新疆图拉尔根镁铁-超镁铁质杂岩体镍铜钴成矿岩浆作用过程:流体化学与碳同位素组成制约     

张铭杰  班舒悦  李思奥  宋哲  仇哲  李立武  惠卫东  李中平 《岩石学报》2020,36(12):3673-3682

东天山造山带的图拉尔根镁铁-超镁铁杂岩体为一个早古生代长期活动的幔源岩浆通道，大型铜镍钴硫化物矿体赋存于Ⅰ号超镁铁质岩体的顶部，不同类型岩石中辉石矿物的流体挥发份化学组成以H₂O为主（平均91%，5400.4mm³/g），其次为H₂（2.0%）、H₂S（2.3%）和CO₂（2.1%）；赋矿角闪橄榄岩中CO₂和H₂S含量最高，辉长岩中流体挥发份含量低于辉石橄榄岩和橄榄辉石岩等岩浆早期结晶的岩石。CO₂和CH₄的δ¹³C值位于地壳与甲烷氧化的范围内，甲烷同系物的碳同位素组成具有正序分布模式，部分样品（TLG512）释出的CH₄和C₂H₆具有较重的δ¹³C值和反序分布特征。表明I号岩体不同类型岩石可能是不同期次岩浆活动的产物，成矿岩浆具有富H₂O和H₂S的特征，可能起源于被流体交代的亏损地幔源区，混染壳源组分可能为俯冲板片来源蚀变沉积有机质组分。  相似文献   

Nine thousand years of upper montane soil/vegetation dynamics from the summit of Caratuva Peak,Southern Brazil     

《Journal of South American Earth Sciences》2014

Biodiversity loss, climate change, and increased freshwater consumption are some of the main environmental problems on Earth. Mountain ecosystems can reduce these threats by providing several positive influences, such as the maintenance of biodiversity, water regulation, and carbon storage, amongst others. The knowledge of the history of these environments and their response to climate change is very important for management, conservation, and environmental monitoring programs. The genesis of the soil organic matter of the current upper montane vegetation remains unclear and seems to be quite variable depending on location. Some upper montane sites in the very extensive coastal Sea Mountain Range present considerable organic matter from the late Pleistocene and other from only the Holocene. Our study was carried out on three soil profiles (two cores in grassland and one in forest) on the Caratuva Peak of the Serra do Ibitiraquire (a sub-range of Sea Mountain Range – Serra do Mar) in Southern Brazil. The δ¹³C isotopic analyses of organic matter in soil horizons were conducted to detect whether C₃ or C₄ plants dominated the past communities. Complementarily, we performed a pollen analysis and ¹⁴C dating of the humin fraction to obtain the age of the studied horizons. Except for a short and probably drier period (between 6000 and 4500 cal yr BP), C₃ plants, including ombrophilous grasses and trees, have dominated the highlands of the Caratuva Peak (Pico Caratuva), as well as the other uppermost summits of the Serra do Ibitiraquire, since around 9000 cal yr BP. The Caratuva region represents a landscape of high altitude grasslands (campos de altitude altomontanos or campos altomontanos) and upper montane rain/cloud forests with soils that most likely contain some organic matter from the late Pleistocene, as has been reported in Southern and Southeastern Brazil for other sites. However, our results indicate that the studied deposits (near the summit) are from the early to late Holocene, when somewhat wetter and warmer conditions (since around 9000 cal yr BP) enabled a stronger colonization of the ridge of Pico Caratuva by mainly C₃ plants, especially grassland species. However, at the same time, even near the summit, the soil core from the forest site already presented the current physiognomy (or a shrubby/elfin or successional forest), indicating that the colonization of the neighboring uppermost saddles and valleys were probably populated mainly by upper montane forest species.  相似文献   

南极半岛邻近海域夏季POC分布特征及其影响因素          下载免费PDF全文

张一成  韩正兵  杨洋  潘建明  张海峰  李栋  赵军  朱秋红  范高晶  张海生 《极地研究》2020,32(1):47-59

海水中的颗粒有机碳(POC)与生物的生命过程、初级生产力关系密切,是海洋食物链中重要的物质基础和能量来源,因此POC的分布特征可以有效反映其生物地球化学环境。利用中国第33次南极考察期间(2016年12月至2017年1月)在南极半岛邻近海域采集的海水颗粒物样品,研究POC的空间分布特征及其影响因素。结果表明,斯科舍海0—200 m的POC浓度范围为7.44—193.52μg·L~(-1),平均浓度为(48.84±35.09)μg·L~(-1);南斯科舍海岭0—200 m的POC浓度范围为9.13—62.17μg·L~(-1),平均浓度为(29.76±14.12)μg·L~(-1);鲍威尔海盆0—200 m的POC浓度范围为5.87—270.72μg·L~(-1),平均浓度为(48.57±38.92)μg·L~(-1)。表层POC高值出现在斯科舍海区和鲍威尔海盆区,而低值出现在海岭区,与叶绿素a(Chla)的变化趋势一致,与营养盐的变化趋势相反。垂向分布上,各个区域POC平均浓度随深度的增加而减少,鲍威尔海盆和斯科舍海POC最高值都出现在25 m层。分析结果表明光合浮游植物是研究海域POC的主要来源, POC的主要影响因素为温度、水团混合以及海冰环境。斯科舍海与鲍威尔海盆整体非生命POC占比高,可能是由于高磷虾生物量、海冰碎屑以及陆源输入的干扰;南斯科舍海岭整体非生命POC占比低。  相似文献   

