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101.
Chemical structure of Jurassic vitrinites isolated from the coals in basins in NW China have been checked using solid state 13C NMR and flash pyrolysis-GC/MS. Study shows some Jurassic collodetrinites are rich in aliphatic products in pyrolysates, consisting with the high amount of methylene carbon in 13C NMR spectra. In contrast, pyrolysates of Jurassic collotelinites are rich in phenols and alkylbenzenes. Also one Pennsylvanian and one Permian vitrinite selected from the Ordos basin, NW China have been checked for comparison. The proportion of aliphatics is low in pyrolysates, and aliphatic carbon peak in 13C NMR spectrum of Permian vitrinite is mostly composed of gas-prone carbons compared with collodetrinites in those Jurassic basins. But both pyrolysis and 13C NMR data shows the Pennsylvanian vitrinite is not only gas-prone but also oil-prone. Relatively high proportion of long chain aliphatic structure of some Jurassic vitrinite in Junggar, Turpan-Hami basins may be due to the contribution of liptodetrinites, which may be included during the formation of vitrinites. And it seems that suberinite is the most possible precursor of long chain aliphatics in the structure of Jurassic collodetrinite. 相似文献
102.
Supercritical gas sorption on moist coals 总被引:2,自引:1,他引:1
The effect of moisture on the CO2 and CH4 sorption capacity of three bituminous coals from Australia and China was investigated at 55 °C and at pressures up to 20 MPa. A gravimetric apparatus was used to measure the gas adsorption isotherms of coal with moisture contents ranging from 0 to about 8%. A modified Dubinin–Radushkevich (DR) adsorption model was found to fit the experimental data under all conditions. Moisture adsorption isotherms of these coals were measured at 21 °C. The Guggenheim–Anderson–de Boer (GAB) model was capable of accurately representing the moisture isotherms over the full range of relative pressures.Moist coal had a significantly lower maximum sorption capacity for both CO2 and CH4 than dry coal. However, the extent to which the capacity was reduced was dependent upon the rank of the coal. Higher rank coals were less affected by the presence of moisture than low rank coals. All coals exhibited a certain moisture content beyond which further moisture did not affect the sorption capacity. This limiting moisture content was dependent on the rank of the coal and the sorbate gas and, for these coals, corresponded approximately to the equilibrium moisture content that would be attained by exposing the coal to about 40–80% relative humidity. The experimental results indicate that the loss of sorption capacity by the coal in the presence of water can be simply explained by volumetric displacement of the CO2 and CH4 by the water. Below the limiting moisture content, the CO2 sorption capacity reduced by about 7.3 kg t− 1 for each 1% increase in moisture. For CH4, sorption capacity was reduced by about 1.8 kg t− 1 for each 1% increase in moisture.The heat of sorption calculated from the DR model decreased slightly on addition of moisture. One explanation is that water is preferentially attracted to high energy adsorption sites (that have high energy by virtue of their electrostatic nature), expelling CO2 and CH4 molecules. 相似文献
103.
Magnetotelluric investigations have been carried out in the Garhwal Himalayan corridor to delineate the electrical structure
of the crust along a profile extending from Indo-Gangetic Plain to Higher Himalayan region in Uttarakhand, India. The profile
passing through major Himalayan thrusts: Himalayan Frontal Thrust (HFF), Main Boundary Thrust (MBT) and Main Central Thrust
(MCT), is nearly perpendicular to the regional geological strike. Data processing and impedance analysis indicate that out
of 44 stations MT data recorded, only 27 stations data show in general, the validity of 2D assumption. The average geoelectric
strike, N70°W, was estimated for the profile using tensor decomposition. 2D smooth geoelectrical model has been presented,
which provides the electrical image of the shallow and deeper crustal structure. The major features of the model are (i) a low resistivity (<50Ωm), shallow feature interpreted as sediments of Siwalik and Indo-Gangetic Plain, (ii) highly resistive (> 1000Ωm) zone below the sediments at a depth of 6 km, interpreted as the top surface of the Indian plate,
(iii) a low resistivity (< 10Ωm) below the depth of 6 km near MCT zone coincides with the intense micro-seismic activity in the
region. The zone is interpreted as the partial melting or fluid phase at mid crustal depth. Sensitivity test indicates that
the major features of the geoelectrical model are relevant and desired by the MT data. 相似文献
104.
