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华北地区一次强灰霾污染的天气学效应 总被引：2，自引：1，他引：1
利用在线耦合的大气化学模式WRF-Chem V3.6(Weather Research Forecasting Model with Chemistry Version 3.6)及环境、气象观测数据,在完成大气化学方案优选的基础上,研究了华北地区一次重霾污染过程(2013年2月15~17日)对气象条件的反馈作用。重点关注一次颗粒物、无机气态成分和挥发性有机污染物的人为排放对PM2.5(空气动力学当量直径小于等于2.5μm的颗粒物,即细颗粒物)生成的贡献,探讨了由此引发的气象条件的变化。模拟结果显示,上述3种人为源的综合排放对华北地区PM2.5浓度的平均贡献率为91.27%,其中对北京、秦皇岛和沧州的贡献率分别达96.9%、95.9%和97.2%。这使区域地面太阳向下短波辐射降低近15.99%,区域平均地面辐射强迫达-26.51 W m-2,由此导致地面温度下降0.14°C(3.68%),逆温增强,垂直温度梯度(?T/?z)升高0.026 K km-1,边界层高度降低18.92 m(8.77%),平均风速减少约0.014 m s-1(0.35%),相对湿度绝对值升高0.51%,地面平均气压降低0.86 Pa。对于15~17日污染过程,人为源综合排放的气溶胶对短波辐射的影响在天气过程中占主导地位,对边界层高度的影响较大,但不起主导作用,对温度、风速、相对湿度、气压的作用则远小于天气系统本身。挥发性有机污染物(Volatile Organic Compounds,VOCs)作为二次有机气溶胶(Secondary Organic Aerosol,SOA)的前体物,其人为排放对SOA浓度的贡献率约为99.6%。同时,VOCs通过调整大气反应活性促进无机气态成分向无机盐转化,它对硫酸盐和硝酸盐浓度的贡献达50%以上。然而,VOCs对整个PM2.5浓度的贡献不及各种源综合贡献的1/4。人为排放的VOCs对气象场的反馈与综合排放的作用基本一致,但对地面气压的影响VOCs排放时以热力因子为主,而人为源综合排放时以动力因子为主。上述结果暗示,灰霾污染过程所引发的气象条件向不利于污染物扩散方向改变,这可能促进污染物的局地累积、增强污染程度并延长区域内重污染的持续时间。因此,在探讨区域性灰霾污染成因时,灰霾自身通过辐射强迫作用对大气的调节是不可忽视的重要影响因素。 相似文献
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In this paper,the RIEMS 2.0 model,source emission in 2006 and 2010 are used to simulate the distributions and radiative effects of different anthropogenic aerosols over China.The comparison between the results forced by source emissions in 2006 and 2010 also reveals the sensitivity of the radiative effects to source emission.The results are shown as follows:(1) Compared with those in 2006,the annual average surface concentration of sulfate in 2010 decreased over central and eastern China with a range of-5 to 0 μg/m~3;the decrease of annual average aerosol optical depth of sulfate over East China varied from 0.04 to 0.08;the annual average surface concentrations of BC,OC and nitrate increased over central and eastern China with maximums of 10.90,11.52 and 12.50μg/m~3,respectively;the annual aerosol optical depths of BC,OC and nitrate increased over some areas of East China with extremes of 0.006,0.007 and 0.008,respectively.(2)For the regional average results in 2010,the radiative forcings of sulfate,BC,OC,nitrate and their total net radiative forcing at the top of the atmosphere over central and eastern China were-0.64,0.29,-0.41,-0.33 and-1.1 W/m~2,respectively.Compared with those in 2006,the radiative forcings of BC and OC in 2010 were both enhanced,while that of sulfate and the net radiative forcing were both weakened over East China mostly.(3)The reduction of the cooling effect of sulfate in 2010 produced a warmer surface air temperature over central and eastern China;the maximum value was 0.25 K.The cooling effect of nitrate was also slightly weakened.The warming effect of BC was enhanced over most of the areas in China,while the cooling effect of OC was enhanced over the similar area,particularly the area between Yangtze and Huanghe Rivers.The net radiative effect of the four anthropogenic aerosols generated the annual average reduction and the maximum reduction were-0.096 and-0.285 K,respectively,for the surface temperature in 2006,while in 2010 they were-0.063 and-0.256 K,respectively.In summary,the change in source emission lowered the cooling effect of anthropogenic aerosols,mainly because of the enhanced warming effect of BC and weakened cooling effect of scattering aerosols. 相似文献
