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11.
从234Th的固/液分配看海洋胶体的作用 总被引：8，自引：2，他引：6
1994—1995年期间,利用β计数法实测了南沙群岛海域、南海东北部海域、厦门湾塔角附近海域和九龙江河口区共计116份海水样品中溶解态与颗粒态234Th的放射性比活度。结果表明,颗粒态234Th占总34Th的份额大小顺序为：九龙江河口区＞厦门海塔角附近海域＞南沙海域。南海东北部海域。234Th的条件分配系数Kd介于1．1×104—20×106dm3／kg之间,平均为2．2×105dm3／kdKd与总悬浮颗粒物含量（7SAN呈负相关关系：lg（Kd）＝－0．59·lg（TSM）＋5．67,这一“颗粒物浓度效应”可归因于海洋胶体物质的存在。由上述关系获得4个研究海区胶体浓度与悬浮颗粒物浓度的函数关系：Cc＝f（TSM0．59）。 相似文献
12.
厦门湾水体中铀、钍同位素及悬浮颗粒物的粒径谱--颗粒物采集方法的影响 总被引：2，自引：0，他引：2
运用增强型混合纤雏素(CN-CA)膜、聚碳酸酯膜和聚丙烯滤芯过滤3种不同的方法采集、研究厦门湾水体中悬浮颗粒物(SPM)及其U、Th同位素的粒径谱．发现3种方法所得SPM总浓度和U、Th各同位素的总比活度具有很好的一致性,但粒级分布存在差异．SPM的浓度随粒径的增大而增加,并且SPM的粒径谱控制着颗粒活性很强的4种钍同位素的拉径谱．对于所研究的3种方法,采用聚碳酸脂膜过滤是研究沿岸海域SPM及颗粒活性核素粒级分布比较理想的方法。 相似文献
13.
九龙江河口区水体中238U、234Th地球化学行为的研究 总被引：5，自引：2，他引：5
对采自九龙江河口区盐度介于0～21.97的10个表层水样,铀、钍同位素的测定结果表明,九龙江河口区水体中溶解态的238U含量与盐度之间存在着良好的相关关系,其相关系数可达0.972,表明九龙江河口区水体中的238U呈现保守行为.当S=0时,溶解态234U/238U放射性比值为1.19和1.55(两份水样);而当S=0.90～21.97时,该比值=1.02～1.14,分别呈现河水及河口水铀同位素组成的特征.对于颗粒态铀,其238U含量则介于0.50～9.83×10-3Bq/dm3,且随盐度的增大而呈逐步降低的趋势.九龙江河口区水体中234Th的地球化学行为属于非保守行为,不可逆稳态清除模型计算的结果表明,当盐度介于9.76～17.07时,234Th相对于化学清除的停留时间为6～19d,远低于盐度为0和21.97所对应的停留时间(分别为203d及117d),反映了在该盐度范围内,胶体絮凝沉降对溶解态234Th的快速清除作用. 相似文献
14.
厦门湾水体中不同粒级颗粒物、Chl-a和234Th随潮汐的变化及其海洋学意义 总被引：3，自引：0，他引：3
在沿岸海域——厦门湾的定点观测站,研究了不同粒径悬浮颗粒物(SPM)、Chl-a和^234Th随潮汐的变化,结果表明,不管采样深度和粒级大小,Chl-a浓度的潮汐变化均为高潮大于低潮．SPM浓度的潮汐变化,表层的规律性很明显,即不管是第一天还是第二天,也不管粒径的大小,SPM浓度无例外地呈现高潮小于低潮之势．从不同粒径SPM、Chl-a的潮汐变化的比较可以看出,浮游植物等生源颗粒物在该研究水域的颗粒物中所占比例很小,颗粒物主要来自九龙江河流输入的悬浮物和表层沉积物的再悬浮．在沿岸海域,颗粒态^234Th是总^234Th的主要组成部分,^234Th各粒级的比活度均呈现高潮大于低潮的普遍趋势,基于^234Th估算的沿岸POC、PON等输出通量也存在潮汐变化的影响．文中对上述研究对象随潮汐变化的原因作了分析和讨论． 相似文献
15.