赣南崇义—大余—上犹矿集区不同类型含矿石英中白云母40Ar/39Ar年龄及其地质意义 总被引:14,自引:0,他引:14
崇义—大余—上犹矿集区是世界著名的黑钨矿床集中区,本文选择钨锡多金属硫化物石英脉型(柯树岭和漂塘矿床)和锡钨石英脉型(仙鹅塘矿床)3个矿床石英中的白云母开展40Ar/39Ar年代学研究,测得坪年龄分别是:钨锡多金属硫化物石英脉型是 158.9 ± 1.4 Ma(漂塘)、158.8 ± 1.2 Ma(柯树岭);钨锡石英脉型的是231.4 ± 2.4 Ma(仙鹅塘),在反等时线图上,其对应的截距年龄分别是158.8 ± 1.6 Ma、158.7 ± 1.9Ma和232.5 ± 2.4 Ma。由此表明,在崇余犹矿集区内存在两个不同成矿时期,即以黑钨矿为主的多金属硫化物石英脉型矿床形成于中侏罗世,集中于160~150Ma之间,与南岭地区钨锡矿床的主成矿期是一致的;而以锡石为主的,并含有大量白钨矿的石英脉型矿床可形成于印支期 相似文献
105.
赣南崇义县淘锡坑钨矿位于南岭东西向构造带东段,属于以黑钨矿石英脉型为主的钨多金属矿床。矿床形成与燕山期中酸性岩浆作用有密切关系,石英矿脉受一组北西向断裂控制,穿切新元古界。本文在淘锡坑钨矿区3个揭露到花岗岩体顶部的中段(206、106、56中段)采集到岩体顶部云英岩样品,利用40Ar/39Ar同位素定年测得云英岩中的白云母的坪年龄分别为152.7 ± 1.5 Ma(206中段),153.4 ± 1.3 Ma(106中段),155.0 ± 1.4 Ma(56中段)。与前人用其他方法测定的花岗岩成岩和成矿年龄几乎一致。花岗岩和云英岩全岩稀土元素均具有M型四分组效应和强烈的Eu亏损特征,反映出花岗质岩浆经历了高度分异演化及其岩体结晶晚期流体/熔体相互作用。综合前人在南岭地区同类矿床的研究资料,可知南岭地区160~150Ma成岩成矿作用主要分布于南岭中-东段,可能为大陆边缘弧后岩石圈伸展的构造动力学背景的产物。 相似文献
106.
Detrital zircon provides a powerful archive of continental growth and recycling processes. We have tested this by a combined laser ablation ICP-MS U–Pb and Lu–Hf analysis of homogeneous growth domains in detrital zircon from late Paleozoic coastal accretionary systems in central Chile and the collisional Guarguaráz Complex in W Argentina. Because detritus from a large part of W Gondwana is present here, the data delineate the crustal evolution of southern South America at its Paleopacific margin, consistent with known data in the source regions.Zircon in the Guarguaráz Complex mainly displays an U–Pb age cluster at 0.93–1.46 Ga, similar to zircon in sediments of the adjacent allochthonous Cuyania Terrane. By contrast, zircon from the coastal accretionary systems shows a mixed provenance: Age clusters at 363–722 Ma are typical for zircon grown during the Braziliano, Pampean, Famatinian and post-Famatinian orogenic episodes east of Cuyania. An age spectrum at 1.00–1.39 Ga is interpreted as a mixture of zircon from Cuyania and several sources further east. Minor age clusters between 1.46 and 3.20 Ga suggest recycling of material from cratons within W Gondwana.The youngest age cluster (294–346 Ma) in the coastal accretionary prisms reflects a so far unknown local magmatic event, also represented by rhyolite and leucogranite pebbles. It sets time marks for the accretion history: Maximum depositional ages of most accreted metasediments are Middle to Upper Carboniferous. A change of the accretion mode occurred before 308 Ma, when also a concomitant retrowedge basin formed.Initial Hf-isotope compositions reveal at least three juvenile crust-forming periods in southern South America characterised by three major periods of juvenile magma production at 2.7–3.4 Ga, 1.9–2.3 Ga and 0.8–1.5 Ga. The 176Hf/177Hf of Mesoproterozoic zircon from the coastal accretionary systems is consistent with extensive crustal recycling and addition of some juvenile, mantle-derived magma, while that of zircon from the Guarguaráz Complex has a largely juvenile crustal signature. Zircon with Pampean, Famatinian and Braziliano ages (< 660 Ma) originated from recycled crust of variable age, which is, however, mainly Mesoproterozoic. By contrast, the Carboniferous magmatic event shows less variable and more radiogenic 176Hf/177Hf, pointing to a mean early Neoproterozoic crustal residence. This zircon is unlikely to have crystallized from melts of metasediments of the accretionary systems, but probably derived from a more juvenile crust in their backstop system. 相似文献
107.
