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81.
82.
Water-soluble organics in atmospheric particles: A critical review of the literature and application of thermodynamics to identify candidate compounds 总被引:15,自引:0,他引:15
Although organic compounds typically constitute a substantial fraction of the fine particulate matter (PM) in the atmosphere, their molecular composition remains poorly characterized. This is largely because atmospheric particles contain a myriad of diverse organic compounds, not all of which extract in a single solvent or elute through a gas chromatograph; therefore, a substantial portion typically remains unanalyzed. Most often the chemical analysis is performed on a fraction that extracts in organic solvents such as benzene, ether or hexane; consequently, information on the molecular composition of the water-soluble fraction is particularly sparse and incomplete.This paper investigates theoretically the characteristics of the water-soluble fraction by splicing together various strands of information from the literature. We identify specific compounds that are likely to contribute to the water-soluble fraction by juxtaposing observations regarding the extraction characteristics and the molecular composition of atmospheric particulate organics with compound-specific solubility and condensibility for a wide variety of organics. The results show that water-soluble organics, which constitute a substantial fraction of the total organic mass, include C2 to C7 multifunctional compounds (e.g., diacids, polyols, amino acids). The importance of diacids is already recognized; our results provide an impetus for new experiments to establish the atmospheric concentrations and sources of polyols, amino acids and other oxygenated multifunctional compounds. 相似文献
83.
利用2019年5月20日机载DMT和SPEC粒子测量系统获取的飞机云微物理探测资料,结合高空、地面、卫星云图产品等常规气象数据,分析了东北冷涡在发展成熟期的云宏微观结构特征。结果表明:飞机探测区域为冷性层积混合云,云水充沛。云粒子探头(CDP)和二维云粒子图像探头(CIP)探测到的最大粒子数浓度分别为362.10cm~(-3)、191.08L~(-1),液态含水量变化范围为0~0.88g/m~3;CDP粒子谱呈指数型下降,谱宽较窄;CIP粒子谱呈双峰结构。云粒子图像探测仪CPI表明,层积云上部主要为冰雪晶粒子,以冰晶的核化和凝华增长为主;中上部粒子主要为小冰晶形态,也有冰晶聚合体和枝状冰晶;中下部是过冷水和冰晶粒子的共存区,过冷水较为丰富。 相似文献
84.
85.
Magnetic properties of tidal flat sediments of the Yangtze Estuary and its relationship with particle size 总被引:6,自引:0,他引:6
Since the 1970s, environmental magnetism has found extensive applications in diverse research areas of geoscience[1]. In China, a lot of environmental magnetic studies have been carried out on loess, lake and marine sediments for the purpose of paleoclima… 相似文献
86.
A numerical model based on smoothed particle hydrodynamics (SPH) was developed and used to simulate immiscible and miscible fluid flows in porous media and to study effects of pore scale heterogeneity and anisotropy on such flows. 相似文献
87.
P. I. A. Kinnell 《地球表面变化过程与地形》2006,31(3):355-367
Rain‐impacted flows dominate sheet and interrill erosion and are important in eroding soil rich in nutrients and other chemicals which may have deleterious effects on water quality. Erosion in rain‐impacted flow is associated with raindrop detachment followed by transport either by the combination of flow velocity and raindrop impact (raindrop‐induced flow transport, RIFT) or the inherent capacity of the flow to transport detached material. Coarse particles tend to be transported by RIFT, while fine particles tend to be transported without any assistance from raindrop impact. Because the transport process associated with coarse particles is not 100 per cent efficient, it generates a layer of loose particles on the soil surface and this layer protects the underlying soil from detachment. Simulations were performed by modelling the uplift and downstream movement of both fine and coarse particles detached from the soil surface by individual raindrop impacts starting with a surface where no loose material was present. The simulations produced a flush of fine material followed by a decline in the discharge of fine material as the amount of loose material built up on the bed. The decline in the discharge of fine material was accompanied by an increase in the discharge of coarse material. The relative amounts of coarse and fine material discharged in the flow varied with flow velocity and cohesion in the surface of the soil matrix. The results indicate that the discharge of various sized sediments is highly dependent on local soil, rain and flow conditions and that extrapolating the results from one situation to another may not be appropriate. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
88.
89.
水敏现象在石油、岩土和环境工程等领域广泛存在。有效地控制水敏现象的发生,不仅具有科学意义,还有一定的经济价值。本文在广泛查阅国内外研究成果的基础上,总结了水敏性在石油、岩土和环境工程方面应用的研究进展,并在此基础上提出了水敏性研究的发展方向。 相似文献
90.
An approximate analytical solution for the deposition of heavy particles released from an elevated line source 总被引:1,自引:1,他引:1
This work re-examines and further develops an analytical solution for the deposition swath of heavy particles released in
the atmosphere from an elevated source over uniform terrain, correcting the particle diffusivity for the crossing trajectory
effect. The revised (approximate) analytical solution proves to be accurate within 20% over a wide range of micrometeorological
conditions and particle size, despite its neglect of the turbulence component of the deposition flux. It compares very satisfactorily
with experimental data and with the simulations of a Lagrangian stochastic model, provided the variable U(H)/w
g
≤7 (ratio of the mean horizontal wind speed at source height to the particle settling velocity). In this domain of validity,
simple formulae relating the statistics of the deposition swath to U(H)/w
g
are derived. 相似文献