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城市通风廊道能增加城市空气流通能力,缓解城市热岛,为了定量评估城市通风廊道的气象效应,本文采用区域边界层化学模式(RBLM-Chem),利用杭州市高分辨率地表类型、城市建筑等资料,开展了杭州市通风廊道影响的模拟研究,模式水平分辨率为250 m。本文针对冬季和夏季两个典型个例进行数值模拟和敏感性试验,夏季个例时间为2013年8月12日,盛行南风,风向顺着通风廊道;冬季个例时间为2014年1月28日,盛行东风,风向垂直于通风廊道。主要结论如下:城市绿色通风廊道有增加风速、降低气温、提高湿度的作用,与没有通风廊道的情况相比,夏季风顺着廊道方向时,廊道区域风速平均增加可达1.4 m/s,廊道区域内60 m高度风速平均增加可达1 m/s。而冬季风垂直于廊道时,廊道区域风速增加较小,仅有0.5 m/s左右。通风廊道夏季降温幅度平均可达2.7°C,冬季降温幅度较小,仅有0.6°C左右。通风廊道对气象场的影响随风向向下游延伸,夏季在通风廊道下游250 m处,风速增加、气温下降、相对湿度增加最大值分别为1.5 m/s、2.9°C、3.1%,即使在通风廊道下游1500 m处,最大降温仍有1.2°C。 相似文献
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城市小区建筑物和屋顶绿化对小区气象环境影响的数值模拟研究 总被引：1，自引：1，他引：0
为了研究城市小区建筑物和屋顶绿化对小区气象环境影响,利用USDSM(城市小区气象与污染扩散数值模式)对杭州市一临钱塘江小区进行敏感性试验。结果表明:(1)小区建筑物的拖曳、阻尼和摩擦作用造成敏感小区内10 m高度平均水平风速减小0.56 m·s-1;对风速的影响范围:迎风向为500 m,背风向为500~600 m,侧风向为200 m,影响高度达到建筑物群平均高度的两倍以上。(2)小区建筑物存在导致低层污染扩散能力减弱,平均污染物浓度达到初始浓度0.01的时间延迟7.6 min。(3)100%的屋顶绿化面积可造成敏感小区平均地表温度下降0.56℃;5 m高度平均气温下降0.70℃;小区平均建筑物高度处气温下降0.94℃。敏感小区内10 m高度平均水平风速增加0.14 m·s-1;小区建筑物下游水平风速显著减小,影响范围达到了600~800 m。 相似文献
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Effect of urbanization on the urban meteorology and air pollution in Hangzhou 总被引：2，自引：1，他引：1 
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下载免费PDF全文 Urbanization has a substantial effect on urban meteorology. It can alter the atmospheric diffusion capability in urban areas and therefore affect pollutant concentrations. To study the effects of Hangzhou’s urban development in most recent decade on its urban meteorological characteristics and pollutant diffusion, 90 weather cases were simulated, covering 9 weather types, with the Nanjing University City Air Quality Prediction System and high-resolution surface-type data and urban construction data for 2000 and 2010. The results show that the most recent decade of urban development in Hangzhou substantially affected its urban meteorology. Specifically, the average urban wind speed decreased by 1.1 m s ?1; the average intensity of the heat island increased by 0.5°C; and the average urban relative humidity decreased by 9.7%. Based on one case for each of the nine weather types, the impact of urbanization on air pollution diffusion was investigated, revealing that the changes in the meteorological environment decreased the urban atmosphere’s diffusion capability, and therefore increased urban pollutant concentrations. For instance, the urban nitrogen oxides concentration increased by 2.1 μg m ?3 on average; the fine particulate matter (diameter of 2.5 μm or less; PM2.5) pollution concentration increased by 2.3 μg m ?3 on average; in highly urbanized areas, the PM2.5 concentration increased by 30 μg m ?3 and average visibility decreased by 0.2 km, with a maximum decrease of 1 km; the average number of daily hours of haze increased by 0.46 h; and the haze height lifted by 100–300 m. The “self-cleaning time” of pollutants increased by an average of 1.5 h. 相似文献
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本文采用RBLM-chem模式,利用杭州市高分辨率城市建筑等资料,定量分析城市动力效应、热力效应以及城市植被、人为热对SO2、NO2、O3、PM2.5等主要污染物浓度的影响。结果表明,城市化过程使得大部分城区温度上升约1℃,相对湿度下降约6%,风速下降约0.8 m·s-1,湍流动能增强约0.03 m2·s-2。城市动力效应主要通过降低城市风速,使得城区污染物浓度升高,SO2浓度有近5 μg·m-3的上升,PM2.5、O3浓度也有近15 μg·m-3的上升。城市热力效应主要通过热岛环流使城区污染物向上输送,令地面污染物浓度降低,在城市大部分区域PM2.5都有大约10 μg·m-3的浓度下降。城市动力效应大于热力效应,城市的总体作用是使污染物浓度升高。城市下垫面使污染物浓度上升的另外一个机制是代替了自然有植被的下垫面,使污染物干沉降速度下降,但这一作用小于动力学效应。另一方面,人为热对城市主要污染物浓度都起着减小的作用,其中SO2、NO2、O3、PM2.5浓度降幅分别在2.5、3.0、6.0、10.0 μg·m-3左右。城市植被可以显著增加污染物干沉降速度,使主要污染物SO2、NO2、O3和PM2.5的干沉降速度分别上升0.1、0.1、0.03、0.06 m·s-1左右,相应地使上述污染物浓度分别下降2.5、6.0、4.0、6.0 μg·m-3左右。 相似文献
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