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1.
Arsenic contamination caused by roxarsone transformation with spatiotemporal variation of microbial community structure in a column experiment
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Liu Ya-ci Zhang Zhao-ji Zhao Xin-yi Wen Meng-tuo Cao Sheng-wei Li Ya-song 《地下水科学与工程》2021,9(4):304-316
Arsenic contamination from roxarsone in livestock manure is common, and livestock manure continuously accumulates in the open environment. Evaluations of the environmental processes of As mobilization and transformation are critical for predicting the fate of As compounds after roxarsone degradation. In this study, spatiotemporal variations in As species and microbial community structure were characterized using laboratory column experiments with background soil collected from Yanggu County (northern Shandong Plain, China), a region of intense poultry production. Organic and inorganic arsenic were detected by high-performance liquid chromatography (HPLC) and HPLC with hydride generation atomic fluorescence spectrometry (HPLC-HG-AFS), respectively. High-throughput sequencing technology was used to describe microbial diversity. Results showed that roxarsone was transformed completely within 7 days, and As(Ⅲ) and As(Ⅴ) were the major degradation products. The concentration of As(Ⅲ) was much lower than that of As(Ⅴ). The As(Ⅲ) concentration increased significantly after Day 14, whereas the As(Ⅴ) concentration increased significantly after Day 84, indicating that As(Ⅲ) was initially produced. The microbial community structure changed significantly as roxarsone transformed into various As compounds. A critical and dominant bacterial strain, norank_f__Family_XVⅢ, was found to be related to the degradation of roxarsone into As(Ⅲ). This study improves our understanding of the fate of As species released from poultry litter to soil and groundwater, which is a threat to human health and environment. 相似文献
2.
We report on a hexactinellid sponge new to science, Walteria demeterae sp. nov., which was collected from the northwestern Pacific seamounts at depths of 1271–1703 m. Its tubular and basiphytous body, extensive lateral processes, numerous oval lateral oscula which are irregularly situated in the body wall, the presence of microscleres with oxyoidal, discoidal and onychoidal outer ends, and the absence of anchorate discohexasters, indicate it belongs to the genus Walteria of family Euplectellidae, which is also supported by molecular phylogenetic evidence from 18S, 28S, 16S rRNA and cytochrome c oxidase subunit I (COI) gene sequences. The unique morphotype, which is structured by a thin and rigid framework of body wall and lateral processes consisting of diactins, characterizes it as a new species. Local aggregations of individuals of this new species coupled with their associated macrofauna in the Suda Seamount are reported, highlighting its functional significance in providing biogenic microhabitats in the deep sea. 相似文献
3.
多宝山矿区发现有侵位于晚奥陶世花岗闪长岩的角闪辉长岩和英云闪长岩,二者具有双峰式侵入岩的特征,在详细的野外地质调查基础上,对多宝山双峰式侵入岩进行了岩石学、年代学、地球化学方面的研究,并初步探讨其构造意义.角闪辉长岩的LA-ICP-MS锆石U-Pb年龄为224.3±1.7 Ma,英云闪长岩为226.3±2.3 Ma,两者形成于同一构造岩浆作用事件;侵入岩的SiO2含量呈双峰式,稀土、微量元素特征表明它们具有岛弧岩浆特征,二者具有相同的岩石圈地幔源区,其源区可能受到了俯冲流体交代作用的影响.结合区域构造背景,认为其形成与鄂霍茨克洋壳俯冲有关,产于活动大陆边缘环境,它们可能是受地壳混染的OIB型玄武质岩浆在地壳中部的一个“双扩散”岩浆房通过结晶分异形成的. 相似文献
4.
