依兰—伊通断裂北段断层氢气的地球化学特征分析     

康健  徐岳仁  姜云爽  杜天然  马艳丽  李继业 《地震地磁观测与研究》2020,41(4):111-120

2017—2018年在依兰—伊通断裂黑龙江段开展断层氢气调查工作,沿断裂选取8个剖面进行跨目标断层观测及土壤氢气采样。结果表明：①断层氢气浓度常存在异常变化;②不同类型的断层,氢气浓度异常变化幅度没有明显差异;③走滑断层异常特征一般为断层两侧低、中间高,呈现“低—高—低”的特点;倾滑断层异常特征一般为断层的上盘略高、下盘略低;④断层氢气排放不仅受微观局部断层的影响,更受宏观的地震活动性大环境的影响。  相似文献   

Moisture origin and stable isotope characteristics of precipitation in southeast Siberia     

Svetlana S. Kostrova  Hanno Meyer  Francisco Fernandoy  Martin Werner  Pavel E. Tarasov 《水文研究》2020,34(1):51-67

The paper presents oxygen and hydrogen isotopes of 284 precipitation event samples systematically collected in Irkutsk, in the Baikal region (southeast Siberia), between June 2011 and April 2017. This is the first high-resolution dataset of stable isotopes of precipitation from this poorly studied region of continental Asia, which has a high potential for isotope-based palaeoclimate research. The dataset revealed distinct seasonal variations: relatively high δ¹⁸O (up to −4‰) and δD (up to −40‰) values characterize summer air masses, and lighter isotope composition (−41‰ for δ¹⁸O and −322‰ for δD) is characteristic of winter precipitation. Our results show that air temperature mainly affects the isotope composition of precipitation, and no significant correlations were obtained for precipitation amount and relative humidity. A new temperature dependence was established for weighted mean monthly precipitation: +0.50‰/°C (r² = 0.83; p <.01; n = 55) for δ¹⁸O and +3.8‰/°C (r² = 0.83, p < 0.01; n = 55) for δD. Secondary fractionation processes (e.g., contribution of recycled moisture) were identified mainly in summer from low d excess. Backward trajectories assessed with the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model indicate that precipitation with the lowest mean δ¹⁸O and δD values reaches Irkutsk in winter related to moisture transport from the Arctic. Precipitation originating from the west/southwest with the heaviest mean isotope composition reaches Irkutsk in summer, thus representing moisture transport across Eurasia. Generally, moisture transport from the west, that is, the Atlantic Ocean predominates throughout the year. A comparison of our new isotope dataset with simulation results using the European Centre/Hamburg version 5 (ECHAM5)-wiso climate model reveals a good agreement of variations in δ¹⁸O (r² = 0.87; p <.01; n = 55) and air temperature (r² = 0.99; p <.01; n = 71). However, the ECHAM5-wiso model fails to capture observed variations in d excess (r² = 0.14; p < 0.01; n = 55). This disagreement can be partly explained by a model deficit of capturing regional hydrological processes associated with secondary moisture supply in summer.  相似文献   

宁芜地区铁磷矿床形成机理探索   总被引：8，自引：0，他引：8  

郑大中 《安徽地质》2000,(4)

描述宁芜地区铁磷矿床的成矿机理。探讨了岩浆及热液铁、磷、钛、稀土等的搬运形式及成矿过程。结果表明,氢化物是成矿物质的主要迁移形式,它们迁移至地壳浅部被氧化成矿。  相似文献   

安徽张八岭构造带石英脉型金矿成矿流体来源研究   总被引：7，自引：1，他引：6  

黄德志  戴塔根  孔华  邱瑞龙  徐祥  王奎仁 《大地构造与成矿学》2000,24(3):231-236

对安徽张八岭构造带石英脉型金矿石英流体包裹体温度、成分和氢、氧同位素进行了研究,对成矿流体来源进行了探讨。研究表明,区内石英脉型金矿具有两类成矿流体,一类为中生代大气降水与经历水/岩交换的演化岩浆水的混合;另一类为中生代大气降水与原始岩浆水的混合。  相似文献   