Middle Permian organic carbon isotope stratigraphy and the origin of the Kamura Event     

《Gondwana Research》2020

Large carbon cycle perturbations associated with the Middle Permian (Capitanian) mass extinction have been widely reported, but their causes and timing are still in dispute. Low resolution carbon isotope records prior to this event also limit the construction of a Middle Permian chemostratigraphic framework and global or local stratigraphic correlation, and hence limit our understanding of carbon cycle and environmental changes. To investigate these issues, we analyzed the ¹³C_org values from the Middle Permian chert-mudstone sequence (Gufeng Formation) in the Lower Yangtze deep-water basin (South China) and compared them with published records to build a chemostratigraphic scheme and discuss the underlying environmental events. The records show increased δ¹³C_org values from late Kungurian to early Guadalupian, followed by a decrease to the late Wordian/early Capitanian. The early-mid Capitanian was characterized by elevated δ¹³C_org values suggesting the presence of the “Kamura Event”: an interval of heavy positive values seen in the δ¹³C_carb record. We propose that these heavy Capitanian δ¹³C values may be a response to a marked decline in chemical weathering rates on Pangea and associated reduction in carbonate burial, which we show using a biogeochemical model. The subsequent negative δ¹³C excursion seen in some carbonate records, especially in shallower-water sections (and in a muted expression in organic carbon) coincide with the Capitanian mass extinction may be caused by the input of isotopically-light carbon sourced from the terrestrial decomposition of organic matter.  相似文献   

A global comparison of carbon-water-food nexus based on dietary consumption     

《Global Environmental Change》2022

Exploring the environmental impact of dietary consumption has become increasingly important to understand the carbon-water-food nexus, vital to achieving UN sustainable development goals. However, the research on diet-based nexus assessment is still lacking. Here, we developed an Environmentally Extended Multi-Regional Input-Output (EE-MRIO) model with compiling a global MRIO table based on the latest Global Trade Analysis Project (GTAP) 10 database, where we specifically constructed a water withdrawal account and matched it to each economy at the sectoral level. The regional heterogeneity and synergy of carbon-water nexus affected by dietary patterns in nine countries was explored. The results show that: (1) Dietary consumption is the main use of water withdrawal for each country; Japan, the US, South Korea, and India have a high per capita dietary water footprint. Mainly due to consumption of processed rice, Japan has the highest per capita value of 488 M³/year, accounting for 63.4% of the total water footprint. (2) The total dietary carbon footprints in China, India, and the US are high, which is mainly caused by the high consumption of animal products (including dairy) either due to the large population (China, India) or animal-based diet (the US). Americans have the highest per capita dietary carbon footprint, reaching 755.4 kg/year, 2.76 times that of the global average. (3) Generally, imported/foreign footprints account for a greater share in dietary water and carbon footprints of developed countries with an animal-based diet. (4) In the nexus analysis, the US, Japan, and South Korea are key-nexus countries, vegetables, fruit and nuts, tobacco and beverages, and other food products are selected as key-nexus sectors with relatively high dietary water and carbon footprint. Furthermore, dietary consumption choices lead to different environmental impacts. It is particularly important to find a sustainable dietary route adapted to each country considering that heterogeneity and synergism exist in key-nexus sectors to achieve the relevant Sustainable Development Goals.  相似文献   

COVID-19疫情期间全球空气质量变化:臭氧响应的区域间差异          下载免费PDF全文

Rong Tang  Xin Huang  Derong Zhou  Haikun Wang  Jiawei Xu  Aijun Ding 《大气和海洋科学快报》2021,14(4):45-51

疫情期间全球各地一次排放大幅削减,而臭氧等二次污染的响应则存在着区域间差异.结合地面和卫星观测发现,同在氮氧化物大幅下降的情况下,臭氧在东亚和欧洲呈现出可达14ppb的上升信号,而北美则下降为主(约2-4ppb).我们结合气象分析和臭氧敏感性进一步讨论了臭氧响应差异性的原因,一方面受臭氧与前体物间关系的影响;另一方面来自于气象,尤其是温度.研究明晰了人为排放,化学和气象三者的内在关联,强调了在臭氧控制过程中考虑前体物削减和气象条件协同的重要性.  相似文献   