在西大别造山带的区调工作中,新识别出一系列中元古代末-新元古代的岩石-构造单元,它们沿着吕王-高桥-永佳河一线展布,并构成一条NNW-SEE向展布的构造混杂岩带.该混杂岩带主要由超镁铁质-镁铁质岩、硅泥质岩、石英质岩、大理岩、含碳陆源碎屑岩、双峰式火山岩以及卷入其中的榴辉岩等多种变质岩块(片)共同组成,并赋存于一套遭受了强烈剪切变形的泥质片岩之中.混杂岩带内各岩块(片)的原岩年龄跨度较大(>4亿年),分别集中在1 200~1 100 Ma和800~700 Ma之间.锆石记录的变质年龄和云母的冷却年龄则主要集中在240~200 Ma之间.结合接触关系、岩性组合、年代学及地球化学数据的综合研究认为,混杂岩带的物质来源既包括中元古代末-新元古代早期的弧-弧后盆地系统的沉积岩-火山岩-侵入岩;也包括叠置其上的新元古代中-晚期大陆裂解期的沉积岩-火成岩.这些不同时代、不同性质岩石在三叠纪不同程度地卷入了华南陆块北缘向华北陆块之下的俯冲,而后快速折返,最终沿着区域上折返断裂(桃花-七角山断裂)就位于西大别造山带之中,形成一条包含高压-超高压变质岩的三叠纪构造混杂岩带.混杂岩带内新厘定的中元古代末弧-弧后岩浆-沉积事件,可与大洪山-黄陵庙湾同时期的地质事件对比,它们共同揭示扬子北缘曾经存在一条中元古代末-新元古代早期的俯冲岩浆带. 相似文献
5.
根据美国地质调查局(United States Geological Survey,缩写为USGS)国家地震信息中心(National Earthquake Information Centre,缩写为NEIC)的测定,2021 年2 月13 日14 时7 分50 秒( UTC) ,日本本州以东发生了一次矩震级高达 MW7.2 的地震,震中位于( 37.745°N, 141.749°E),震源深度为 49.94 km,这是截至本文发稿时最终更新的定位结果,更新前为(37.686°N,141.992°E),震源深度为54.0 km.美国地质调查局(USGS,2021)和全球矩心矩张量组( GCMT, 2021)随后发布了这次地震的矩心矩张量解(表1).震后48小时内累计发生M>2.5 余震13 次,其中最大的余震震级达到MW5.3,主震和余震的深度分布在35—65 km之间.该事件所在区域曾于2011 年3 月11 日发生过MW9.1 特大地震(Duputel et al,2012a)并引起破坏性海啸,相较于2011年MW9.1事件,本次事件的位置更靠近西侧,发生在俯冲带较深的区域. 相似文献
6.
Li Zhang Jianping Huang Haipeng Yu Xiaoyue Liu Yun Wei Xinbo Lian Chuwei Liu Zhikun Jing 《大气和海洋科学快报》2021,14(4):58-62
现如今,新冠肺炎(COVID-19)严重威胁着世界各国人民的生命健康.许多流行病学模型已经被用于为政策制定者和世界卫生组织提供决策参考.为了更加深刻的理解疫情趋势的变化特征,许多参数优化算法被用于反演模型参数.本文提议使用结合了高斯-牛顿法和梯度下降法的Levenberg-Marquardt(LMA)算法来优化模型参数.使用四个病例数相对较多的国家来验证这一算法的优势:相较于传统流行病学模型模拟曲线过早过快的到达峰值,应用 LMA 的 Statistical-SIR(Statistical-Susceptible-Infected-Recovered)模型可以更好地拟合实际疫情曲线. 相似文献
7.
利用2015年1月至2021年5月28日期间我国云南省漾濞县及周边地区固定台站和漾濞地震后布设的流动台站所记录到的近震资料,使用双差层析成像方法获得了该地震震区的高分辨率地壳三维速度结构和震源位置。重定位结果显示,漾濞M6.4地震序列主要沿NW?SE向展布,与维西—乔后—巍山断裂走向一致,地震主要集中在4—10 km的深度范围,呈约80°高倾角分布。结合定位结果与三维速度结构显示:漾濞M6.4地震序列的空间分布与速度结构变化具有相关性,主震位于P波、S波高低速异常交界处,这种介质物性变化的交界地带可能有利于中强地震的孕育和发生,余震主要分布在低P波速度、高S波速度和低波速比的脆性区域;沿漾濞地震序列的分布走向,主震两侧呈现完全不同的速度结构,其西北部具有明显的高P波速度、低S波速度特征,该地区高密度、强韧性的地层可能是阻挡漾濞地震的NW向破裂而呈单向破裂特征的原因。 相似文献
8.
