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AbstractThe impact of Brown Carbon (BrC) to aerosol light absorption has been paid more attention recently and there are a large number of studies showing that the influence of BrC on radiative forcing should not be ignored. BrC also acts as an important component of haze pollution which is occurring frequently in Wuhan, China. Therefore, it is essential to estimate their optical properties, composition, and mass concentration. Considering most haze pollution happens during the coldest time, we retrieved BrC columnar content during winter in Wuhan for the first time. Our method bases on the fact that BrC showed the strong spectral dependence on UV-light absorption. Using this method, we found that BrC makes up the small proportions of total aerosol volume (less than 10%). In the winter of 2011, we retrieved the daily-averaged columnar-integrated mass concentration of BrC on clear day is 4.353 mg/m2 while that of haze day is 12.750 mg/m2. According to the sensitivity study, we found that the results highly relied on the assumed aerosol refractive index. To reduce the uncertainty of this approach, we need to gain a better understanding of the temporal variability of the radiation absorbing components of these aerosols in the future. 相似文献
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Black carbon aerosols and their radiative properties in the Pearl River Delta region 总被引：13，自引：0，他引：13
Dui Wu JieTai Mao XueJiao Deng XueXi Tie YuanHang Zhang LiMin Zeng Fei Li HaoBo Tan XueYan Bi XiaoYing Huang Jing Chen Tao Deng 《中国科学D辑(英文版)》2009,52(8):1152-1163
The climatic and environmental effects of atmospheric aerosols are a hot topic in global science community, and radiative
properties of the aerosols are one of the important parameters in assessing climatic change. Here we studied the black carbon
concentration and absorption coefficient measured with aethalometers, scattering coefficient measured with nephelometers,
and single scattering albedo derived at an atmospheric composition watch station in Guangzhou from 2004 to 2007. Our main
results are as follows. The data of black carbon concentration and absorption coefficients measured with instruments cannot
be directly used until they are measured in parallel with internationally accepted instruments for comparison, calibration,
and reduction. After evaluation of the data, the result shows that the monthly mean of BC concentration varies 3.1–14.8 μg·m−3 and the concentration decreases by about 1 μg·m−3 in average over the four years; It is higher in the dry season with a multi-year mean of 8.9 μg/m3 and lower in the rainy season with a multi-year mean of 8.0 μg·m−3; The extreme maximum of monthly mean concentration occurred in December 2004 and extreme minimum in July 2007, and a 4-year
mean is 8.4 μg·m−3. It is also shown that monthly mean scattering coefficient derived varies 129 −565 Mm−1, monthly mean absorption coefficient 32–139 Mm−1, and monthly mean single scattering albedo 0.71–0.91, with annual mean values of 0.80, 0.82, 0.79 and 0.84 for 2004, 2005,
2006 and 2007, respectively. Three instruments were used to take simultaneous measurements of BC in PM10, PM2.5, and PM1 and the results showed that PM2.5 took up about 90% of PM10 and PM1 accounted for about 68% of PM2.5, and BC aerosols are mainly present in fine particulates. The variability of BC concentrations is quite consistent between
the Nancun station (141 m above sea level) and the Panyu station (13 m above sea level), which are 8 km apart from each other.
The concentration in higher altitude station (Panyu) is consistently lower than the lower altitude station (Nancun), and the
difference of annual mean is about 4 μg·m−3.
Supported by Natural Science Foundation of China (Grant Nos. U0733004, 40375002, 40418008, 40775011), National High Technology
R & D Program of China (Grant Nos. 2006AA06A306 and 2006AA06A308) and National Basic Research Program of China (Grant No.
2005CB422207) 相似文献
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河套断陷带主要活动断裂最新地表破裂事件与历史大地震 总被引：9，自引：4，他引：5
对于历史记录的公元849年大地震的发震构造尚存在一定争议,公元前7年大地震是否发生在河套断陷带,也没有得到确认。通过影像解译、野外地质地貌调查和探槽开挖,结合14C和单颗粒OSL测年,利用构造地貌分析及古地震手段,对大青山山前断裂、乌拉山山前断裂及狼山山前断裂的最新破裂事件进行了对比研究。为了尽可能降低古地震定年的不确定性,采取了序列采样、重点层位多采样等措施。结合以往研究成果认为,大青山山前断裂应为公元849年大地震的发震构造,而狼山山前断裂最近1次地震破裂事件可能与公元前7年大地震有关。 相似文献
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Analysis of South Asian Monsoons within the Context of Increasing Regional Black Carbon Aerosols 
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下载免费PDF全文 South Asian monsoons were analyzed within the context of increasing emissions of black carbon(BC) aerosols using a global atmospheric general circulation model.The BC aerosols were allowed to increase only over the south Asian domain to analyze the impacts of regional black carbon over the climatological patterns of monsoons.The black carbon significantly absorbed the incoming short wave radiation in the atmosphere,a result that is consistent with previous studies.Pre-monsoon(March-April-May) rainfall showed positive anomalies,particularly for some coastal regions of India.The summer(June-July-August) rainfall anomalies were negative over the northern Himalayas,Myanmar,southern China,and most of the regions below 20°N due to the decrease in temperature gradients induced by the absorption of radiation by BC aerosols.The vertical wind speed anomalies indicated that these regions experienced less convection,which reduces the precipitation efficiency of the monsoon system in South Asia. 相似文献
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乌鲁木齐大气黑碳气溶胶浓度变化特征及影响因素分析 总被引：1，自引：0，他引：1
刘新春 《沙漠与绿洲气象(新疆气象)》2013,7(3):36-42
利用乌鲁木齐大气成分观测站2009年11月—2010年2月(2009年冬季)黑碳气溶胶(BC)质量浓度观测资料,同时结合该站观测的PM数据以及国内外其它地区的BC观测结果,分析了该地区黑碳气溶胶的变化特征及影响因素。结果表明:(1)BC日平均浓度为12.442±5.407μg.m-3,其变化范围为2.685~26.691μg.m-3。BC质量浓度与API指数的变化趋势基本一致,相关系数为0.660。(2)BC浓度的日变化具有明显的双峰值特征,其峰值区主要出现在上午和夜间,谷值区出现在凌晨和下午。逐日分布具有2~3 d到数天不等的急剧上升的变化,与天气过程活动周期基本吻合。(3)周一至周四BC平均浓度呈总体降低趋势,周五开始逐渐增加,总体的变化幅度不大,工作日和周末差别较小。(4)BC小时平均浓度出现频数符合对数正态分布,冬季本底浓度为6.146μg.m-3。(5)BC与PM10,PM2.5,PM1.0日平均浓度在0.001水平上均呈正相关,线性相关系数分别为0.526,0.538和0.548;BC在PM10,PM2.5,PM1.0中分别约占6.8%,8.2%和9.2%,表明BC是PM的重要组成部分。(6)乌鲁木齐城市冬季BC气溶胶浓度高于国内外部分城市,明显高于较为洁净的边远地区,远高于瓦里关本底站及南极观测的结果。 相似文献