碳市场与电力市场机制影响下发电机组成本分析与竞争力研究     

孙友源  郭振  张继广  秦亚琦 《气候变化研究进展》2021,17(4):476-483

碳市场和电力市场将共同发挥市场对资源优化配置的决定性作用,对共同市场主体发电企业带来经营和发展挑战。在考虑碳成本的基础上,采用发电机组经济性影响模型,定量分析了碳市场不同发展阶段对发电机组发电成本的影响,定量评价不同能源结构投资收益经济性,以及对集中竞价市场出清顺序的影响。结果表明,随着有偿配额比例和碳价增加,碳成本占发电成本比例逐步攀升,燃煤机组碳成本占发电成本比例最高将达29%,燃气机组此比例达6%;在设定碳市场高比例配额有偿分配和高碳价情况下,煤电和气电单位发电收益逐步降低甚至出现亏损,远低于可再生能源,推动投资逐步向清洁高效火电机组和可再生能源倾斜;碳成本将成为竞价市场需考虑的重要因素,并影响发电机组出清顺序,进一步巩固高效率、低排放机组在集中竞价市场中的竞争力。  相似文献   

IPCC AR6报告解读：气候系统对太阳辐射干预响应     

曹龙 《气候变化研究进展》2021,17(6):671-684

IPCC第六次评估报告（AR6）第一工作组报告评估了太阳辐射干预（Solar radiation modification,SRM）对气候系统和碳循环的影响。在大幅度减排基础上,太阳辐射干预有潜力作为应对气候变化的备用措施。目前,对于太阳辐射干预气候影响的评估都是基于模式模拟结果。评估主要结论如下：太阳辐射干预可以在全球和区域尺度上抵消一部分温室气体增加造成的气候变化（高信度);但是太阳辐射干预无法在全球和区域尺度上完全抵消温室气体增加引起的气候变化（几乎确定);有可能通过适当的太阳辐射干预设计,同时实现多个温度变化减缓目标（中等信度);在高强度温室气体排放情景下,如果太阳辐射干预实施后突然终止,并且这种终止长时间持续,将会造成快速的气候变化（高信度);如果在减排和CO₂移除的情况下,太阳辐射干预的实施强度逐渐减小至零,将显著降低太阳辐射干预突然终止产生的快速气候变化风险（中等信度);太阳辐射干预会通过降温作用,促进陆地和海洋对大气CO₂的吸收（中等信度),但是太阳辐射干预无法缓解海洋酸化（高信度);太阳辐射干预对其他生物化学循环影响的不确定性大。由于对云-气溶胶-辐射过程的相互作用和微物理过程认知有限,目前对平流层气溶胶注入、海洋低云亮化、高层卷云变薄等太阳辐射干预方法的冷却潜力和气候效应的认知还有很大的不确定性。  相似文献   

全球2℃温升碳约束下中国煤电搁浅资产研究     

张为荣  袁家海 《气候变化研究进展》2021,17(1):36-44

作为全球煤电装机规模最大且仍在扩张的国家,中国需要慎重评估兑现《巴黎协定》温室气体减排承诺带来的潜在煤电资产搁浅问题。研究运用“上下交互”的碳锁定曲线模型,识别不同产能扩张情景下（无新增、新增200、300和400 GW）的搁浅煤电机组。首先,从“自上而下”角度匡算中国煤电行业2℃温升目标下的碳配额。然后,从“自下而上”角度,根据高精度的燃煤电站信息核算煤电累积CO₂排放量。最后基于“上下交互”模式筛选出搁浅燃煤电站,在此基础上运用现金流量法估算其潜在的搁浅价值,并对其关键因素进行敏感性分析。结果表明,在无新增情景下,煤电搁浅资产规模约为0.38万亿元;若继续增加200~400 GW煤电装机,则搁浅价值将较无新增情景增加3.7~8.2倍。因此,建议“十四五”期间应树立煤电规模峰值意识,严控煤电新增产能,避免错过最佳减排时机。  相似文献   

碳市场顶层设计路线图     

邹骥  柴麒敏  陈济  傅莎  葛兴安  胡敏  李昂  林丹妮  林殷  刘冬惠  刘俊伶  刘爽  祁悦  王克  王庶  张俊杰 《气候变化研究进展》2019,15(3):217-221

中国正面临着低碳减排和保持经济增速的双重挑战。为利用碳排放权交易机制以最低的社会成本实现减排目标,我国自2013年起开始建设碳排放权交易试点,并于2017年12月起宣布正式启动全国碳市场。然而碳市场的顶层设计不可一蹴而就,需要在我国宏观经济改革的大背景下分阶段逐步推进。短期（2020年前）碳市场建设重在强化产权制度建设,完善市场交易基础。中期（2021—2030年）碳市场建设要形成活跃的市场氛围,充分降低我国的温室气体达峰成本。长期（2031—2050年）碳市场建设要形成稳定上升的碳价趋势,为我国的低碳转型提供长期动力。  相似文献