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In recent years,several studies pointed out that anthropogenic emission sources in China which significantly contribute to the PM2.5mass burden was an important cause of particulate pollution in South Korea.However,most studies generally focused upon a single pollution event.It is rare to see comprehensive research that captures those features prone to interannual variations concerning the transboundary pollutant contribution in South Korea using a unified method.In this paper,we establish the emission inventories covering East Asia in 2010,2015,and 2017,and then conduct the source apportionment by applying a coupled regional air quality model called the Integrated Source Apportionment Module(ISAM).Comparison of simulated and observed PM2.5mass concentration at 165 CNEMC(China National Environmental Monitoring Center)sites suggests that the PM2.5concentrations are well represented by the modeling system.The model is used to quantitatively investigate the contribution from emission sources in China to PM2.5concentrations over South Korea and those features found to be prone to interannual variations are then discussed.The results show that the average annual contribution of PM2.5has dropped significantly from 28.0%in 2010 to 15.7%in 2017,which strongly suggests that China has achieved remarkable results in the treatment of atmospheric particulates. 相似文献
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将INTEX-B排放源应用到空气质量模型Model3-CMAQ中,对中国地区对流层NO2的浓度分布进行了数值模拟,并与OMI卫星对流层NO2资料进行了对比和验证。结果表明：将INTEX-B排放源应用到Model3-CMAQ模式,模拟的NO2浓度在中国地区的分布、季节变化规律与卫星资料所得结果一致。敏感性试验表明,工业及电厂排放对NO2的浓度贡献最大,而交通排放的贡献相对较小,两种排放均主要集中在京津、长江三角洲等经济发达地区。 相似文献
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We present comparisons of the NO2 regional Chemical Transport Model （CTM） simulations over North-eastern North America during the time period from May to September, 1998 with hourly surface NO2 observations and the NO2 columns retrieved from the GOME （Global Ozone Monitoring Experiment） satellite instrument. The model calculations were performed using the Mesoscale Meteorological Model 5 （MM5）, Sparse Matrix Operator Kernal Emissions （SMOKE）, and Community Multiscale Air Quality （CMAQ） modeling systems, using the emission data from the National Emissions Inventory （NEI） databases of 1996 （U.S.） and 1995 （Canada）. The major objectives were to assess the performance of the CMAQ model and the accuracy of the emissions inventories as they affected the simulations of this important short-lived atmospheric species. The modeled （NcMAQ） and measured （NGOME） NO2 column amounts, as well as their temporal variations, agreed reasonably well. The absolute differences （NcMAQ-NGOME） across the domain were between ±3.0×10^15 molecules cm^-2, but they were less than ±1.0×10^15 molecules cm^-2 over the majority （80%） of the domain studied. The overall correlation coefficient between the measurements and the simulations was 0.75. The differences were mainly ascribed to a combination of inaccurate emission data for the CTM and the uncertainties in the GOME retrievals. Of these, the former were the more easily identifiable. 相似文献
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为更好地改进提高模式预报性能,评估了新一代WRF-CMAQ（Weather Research and Forecasting model-Community Multi-scale Air Quality model）模式系统的不同网格分辨率预报产品对2018年北京市城六区空气质量预报结果的影响。分析表明:（1）基于首要污染物为PM2.5的预报数据集,模式系统1 km网格分辨率（BJ01）和3 km网格分辨率（BJ03）等级准确率优于官方预报结果,模式系统BJ01和BJ03区域4天内预报等级准确率均达到50%以上,24 h内准确率达60%以上,官方预报24 h内等级准确率为59%。本文引入预报综合评分法,基于IAQI（Individual Air Quality Index）和等级级别正确性双因素的预报综合评分结果显示,模式系统BJ03得分75.0分最高,BJ01次之,优于官方预报结果,模式9 km网格分辨率（BJ09）得分69.1分最低。（2）基于模式系统2018年长时间序列预报结果分析表明:模式系统预报的PM2.5浓度与实测的变化趋势较为一致,其中模式系统BJ03结果与实测PM2.5浓度相关系数达0.76,覆盖区域较大的BJ03和BJ09对PM2.5浓度峰值模拟较好。中重度污染过程的PM2.5浓度峰值模式预测误差表明,不同分辨率模式预报峰值误差的变化趋势基本一致,覆盖区域更大的粗分辨率模式预报结果高于覆盖区域小的细分辨率模式预报结果。与预报综合评分结果一致,统计分析结果也表明BJ03区域预报效果最好,平均偏差为0.83 μg/m3;而BJ01区域预报整体偏低,BJ09区域预报整体偏高。（3）基于不同网格分辨率预报效果的空间差异性分析表明:同一站点在不同分辨率上表现不一致,BJ01区域中农展馆站表现最好,BJ03区域中万柳站表现最好,BJ09区域中东四站表现最好。 相似文献