Wanying Chen Jieying Na Chengcheng Shen Ruiyan Zhang Bo Lu Hong Cheng Chunsheng Wang Dongsheng Zhang 《海洋学报(英文版)》2021,40(12):55-78
Seamounts are vulnerable ecosystems in the deep sea and can be heavily impacted by human activities, such as bottom fishing and deep-sea mining. The species composition and distribution patterns of benthic fauna is key information for the designation of marine protected areas and environmental management plans. Three contracts for cobalt-rich crust exploration have been granted to China, Japan and Korea in the Northwest Pacific Ocean by the International Seabed Authority. However, our knowledge of benthic biodiversity in this area is extremely insufficient. During 2013–2020, eight Chinese Ocean Mineral Resources R&D Association (COMRA) cruises were conducted to investigate the benthic assemblages of nine seamounts in this region. In this study, 191 ophiuroids collected from seamounts in the Northwest Pacific were identified into 29 species in 11 families. Ophiacanthidae and Euryalidae were the two most dominant families with 12 and 6 species, respectively. Ophiotomidae and Ophiopyrgidae were represented by two species each, while seven families were represented by only one species. Four species were widely distributed among 4–5 seamounts, and 17 species were found only at a single site. An integrated regional taxonomic dataset of Ophiuroidea was generated and analyzed. A total of 23 and 14 species were obtained from the Magellan Seamount Chain (MSC) and the Marcus-Wake seamounts (MWS), respectively, with 8 species shared between the two seamount groups. The individual-based rarefaction curves did not reach an asymptote, suggesting that the sampling effort was inadequate for either the entire region or each single seamount. Most species distributed in a narrow depth range, and the species composition was different between water depths above and below 2000 m. Our results greatly improve the understanding of megafaunal biodiversity from seamounts in the Northwest Pacific Ocean, and highlight the necessity of further surveys to provide more robust information for environmental protection and management in this region. 相似文献
9.
A suction caisson can be extracted by applying reverse pumping water,which cannot be regarded as the reverse process of installation because of the dramatically different soil?structure interaction behavior.Model tests were first carried out in this study to investigate the extraction behavior of the modified suction caisson(MSC)and the regular suction caisson(RSC)in sand by reverse pumping water.The effects of the installation ways(suction-assisted or jacking installation)and the reverse pumping rate on the variations of the over-pressure resulting form reverse pumping water were investigated.It was found that neither the RSC nor the MSC can be fully extracted from sand.When the maximum extraction displacement is obtained,the hydraulic gradient of the sand in the suction caisson reaches the critical value,leading to seepage failure.In addition,the maximum extraction displacement decreases with the increasing reverse pumping rate.Under the same reverse pumping rate,the final extraction displacements for the RSC and MSC installed by suction are lower than those for the RSC and MSC installed by jacking.The final extraction displacement of MSC is almost equal to that of the RSC with the same internal compartment length.Based on the force equilibrium,a method of estimating the maximum extraction displacement is proposed.It has been proved that the proposed method can rationally predict the maximum extraction displacement and the corresponding over-pressure. 相似文献
10.
A well‐constrained plate deformation model may lead to an improved understanding of sedimentary basin formation and the connection between subduction history and over‐riding plate deformation. Building quantitative models of basin kinematics and deformation remains challenging often due to the lack of comprehensive constraints. The Bohai Bay Basin (BBB) is an important manifestation of the destruction of the North China Craton, and records the plate kinematic history of East Asia during the Cenozoic. Although a number of interpretations of the formation of the BBB have been proposed, few quantitative basin reconstruction models have been built to test and refine previous ideas. Here, we developed a quantitative deformation reconstruction of the BBB constrained with balanced cross‐sections and structural, stratigraphic and depositional age data. Our reconstruction suggests that the basin formation process was composed of three main stages: Paleocene‐early Eocene (65–42 Ma) extension initiation, middle Eocene‐early Oligocene (42–32.8 Ma) extension climax and post‐Oligocene (32.8–0 Ma) post‐extensional subsidence. The deformation of the BBB is spatially heterogeneous, and its velocity directions rotated clockwise during the basin formation process. The reconstruction supports the interpretation that the BBB formed via strike‐slip faulting and orthogonal extension and that the basin is classified as a composite extensional‐transtensional basin. We argue that the clockwise rotation of the basin velocity field was driven by the counter‐clockwise rotation in the direction of Pacific Plate subduction. The kinematics of the BBB imply that the Pacific Plate may have been sufficiently coupled to the over‐riding East Asian Plate during the critical period of Pacific Plate reorganization. The new reconstruction provides a quantitative basis for studies of deformation processes not only in the vicinity of the BBB, but also more broadly throughout East Asia. 相似文献