四川盆地H2S的硫同位素组成及其成因探讨   总被引：23，自引：3，他引：20  

朱光有  张水昌  梁英波  戴金星 《地球化学》2006,35(4):432-442

四川盆地天然气绝大部分含有硫化氢,部分含量高达15%以上。其中高含硫化氢天然气主要分布在三叠系飞仙关组、雷口坡组和嘉陵江组;震旦系、石炭系、二叠系属于低含硫化氢,上三叠统须家河组和侏罗系属于微含硫化氢或不含硫化氢天然气藏。研究表明,三叠系飞仙关组、雷口坡组和嘉陵江组、震旦系、石炭系储层中发育的膏质岩类为TSR形成硫化氢提供了物质基础;富含有机硫源岩的高温裂解是二叠系低含硫化氢天然气的主要成因。硫同位素组成表明,高含硫化氢天然气的硫同位素比储层硫酸盐硫同位素δ34S亏损7‰～11‰;而低含硫化氢天然气硫同位素分布区间较宽,在0‰～20‰之间,大部分比同期硫酸盐的硫同位素轻15‰左右。四川盆地三叠系膏岩的硫同位素值分布较宽,并呈现阶梯状变化,而硫化氢的硫同位素则呈现出相似的分布规律,表明各气层硫化氢中的硫来自于本层系的硫酸盐,即TSR发生在各自的储集层中;另外四川盆地三叠系TSR发生时各气藏的温度条件相近,即各气藏的硫化氢在大致相同的温度条件下发生;同时也说明TSR过程中硫同位素的分馏过程与硫酸盐本身硫同位素数值的高低无关,而与TSR反应的温度条件和反应程度有关。还建立了运用硫化氢的硫同位素和含量判识硫化氢成因类型的模式。  相似文献   

Mechanisms of isotopic control of precipitation in the Yellow River source region     

Linlin Ye  Xinrui Lin  Guofeng Zhu  Yuwei Liu  Dongdong Qiu  Wenhao Zhang  Jiawei Liu  Siyu Lu 《水文研究》2024,38(2):e15087

The study of water vapour sources and water cycle patterns in the Yellow River source region is of great significance for ensuring water resource security in the arid and semi-arid regions of northern China. We established a precipitation stable isotope observation system in the Yellow River source region for three consecutive years (2020–2022), systematically analysed the spatial and temporal distribution characteristics of precipitation stable isotopes ²H and ¹⁸O in the Yellow River source region and their interrelationships with environmental factors and topography, and explored the regional water vapour transport pathways by using the HYSPLIT model and combining with the global reanalysis data. The results show that: (1) the δ¹⁸O and δ²H values of precipitation in the Yellow River source region follow the seasonal pattern, with the first half of the year being richer than the second half of the year; (2) the spatial variations of δ¹⁸O of precipitation in the Yellow River source region show a low in the southwest and a high in the northeast; (3) the water vapour source in the source area is basically stable, and the complex transport paths and the cross-effects of the local factors determine the stable isotope characteristics of the water, and the stable isotope characteristics of the water are determined by the cross-effects of the local factors, because the source of the water vapour and the local factors such as the height will not change significantly in the short term. Since the source of water vapour and local elevation factors will not change significantly in the short term, the precipitation pattern in the source area of the Yellow River can be considered to be basically stable.  相似文献   

海洋沉积物中氧化亚铁的分析测定   总被引：2，自引：0，他引：2  

郑凯清  张仲平 《岩矿测试》1999,18(3):198-200

海洋沉积物试样用Ｈ２Ｏ２－ＨＡｃ浸取,用以除去干扰测定ＦｅＯ的锰化合物和硫化珠,并以Ｈ２ＳＯ３－Ｎａ２ＳＯ３混合溶液破坏过乘的Ｈ２Ｏ２,不需过滤分离,即可用ＨＦ－Ｈ２ＳＯ４分解试样,Ｋ２Ｃｒ２Ｏ７标准溶液滴定ＦｅＯ。方法经海洋沉积物国家标准物质分析验证,结果与参考值相符,ＲＳＤ为６．３３％。  相似文献   