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大气污染物排放清单是空气质量模拟和空气污染治理的重要依据.本研究比较分析了两套覆盖江苏省的2017年大气污染物排放清单，即分别由上海市环境科学研究院、江苏省环境科学研究院编制的"长三角清单"和"江苏省清单"，并结合区域空气质量模型CMAQ评估不同清单对长三角地区2017年1、4、7、10月的空气质量模拟的影响.清单比较结果表明，除二氧化硫（SO2）以外，江苏省清单估算的各污染物排放量较长三角清单低.通过与观测数据比较，发现两套清单对SO2、氮氧化物（NOx）、臭氧（O3）和细颗粒物（PM2.5）的模型模拟性能均较好.江苏省清单与长三角清单两者的模拟结果空间分布接近，其中江苏省清单模拟的PM2.5和O3在长三角多数地区略低于长三角清单的模拟结果（1月O3除外）.江苏省清单与长三角清单均能够用于空气质量模式模拟，可为江苏地区的细颗粒物和光化学烟雾污染的控制策略制定提供参考. 相似文献
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The simulation of aerosol transport over East Asia region 总被引：1，自引：0，他引：1
Youn-Seo Koo Sung-Tae Kim Hui-Young Yun Jin-Seok Han Jung-Young Lee Ki-Hyun Kim Eui-Chan Jeon 《Atmospheric Research》2008,90(2-4):264-ICNAA07
This study was carried out to understand the contribution of PM10 from China emission to Seoul Metropolitan Area (SMA) during high concentration period in January, 2007. The hourly PM10 concentration in Seoul Metropolitan Area had reached up to over 150 μg/m3 on 17th and 23rd of January in 2007. The aerosol transports from China along the Northwestern wind becomes the background concentrations in Korea and the assessment of the amount of contribution from China is very important in managing the air quality improvement plan in SMA.The U.S. EPA's Models-3/CMAQ (Community Multiscale Air Quality) was used to simulate PM10 concentration. The CMAQ performance was evaluated by comparing with the measurements in SMA for the episode period. The predictions were relatively in a good agreement with the measurements.The results show that the PM10 transport from China to Korea is significant and its contribution reaches up to 80% in the episode period. In order to assess more extensively the aerosol transport in East Asia region, the study to run the model in full year with speciated PM component measurements in super site is underway. 相似文献
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An emission source inversion model based on satellite data and its application in air quality forecasts 总被引：1，自引：0，他引：1
CHENG XingHong XU XiangDe & DING GuoAn Chinese Academy of Meteorological Sciences Beijing China National Climate Center 《中国科学:地球科学(英文版)》2010,(5)
This paper aims at constructing an emission source inversion model using a variational processing method and adaptive nudging scheme for the Community Multiscale Air Quality Model (CMAQ) based on satellite data to investigate the applicability of high resolution OMI (Ozone Monitoring Instrument) column concentration data for air quality forecasts over the North China. The results show a reasonable consistency and good correlation between the spatial distributions of NO2 from surface and OMI satellite measur... 相似文献
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A dust deflation module was developed and coupled with the air quality modeling system RAMS-CMAQ to simultaneously treat all the major tropospheric aerosols（i.e.,organic and black carbons,sulfate,nitrate, ammonia,soil dust,and sea salt）.Then the coupled system was applied to East Asia to simulate Asian dust aerosol generation,transport and dry/wet removal processes during 14-25 March 2002 when two strong dust storms occurred consecutively.To evaluate model performance and to analyze the observed features of dust aerosols over the East Asian region,model results were compared to concentrations of suspended particulate matter of 10μm or less(PM10;1-h intervals) at four remote Japanese stations and daily air pollution index （API） values for PM10 at four large Chinese cities.The modeled values were generally in good agreement with observed data,and the model reasonably reproduced two dust storm outbreaks and generally predicted the dust onset and cessation times at each observation site.In addition,hourly averaged values of aerosol optical thickness（AOT） were calculated and compared with observations at four Aerosol Robotic Network （AERONET） stations to assess the model’s capability of estimating dust aerosol column burden.Analysis shows that modeled and observed AOT values were generally comparable and that the contribution of dust aerosols to AOT was significant only with regard to their source regions and their transport paths. 相似文献