The land-use projections and resulting emissions in the IPCC SRES scenarios scenarios as simulated by the IMAGE 2.2 model   总被引：1，自引：0，他引：1  

Bart?StrengersEmail author  Rik?Leemans  Bas?Eickhout  Bert?de?Vries  Lex?Bouwman 《GeoJournal》2004,61(4):381-393

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Measurements of stable carbon isotopic composition of ethane and propane over the western North Pacific and eastern Indian Ocean: A useful indicator of atmospheric transport process     

Hideki Nara  Sakae Toyoda  Naohiro Yoshida

《Journal of Atmospheric Chemistry》2007,56(3):293-314

Stable carbon isotopic composition of ethane and propane over the western North Pacific and eastern Indian Ocean between 31°N and 26°S was investigated from February through March 2004. The isotopic composition of ethane ranged from −28 to −18‰ and showed a gradual increase from north to south. Conversely, that of propane was between −31 and −24‰; it showed no systematic latitudinal variation. Investigation of the ethane/propane ratio indicates that ethane and propane that originated from northern mid-latitude countries in the eastern part of Eurasia were both transported into the western North Pacific region. However, the results of the isotopic analyses indicate the contribution of oceanic emission to the atmospheric propane during transport, although that contribution can not be discerned for ethane. A ship based stationary observation conducted in the western equatorial North Pacific showed that the isotopic composition of ethane varied from −25 to −19‰ and showed clear systematic diurnal variation: propane ranged between −32 to −26‰ and no such isotopic diurnal signal was observed. The diurnal variation for ethane is explained by entrainment of free tropospheric air, whereas the variation for propane was influenced by oceanic emissions as well as the entrainment. The contribution of oceanic emissions to the atmospheric propane inventory was considered from our isotopic observation. Isotopic composition of dissolved propane is estimated to be less than −38‰, and the contribution up to 79% was calculated when the isotopic composition of dissolved propane is assumed to be −40‰. Our study demonstrates that isotopic analysis can be more useful than ratio-based analysis to improve our present understanding of transport processes, especially for impact of the oceanic emissions on the atmospheric distribution of low level C₂–C₅ non-methane hydrocarbons such as propane in the remote marine atmosphere.  相似文献   

On the Retrieval of Volcanic Sulfur Dioxide Emissions from GOME Backscatter Measurements     

W. Thomas  T. Ruppert  M. Van Roozendael  J. Verdebout  D. Balis  C. Meleti  C. Zerefos 《Journal of Atmospheric Chemistry》2005,50(3):295-320

We focus on the retrieval of volcanic sulfur dioxide (SO₂) emissions from an analysis of atmospheric UV backscatter spectra obtained by the Global Ozone Monitoring Experiment (GOME) spectrometer on board the ESA European Remote Sensing Satellite (ERS-2). Here, the last major eruptions of Mt. Etna on Sicily (Italy) in July/August 2001 and October/November 2002 provided an excellent opportunity to study the retrieval of SO₂ columnar amounts from ground-based, LIDAR and satellite measurements. Our study shows that the bulk of emitted SO₂ was confined in the troposphere, mainly between 700 hPa and 400 hPa which is confirmed by trajectory analysis, by LIDAR observations and AVHRR observations. The area of influence of Mt. Etna eruptions ranges from the Western Saharan Desert to Greece and the near east states and even down to the basin of Tschad, Africa. Our analysis revealed that information about the plume height of volcanic eruptions and aerosol parameters is necessary for a reliable quantitative retrieval of SO₂ from space-borne sensor data at periods perturbed by volcanic eruptions.  相似文献   

Thermal infrared remote sensing of volcanic emissions using the moderate resolution imaging spectroradiometer   总被引：1，自引：0，他引：1  

I. M. Watson  V. J. Realmuto  W. I. Rose  A. J. Prata  G. J. S. Bluth  Y. Gu  C. E. Bader  T. Yu 《Journal of Volcanology and Geothermal Research》2004,135(1-2):75

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NOx or VOC Limitation in East German Ozone Plumes?     

O. Klemm  W. R. Stockwell  H. Schlager  M. Krautstrunk 《Journal of Atmospheric Chemistry》2000,35(1):1-18

The ozone forming potential of VOCs and NO_x for plumes observed from several cities and a power plant in eastern Germany was investigated. A closed box model with a gas phase photochemical reaction mechanism was employed to simulate several scenarios based upon aircraft observations. In several of the scenarios, the initial concentrations of NO_x, VOCs, and SO₂, were reduced to study the factors limiting the O₃ production. Ozone production was limited by the initial VOC concentrations for all of the simulated plumes. Higher O₃ concentrations were produced with reduced initial NO_x. In one sample with high SO₂ mixing ratios (>100 ppb), SO₂ was also identified as a significant contributor to the production of O₃.  相似文献   

Methane exchange between coal-bearing basins and the atmosphere: the Ruhr Basin and the Lower Rhine Embayment, Germany   总被引：1，自引：0，他引：1  