厦门湾水体中颗粒有机碳的垂向输出通量:234Th/238U不平衡的应用 总被引：2，自引：1，他引：2
对厦门湾塔角附近海域某站位叶绿素 a、POC、初级生产力、234Th/238U不平衡进行的周日变化研究表明,POC含量介于14.4～34.6 mmol/m3之间,其中碎屑有机碳与活体有机碳所占份额分别为74%～92%和8%～26%.POC垂直分布呈现由表及底降低的趋势,且白昼期间POC含量高于晚间,说明研究海域POC含量与生物过程具有密切联系.初级生产力水平在1d之中变化达5倍,垂直分布亦随深度增加而降低,与叶绿素a的变化相对应.短时间(2h)培养获得的初级生产力水平明显高于长时间培养(24 h)的结果,证实部分新固定的碳被优先呼吸排出.结合234Th/238U不平衡法获得的颗粒态234Th输出通量及输出界面颗粒物中的POC/PTh比值,可计算出真光层 POC的垂向输出通量为16.0mmol/(m2·d),其中碎屑有机碳与活体有机碳贡献的数量分别为13.3和2.7mmol/(m2·d).POC输出通量与初级生产力的比值(ThE比值)平均为0.31,真光层POC停留时间平均为11d.上述结果与Aksnes和Wassmann[1]的模型计算结果相吻合,但与其他大多数模型的结果仍存在一定的差异. 相似文献
16.
In the present study, we report N_2 fixation rate(~(15)N isotope tracer assay) and the diazotroph community structure(using the molecular method) in the western tropical North Pacific Ocean(WTNP)(13°–20°N, 120°–160°E). Our independent evidence on the basis of both in situ N_2 fixation activity and diazotroph community structure showed the dominance of unicellular N_2 fixation over majority of the WTNP surface waters during the sampling periods.Moreover, a shift in the diazotrophic composition from unicellular cyanobacteria group B-dominated to Trichodesmium spp.-dominated toward the western boundary current(Kuroshio) was also observed in 2013. We hypothesize that nutrient availability may have played a major role in regulating the biogeography of N_2 fixation.In surface waters, volumetric N_2 fixation rate(calculated by nitrogen) ranged between 0.6 and 2.6 nmol/(L·d) and averaged(1.2±0.5) nmol/(L·d), with 10 μm size fraction contributed predominantly(88%±6%) to the total rate between 135°E and 160°E. Depth-integrated N_2 fixation rate over the upper 200 m ranged between 150 μmol/(m~2·d)and 480 μmol/(m~2·d)(average(225±105) μmol/(m~2·d). N_2 fixation can account for 6.2%±3.7% of the depthintegrated primary production, suggesting that N_2 fixation is a significant N source sustaining new and export production in the WTNP. The role of N_2 fixation in biogeochemical cycling in this climate change-vulnerable region calls for further investigations. 相似文献
17.