Development of a 3D GIS and its application to karst areas 总被引:1,自引:0,他引:1
There is a growing interest in modeling and analyzing karst phenomena in three dimensions. This paper integrates geology,
groundwater hydrology, geographic information system (GIS), database management system (DBMS), visualization and data mining
to study karst features in Huaibei, China. The 3D geo-objects retrieved from the karst area are analyzed and mapped into different
abstract levels. The spatial relationships among the objects are constructed by a dual-linker. The shapes of the 3D objects
and the topological models with attributes are stored and maintained in the DBMS. Spatial analysis was then used to integrate
the data in the DBMS and the 3D model to form a virtual reality (VR) to provide analytical functions such as distribution
analysis, correlation query, and probability assessment. The research successfully implements 3D modeling and analyses in
the karst area, and meanwhile provides an efficient tool for government policy-makers to set out restrictions on water resource
development in the area. 相似文献
108.
Quick-look assessments to identify optimal CO2 EOR storage sites 总被引:1,自引:0,他引:1
Vanessa Núñez-López Mark H. Holtz Derek J. Wood William A. Ambrose Susan D. Hovorka 《Environmental Geology》2008,54(8):1695-1706
A newly developed, multistage quick-look methodology allows for the efficient screening of an unmanageably large number of
reservoirs to generate a workable set of sites that closely match the requirements for optimal CO2 enhanced oil recovery (EOR) storage. The objective of the study is to quickly identify miscible CO2 EOR candidates in areas that contain thousands of reservoirs and to estimate additional oil recovery and sequestration capacities
of selected top options through dimensionless modeling and reservoir characterization. Quick-look assessments indicate that
the CO2 EOR resource potential along the US Gulf Coast is 4.7 billion barrels, and CO2 sequestration capacity is 2.6 billion metric tons. In the first stage, oil reservoirs are screened and ranked in terms of
technical and practical feasibility for miscible CO2 EOR. The second stage provides quick estimates of CO2 EOR potential and sequestration capacities. In the third stage, a dimensionless group model is applied to a selected set
of sites to improve the estimates of oil recovery and storage potential using appropriate inputs for rock and fluid properties,
disregarding reservoir architecture and sweep design. The fourth stage validates and refines the results by simulating flow
in a model that describes the internal architecture and fluid distribution in the reservoir. The stated approach both saves
time and allows more resources to be applied to the best candidate sites. 相似文献
109.
On CO<Subscript>2</Subscript> fluid flow and heat transfer behavior in the subsurface,following leakage from a geologic storage reservoir 总被引:1,自引:0,他引:1
Karsten Pruess 《Environmental Geology》2008,54(8):1677-1686
Geologic storage of CO2 is expected to produce plumes of large areal extent, and some leakage may occur along fractures, fault zones, or improperly
plugged pre-existing wellbores. A review of physical and chemical processes accompanying leakage suggests a potential for
self-enhancement. The numerical simulations presented here confirm this expectation, but reveal self-limiting features as
well. It seems unlikely that CO2 leakage could trigger a high-energy run-away discharge, a so-called “pneumatic eruption,” but present understanding is insufficient
to rule out this possibility. The most promising avenue for increasing understanding of CO2 leakage behavior is the study of natural analogues. 相似文献
110.
Curtis M. Oldenburg 《Environmental Geology》2008,54(8):1687-1694
A screening and ranking framework (SRF) has been developed to evaluate potential geologic carbon dioxide (CO2) storage sites on the basis of health, safety, and environmental (HSE) risk arising from CO2 leakage. The approach is based on the assumption that CO2 leakage risk is dependent on three basic characteristics of a geologic CO2 storage site: (1) the potential for primary containment by the target formation; (2) the potential for secondary containment
if the primary formation leaks; and (3) the potential for attenuation and dispersion of leaking CO2 if the primary formation leaks and secondary containment fails. The framework is implemented in a spreadsheet in which users
enter numerical scores representing expert opinions or published information along with estimates of uncertainty. Applications
to three sites in California demonstrate the approach. Refinements and extensions are possible through the use of more detailed
data or model results in place of property proxies. 相似文献