The Great Dun Fell Experiment 1995: an overview     

K. N. Bower  T. W. Choularton  M. W. Gallagher  R. N. Colvile  K. M. Beswick  D. W. F. Inglis  C. Bradbury  B. G. Martinsson  E. Swietlicki  O. H. Berg  S. -I. Cederfelt  G. Frank  J. Zhou  J. N. Cape  M. A. Sutton  G. G. McFadyen  C. Milford  W. Birmili  B. A. Yuskiewicz  A. Wiedensohler  F. Stratmann  M. Wendisch  A. Berner  P. Ctyroky  Z. Galambos  S. H. Mesfin  U. Dusek  C. J. Dore  D. S. Lee  S. A. Pepler  M. Bizjak  B. Divjak 《Atmospheric Research》1999,50(3-4)

During March and April of 1995 a major international field project was conducted at the UMIST field station site on Great Dun Fell in Cumbria, Northern England. The hill cap cloud which frequently envelopes this site was used as a natural flow through reactor to examine the sensitivity of the cloud microphysics to the aerosol entering the cloud and also to investigate the effects of the cloud in changing the aerosol size distribution, chemical composition and associated optical properties. To investigate these processes, detailed measurements of the cloud water chemistry (including the chemistry of sulphur compounds, organic and inorganic oxidised nitrogen and ammonia), cloud microphysics and properties of the aerosol and trace gas concentrations upwind and downwind of the cap cloud were undertaken. It was found that the cloud droplet number was generally strongly correlated to aerosol number concentration, with up to 2000 activated droplets cm⁻³ being observed in the most polluted conditions. In such conditions it was inferred that hygroscopic organic compounds were important in the activation process. Often, the size distribution of the aerosol was substantially modified by the cloud processing, largely due to the aqueous phase oxidation of S(IV) to sulphate by hydrogen peroxide, but also through the uptake and fixing of gas phase nitric acid as nitrate, increasing the calculated optical scattering of the aerosol substantially (by up to 24%). New particle formation was also observed in the ultrafine aerosol mode (at about 5 nm) downwind of the cap cloud, particularly in conditions of low total aerosol surface area and in the presence of ammonia and HCl gases. This was seen to occur at night as well as during the day via a mechanism which is not yet understood. The implications of these results for parameterising aerosol growth in Global Climate Models are explored.  相似文献   

国内外氢能发展战略及其重要意义     

王朋飞  姜重昕  马冰 《中国地质调查》2021,8(4):33-39

为应对世界气候变化并丰富能源供给手段,实现碳中和目标,世界主要发达国家和地区均在2020年制定了本国的氢能战略,将发展氢能产业提升到国家能源战略的高度,旨在于2030—2050年间完成CO2减排目标.详细介绍了世界各国的氢能发展战略、发展氢能在解决能源安全和生态安全中起到的作用、氢能制取的技术路线以及发展氢能带来的经济...  相似文献   

波流联合作用下掺氢输气海管泄漏扩散研究     

朱红钧  黄栏  高岳  唐堂 《海洋工程》2024,(3):107-118

由于氢气密度低,泄漏后的掺氢天然气在海洋波流作用下的浮升扩散行为有别于纯天然气,其泄漏扩散规律有待明晰。利用计算流体力学方法数值模拟了波流联合作用下掺氢输气海管泄漏扩散的过程,结果表明气体泄漏的过程可分为泄漏初期、向上浮升以及横向迁移3个阶段。当掺氢比φH2 <50%时,氢气泡的运动轨迹受天然气泡的影响显著。气体浮升高度和扩散直径的变化与时间成正相关,且随着掺氢比的增大,泄漏气体到达液面所需的时间延长。天然气泡和氢气泡直径在上升的过程中都逐渐增大,两者的浮升速度随浮升高度的增加先增大后减小,天然气泡的浮升速度衰减更快。氢气泡直径随掺氢量的增加而增大,天然气泡直径随掺氢量的增大而减小,两者的上升速度随着掺氢量的增大都表现出先增大后减小的趋势,且氢气泡的上升速度大于天然气泡的上升速度。波长和海流流速越大,泄漏气体的扩散直径越大。  相似文献