楚科奇和西伯利亚陆架颗粒有机物的来源：碳、氮同位素的线索 总被引：2，自引：1，他引：1
The stable isotopic composition(δ~(13)C and δ~(15)N) and carbon/nitrogen ratio(C/N) of particulate organic matter(POM) in the Chukchi and East Siberian shelves from July to September, 2016 were measured to evaluate the spatial variability and origin of POM. The δ~(13)C_(POC) values were in the range of -29.5‰ to-17.5‰ with an average of -25.9‰±2.0‰, and the δ~(15)N_(PN) values ranged from 3.9‰ to 13.1‰ with an average of 8.0‰±1.6‰. The C/N ratios in the East Siberian shelf were generally higher than those in the Chukchi shelf, while the δ~(13)C and δ~(15)N values were just the opposite. Abnormally low C/N ratios(4), low δ~(13)C_(POC)(almost-28‰) and high δ~(15)N_(PN)(10‰) values were observed in the Wrangel Island polynya, which was attributed to the early bloom of small phytoplankton. The contributions of terrestrial POM, bloom-produced POM and non-bloom marine POM were estimated using a three end-member mixing model. The spatial distribution of terrestrial POM showed a high fraction in the East Siberian shelf and decreased eastward, indicating the influence of Russian rivers. The distribution of non-bloom marine POM showed a high fraction in the Chukchi shelf with the highest fraction occurring in the Bering Strait and decreased westward, suggesting the stimulation of biological production by the Pacific inflow in the Chukchi shelf. The fractions of bloom-produced POM were highest in the winter polynya and gradually decreased toward the periphery. A negative relationship between the bloom-produced POM and the sea ice meltwater inventory was observed, indicating that the net sea ice loss promotes early bloom in the polynya.Given the high fraction of bloom-produced POM, the early bloom of phytoplankton in the polynyas may play an important role on marine production and POM export in the Arctic shelves. 相似文献
18.
Bacterial productivity was measured using 3H-thymidine methods in the Prydz Bay and its adjacent waters in the Southern Ocean during the 16th National Antarctic Research Expedition of China (CHINARE). The results showed that bacterial productivity in our study areas ranged from 4.5 to 191 ngC·dm -3·h -1, with an average of 50.4 ngC·dm -3·h -1. These values were comparable to those reported for the Ross Sea. The mean ratio of bacterial productivity to primary productivity in our study areas was 41%. The general characteristics in the vertical profiles showed a subsurface maximum at most of the stations, which was also consistent with those observed in the other sea areas in the Southern Ocean. The spatial distribution of bacterial productivity and dissolved organic carbon in the surface waters showed that their variations were inversely correlative. The relationship among bacterial productivity, primary productivity and dissolved organic carbon suggested that bacterial productivity in the Prydz Bay and its adjacent water was influenced mostly by phytoplankton activities and the hydrologic conditions. 相似文献
19.
对南沙海域表层水中溶解态(<0.45 mm)和颗粒态(>0.45 mm)210Po和210Pb进行了研究. 结果表明, 南沙海域表层水中溶解态和颗粒态210Po平均比活度分别为0.61 Bq/m3(n = 24)和0.43 Bq/m3 (n = 23). 溶解态和颗粒态210Pb 平均比活度分别为1.66 Bq/m3 (n = 24)和0.23 Bq/m3(n = 23). 颗粒态210Pb比活度约占总210Pb比活度的12%, 与开阔大洋相应值吻合; 而颗粒态210Po占总210Po的比例约40%, 明显高于开阔大洋和富营养海域. 根据稳态不可逆模型得到总210Po和210Pb的停留时间分别为0.82 和1.16 a. 清除过程中210Po和210Pb的平均分馏因子由清除速率常数法和固-液分配系数法计算分别为5.42和6.69, 揭示了210Po和210Pb从溶解相清除至颗粒相的过程中发生了明显的分馏. 进一步的研究证明了南沙海域210Po和210Pb的分馏主要由微生物控制, 与富营养海域的分馏机制不同: 在富营养海域, 浮游植物颗粒和粪粒充当210Po和210Pb清除和迁出过程的主要载体, 210Po和210Pb的分馏主要发生于浮游植物颗粒和粪粒对两核素的清除过程; 在寡营养南沙海域, 由于浮游植物颗粒和粪粒的相对贫乏, 使微生物对210Po的清除作用相对突出, 并在此过程中使210Po和210Pb产生明显的分馏效应. 这与寡营养的马尾藻海的研究结果极为相似, 进一步证实寡营养海域和富营养海域210Po生物地球化学行为和循环路径的差异. 这表明210Po可能是研究与微生物有关的海洋学过程, 尤其是研究硫族元素(S, Se, Te和Po)生物地球化学循环的有用示踪剂. 相似文献
20.