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Calcium and magnesium levels have been monitored in slope foot drainage waters on a dolomite bedrock. Both calcium and magnesium rich pulses occur. Short term dissolution experiments demonstrate high calcium levels in solution while other authors have suggested that long residence time groundwater has relatively high levels of magnesium due to calcite precipitation. Patterns of field fluctuations in Ca: Mg ratios can thus be tentatively interpreted in terms of short residence time water of high calcium content mixing with long residence time water of high magnesium content. Fluorometric dye tracing has been used to indicate the orders of magnitude of soil water residence times, suggesting that quickflow components are resident in the system for a few hours to a few days. Further work is in progress. 相似文献
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用高精度振动管在 273.15 至 308.15 K 的温度范围内以 5 K 的间隔对两个二元系统(LiCl-H2O 和 MgCl2-H2O)和三元系统(LiCl-MgCl2-H2O)的密度进行了实验测定密度计。基于 Vogel-Fulcher-Tamman (VFT) 方程,对 LiCl(aq) 和 MgCl2(aq) 密度与温度和摩尔浓度的相关方程的系数进行了参数化。 Young的理想混合规则被成功地应用于基于相关的二元解性质关联三元系统的密度。根据二元和三元体系的体积特性数据,根据 Pitzer 离子相互作用理论,得到 Pitzer 单盐参数和混合离子相互作用参数。在本工作中确定了三元体系在恒定离子强度下的混合体积 (ΔVm)。 相似文献
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《Chemie der Erde / Geochemistry》2019,79(4):125524
Due to their common occurrence in various types of chondrites, igneous rims formed on pre-existing chondrules throughout chondrule-forming regions of the solar nebula. Although the peak temperatures are thought to reach similar values to those achieved during chondrule formation events, the heating duration in chondrule rim formation has not been well defined. We determined the two-dimensional chemical and oxygen isotopic distributions in an igneous rim of a chondrule within the Northwest Africa 3118 CV3oxA chondrite with sub-micrometer resolution using secondary ion mass spectrometry and scanning electron microscopy. The igneous rim experienced aqueous alteration on the CV parent body. The aqueous alteration resulted in precipitation of the secondary FeO-rich olivine (Fa40–49) and slightly disturbed the Fe-Mg distribution in the MgO-rich olivine phenocrysts (Fa11–22) at about a 1 μm scale. However, no oxygen isotopic disturbances were observed at a scale greater than 100 nm. The MgO-rich olivine, a primary phase of igneous rim formation, has δ17O = −6 ± 3‰ and δ18O = −1 ± 4‰, and some grains contain extreme 16O-rich areas (δ17O, δ18O = ∼−30‰) nearly 10 μm across. We detected oxygen isotopic migration of approximately 1 μm at the boundaries of the extreme 16O-rich areas. Using oxygen self-diffusivity in olivine, the heating time of the igneous rim formation could have continued from several hours to several days at near liquidus temperatures (∼2000 K) in the solar nebula suggesting that the rim formed by a similar flash heating event that formed the chondrules. 相似文献
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