Thomas Thielemann  Andreas Lücke  Gerhard H. Schleser  Ralf Littke   《Organic Geochemistry》2000,31(12):121

A precise knowledge of methane exchange processes is required to fully understand the recent rise of atmospheric methane concentration. Three of these processes take place at the lithosphere/atmosphere boundary: bacterial consumption of methane and emission of bacterial or thermogenic methane. This study was initiated to quantify these processes on a regional scale in the Ruhr Basin and the Lower Rhine Embayment. Since these areas are subject to bituminous coal and lignite mining, natural and anthropogenically-induced methane exchange processes could be studied. The methane emission and consumption rates and their carbon isotope signal were measured at the lithosphere/atmosphere boundary using flux chambers. On most of the soils studied, methane consumption by bacteria was identified. Thermogenic methane was released only at some of the natural faults examined. In active and abandoned bituminous coal mining areas methane emissions were restricted to small areas, where high emission rates were measured. The carbon isotope composition of methane at natural faults and in mining subsidence troughs was typical of thermogenic methane (−45 to −32 ‰ δ¹³C). Methane exchange balancing revealed that natural methane emissions from these two basins represent no source of atmospheric importance. However, methane release by upcast mining shafts dominates the methane exchange processes and is by about two orders of magnitude greater than methane consumption by bacterial oxidation in the soils.  相似文献   

Magnetic quantification of urban pollution sources in atmospheric particulate matter   总被引：9，自引：0，他引：9  

S. Spassov  R. Egli  F. Heller  D. K. Nourgaliev  J. Hannam 《Geophysical Journal International》2004,159(2):555-564

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长江三角洲碳排放与植被覆盖耦合协调时空格局及影响因素分析     

刘崇刚  孙伟  张落成 《地理科学》2023,43(1):142-151

通过构建评价指标体系和分析框架,利用综合指数法、耦合协调度模型和灰色关联度模型分析2005―2017年长江三角洲（长三角）碳排放与植被固碳耦合协调时空变化特征及驱动因素,并模拟政府决策优先级对耦合协调度趋势的影响。结果表明：长三角碳排放空间集聚特征显著,基本形成了以长江沿线和长三角东南沿海区域为核心的沿江沿海高排放带;长三角碳排放与植被固碳耦合协调度具有明显的空间分异特征,呈现出南京-上海沿线一般失调区域为核心的圈层结构特征;植被覆盖综合评价值高于碳排放综合评价值的地区耦合协调度普遍较高,人口的集聚和变化、城市建设和能源消耗对耦合协调度影响最大;同时,政府决策的优先级会显著影响耦合协调趋势。  相似文献   

The marker quantification of the Shared Socioeconomic Pathway 2: A middle-of-the-road scenario for the 21st century     

《Global Environmental Change》2017

Studies of global environmental change make extensive use of scenarios to explore how the future can evolve under a consistent set of assumptions. The recently developed Shared Socioeconomic Pathways (SSPs) create a framework for the study of climate-related scenario outcomes. Their five narratives span a wide range of worlds that vary in their challenges for climate change mitigation and adaptation. Here we provide background on the quantification that has been selected to serve as the reference, or ‘marker’, implementation for SSP2. The SSP2 narrative describes a middle-of-the-road development in the mitigation and adaptation challenges space. We explain how the narrative has been translated into quantitative assumptions in the IIASA Integrated Assessment Modelling Framework. We show that our SSP2 marker implementation occupies a central position for key metrics along the mitigation and adaptation challenge dimensions. For many dimensions the SSP2 marker implementation also reflects an extension of the historical experience, particularly in terms of carbon and energy intensity improvements in its baseline. This leads to a steady emissions increase over the 21st century, with projected end-of-century warming nearing 4 °C relative to preindustrial levels. On the other hand, SSP2 also shows that global-mean temperature increase can be limited to below 2 °C, pending stringent climate policies throughout the world. The added value of the SSP2 marker implementation for the wider scientific community is that it can serve as a starting point to further explore integrated solutions for achieving multiple societal objectives in light of the climate adaptation and mitigation challenges that society could face over the 21st century.  相似文献   

区域碳排放转移的演变特征与结构分解及减排对策分析——以河南省为例   总被引：2，自引：1，他引：1  

钟章奇  吴乐英  陈志建  何凌云 《地理科学》2017,37(5):773-782

通过耦合投入产出分析方法和结构分解模型,探讨2002~2010年区域碳排放转移的演变特征、驱动因素及其地理源特征。研究发现：2002~2010年流出和流入河南省的贸易隐含碳排放均处于不断增加的趋势,其中流出贸易隐含碳排放主要是受外部最终需求的影响,且主要集中在中国的中部和东南部地区,而流入贸易隐含碳排放则主要是受本地最终需求和本地最终产品结构的影响最为显著,且主要来源于中国的东部、东北部和中部地区。研究还发现,为减轻贸易对区域碳排放及其减排责任的影响,开展区域合作来共同减排比单个地区独自应对更为有利,但在区域合作中各地区的获益程度可能会有所差别。  相似文献