other headlands in oscillatory flow. These flow conditions are observed to strongly influence the buoyant river plume, as predicted by the “small-scale” or “narrow” dynamical classification using Garvine's (1995) system. Because of the transient eddies and the location of the river mouth on the headland, flow immediately offshore of the river mouth is directed eastward twice as frequently as it is westward. This results in a buoyant plume that is much more frequently “bent over” toward the east than the west. During bent over plume conditions, the plume was attached to the eastern shoreline while having a distinct, cuspate front along its westernmost boundary. The location of the front was found to be related to the magnitude and direction of local flow during the preceding O(1 h), and increases in alongshore flow resulted in deeper freshwater mixing, stronger baroclinic anomalies, and stronger hugging of the coast. During bent over plume conditions, we observed significant convergence of river plume water toward the frontal boundary within 1 km of the river mouth. These results show how coastal topography can strongly influence buoyant plume behavior, and they should assist with understanding of initial coastal sediment dispersal pathways from the Elwha River during a pending dam removal project.  相似文献   

纳米铁还原脱氮动力学及其影响因素   总被引：3，自引：1，他引：2  

黄园英  秦臻  刘丹丹  王晓春 《岩矿测试》2011,30(1):53-58

饮用水中硝酸盐(NO3-)对人体健康有危害。为了去除水溶液中NO3-,在实验室制得纳米铁颗粒。它的粒径为20～40 nm,比表面积(BET)为49.16 m2/g。本研究通过批实验考察了纳米铁对NO3-还原脱氮动力学性质和影响NO3-脱氮快慢的主要因素,如反应pH、纳米铁投加量和NO3-起始浓度。实验结果表明,pH越低越有利于NO 3-还原。在一定范围内,NO 3-还原速率随纳米铁投加量增加而增大,而随NO 3-起始浓度升高而降低,反应遵循准一级反应动力学方程,表面吸附和氧化还原反应是纳米铁对NO3-脱氮的主要去除机理。纳米铁对NO3-还原过程中可能反应的途径进行了讨论,NO3-还原产物取决于反应条件。在本研究条件下,纳米铁对NO3-脱氮的最终产物主要为NH4+-N而不是N2,必须进行更多的研究来解决这一问题。  相似文献   

坡缕石粘土固定辣根过氧化酶处理硝基酚废水     

舒林  彭书传  刘海波  鲍腾  刘文静 《岩石矿物学杂志》2011,30(6):1063-1068

以坡缕石粘土、淀粉、水玻璃为原料,研究了固定化酶载体的制备工艺,探究了固定化酶载体在辣根过氧化酶(HRP)降解硝基酚废水中的作用,并探讨了反应时间、酶浓度、H2O2及硝基酚浓度对降解效果的影响。结果表明,固定化酶载体的最佳制备工艺为:水玻璃12%,淀粉20%,煅烧温度550℃,煅烧时间2 h;固定化酶对硝基酚的去除效果明显高于原酶;固定化酶去除水中硝基酚的最佳反应条件为:反应时间1.5 h,加酶量150 U,H2O2浓度0.12%,硝基酚浓度100 mg/L;固定化酶重复使用7次后对硝基酚的去除率仍高于60%。  相似文献   

基于混合像元分解提取多种类覆盖区遥感蚀变信息 ——以甘肃省岷县寨上金矿区为例     

陈勇敢 《地质与勘探》2011,47(6):1171-1176

在多种类覆盖区,由于植被、河道、阴影、第四系等干扰因素影响,难于客观有效提取与成矿有关的遥感蚀变信息。应用混合像元分解的方法技术可以区分出混合像元中各类干扰信息的反射率值及其所占丰度值,从混合像元光谱中减去各干扰因素的反射率值及其所占份额,可以获取土壤或岩石的反射率值及其所占丰度值,将土壤或岩石反射率值除以其所占的份额...  相似文献   

不同坡度缓冲带滞缓径流及污染物去除定量化   总被引：8，自引：0，他引：8       下载免费PDF全文

吴建强 《水科学进展》2011,22(1):112-117

利用构建的东风港缓冲带现场试验基地和设计的径流流量测定装置,模拟上海地区农业面源污染物浓度和典型单次降雨历时及降雨量,对不同坡度缓冲带滞缓径流和农田氮磷污染物去除能力开展定量化试验研究。结果表明:相同植被缓冲带,坡度越小,其滞缓径流和土壤水力渗透的能力越强,19 m长的2%坡度缓冲带径流初始出水时间比5%坡度缓冲带延长了7.3 min,两者的渗流水量比值达到1.74;不同坡度缓冲带渗流氮磷污染物去除量显著高于径流,2%、3%、4%和5%坡度缓冲带对于氮磷污染物的渗流去除量与径流去除量的比值分别为2.32、2.15、1.82和1.64;坡度的变化对缓冲带净化面源氮磷污染物效果的影响显著,坡度越小,缓冲带渗流水量越大,其氮磷污染物的总去除率和单位面积去除负荷也越高,2%坡度缓冲带对氮磷污染的总去除率和单位面积污染去除负荷分别是5%坡度的1.56倍和1.66倍,2%坡度缓冲带对TN、NH₃--N、TP的单位面积去除负荷均最高,分别达到0.661 g/m2、0.672 g/m2和0.044 g/m2。  相似文献