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以华北地区为研究区域,利用地面监测数据、高空观测资料、NCEP FNL资料及HYSPLIT后向轨迹模式,对2016年12月26日至2017年1月9日该地区的雾霾天气过程进行综合分析。结果表明,雾霾期间高空以纬向环流为主,冷空气势力偏弱,主要受高压、弱高压或均压场控制,有利于华北地区静稳天气形成。同时,雾霾期间边界层平均高度约600~900 m,污染物浓度与边界层高度呈负相关,且污染物浓度变化较边界层高度变化存在滞后现象。逆温层的长期存在,不利于污染物垂直扩散,能见度一直维持在5 km以下。后向轨迹集合模拟与聚类分析表明,以北京地区为核心的华北地区雾霾天气期间,外来污染物中,80%来自西北方气团,20%来自河北西南地区气团。 相似文献
3.
利用2006年"珍珠"台风影响福建省期间的酸雨监测资料和新一代天气雷达回波资料,对城市降水酸度分布特征及福州市短时段降水酸度进行分析,结果表明:来自海上的台风降水呈偏碱性;登陆后台风对福建省城市降水酸度的影响与其螺旋雨带上降水云团的移动路径及城市周边污染源分布有关;"珍珠"台风的短时段降水酸度并非保持恒定,对福州市降水酸度的影响会随着台风强度、风场结构的变化及螺旋雨带上降水云团途经下垫面城市大气污染排放状况而发生改变. 相似文献
4.
Diatoms were identified and enumerated from a surface sediment calibration set of 50 lakes in northwestern Québec. The relationship
between species composition and environmental variables was examined using canonical correspondence analysis (CCA). Forward
selection and Monte Carlo permutation tests in CCA indicated that diatom species distributions in the data set are most strongly
correlated to lakewater pH. A strong (r
2
boot = 0.83) weighted averaging calibration model, that includes bootstrapped error estimates, was developed for inferring past
lakewater pH. Using this model, temporal changes in pH were reconstructed for two kettle lakes, Lac de la Pépinière and Lac
Perron. Based on limnological data, both the study lakes were expected to have recently acidified due to increased acidic
precipitation and increases in anthropogenic metal loading. However, our long-term pH inference data indicate that these lakes
were naturally acidic during pre-industrial times. Nonetheless, the rate of acidification, particularly in Lac de la Pépinière,
has accelerated in the last ∼75 years. These long-term pH records developed for the dilute lakes in northwestern Québec suggest
that the region has received increased atmospheric pollutants from the nearby Horne smelter in Rouyn-Noranda. The pH inference
profiles are markedly different from many other paleolimnological studies in acid-sensitive regions of Canada that have become
acidic primarily as a result of industrial activities.
Electronic supplementary material The online version of this article (doi: ) contains supplementary material, which is available to authorized users. 相似文献
5.
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A simulation was undertaken within a climatic chamber to investigate limestone dissolution under varied carbonic acid (H2CO3) strengths as a possible analogue for future increases in atmospheric CO2 arising from global warming. Twenty‐eight samples cut from a block of Bath (Box Hill) limestone from Somerville College, Oxford, which had been removed during restoration after 150 years in an urban environment, were weighed and placed in closed bottles of thin plastic containing varying concentrations of H2CO3. Half of the stone samples were derived from exposed surfaces of the stone block (weathered) while the others were obtained from the centre of the block on unexposed surfaces (unweathered). The purpose of this was to compare dissolution of previously weathered versus unweathered surfaces in strong (pH 4·73) versus weak (pH 6·43) solutions of H2CO3. A temperature of c. 19 °C was maintained within the chamber representing a plausible future temperature in Oxford for the year 2200 given current warming scenarios. The simulation lasted 25 days with a few stone samples being removed midway. Stone samples show reduced weight in all cases but one. There was greater dissolution of stone samples in a strong H2CO3 solution as conveyed by higher concentrations of total hardness and Ca2+ in the water samples as well as enhanced microscopic dissolution features identified using SEM. The simulation confirms that enhanced atmospheric CO2 under global warming, given adequate moisture, will accelerate dissolution rates particularly of newly replaced limestone building stones. However, previously weathered surfaces, such as those on historical stone exposed for a century or more, appear to be less susceptible to the effects of such increased rainfall acidity. Conservation techniques which remove weathered surfaces, such as stone cleaning, may accelerate future decay of historical limestone structures by increasing their susceptibility to dissolution. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
7.
No author 《Aquatic Sciences - Research Across Boundaries》2005,67(3):392-291
No Abstract. .The following two amendments concern the above mentioned article that appeared electronically Online First on June13, 2005 (this issue, pp. 274–291).1. the first name of the author Cooper is Philip (and not Phillip).2. the correct grant reference number is EVK1-CT-1999-00032 (instead of: EVK1-CT-2002-00121). 相似文献
8.
过硫酸铵氧化容量法测定矿石中锰方法的改进 总被引:5,自引:1,他引:5
采用过硫酸铵氧化容量法测定锰时,可在低酸度(0.18mol/LH2SO4、0.29mol/LH3PO4)和大体积(300mL)溶液中氧化Mn2 至Mn7 。所测得的结果十分稳定,回收率为100%。采用管理样分析验证方法,其结果与铋酸钠容量法结果一致。对于w(Mn)=11.36%的试样进行10次分析测定,RSD=0.33%。方法可测定w(Mn)≥0.01%的常见矿种样品。 相似文献
9.
This paper deals with the infrared spectra of " amino acid- clay , calcium carbonate and y-AlOOH" and " Cu (II )-clay-amino acid" model systems, and shows that the model of the ternary surface complex is M-OHLCu (L = amino acid) for marine solid particle-Cu (II)-amino acid. Study of the formation mechanism of the ternary surface complex shows that the specific surface area , and especially the intrinsic acidity constant, determine whether the ternary surface complex is easily formed, and that factor, FTSC,quantifies the relationship between the promoting effect of organics on Mt-marine solid particle ion exchange and the intrinsic acidity constant and specific surface area. 相似文献
10.
可变电荷土壤和恒电荷土壤与氢离子相互作用机理 总被引:2,自引:4,他引:2
研究了可变电荷土壤和恒电荷土壤与H相互作用的机理,并比较了它们之间的差别,研究结果表明,氢离子输入土壤后可以转化为表面正电荷,可溶性铝和可交换性酸,但是由于土壤的组成和性质不同,不同土壤中H+三种去向的贡献不同。H+转化为表面正电荷是由于土壤表面Fe-OH,Al-OH的质子化造成的,因此H+转化为表面正电荷的能力与土壤中氧化铁的含量密切相关,从而可变电荷土壤中H+转化为表面正电荷的贡献比恒电荷土壤中的大。H+转化为可溶性铝的能力与土教育部 的矿物组成密切相关,随着H+输入量的增加,土壤中可溶性铝的含量也增加。可变电荷土壤中可溶性铝增加的顺序为红壤>赤红壤>铁质砖红壤,在H+的加入量小于15mmol/kg时,黄棕壤的可溶性铝介于红壤和赤红壤之间,当H+的加入量大于约15mmol/kg时,黄棕壤的可溶性铝略小于赤红壤,棕壤的可溶性铝明显小于红壤和赤红壤,但比铁质砖红壤高,恒电荷土壤的可变性酸量明显大于可变电荷土壤,但从总的看来,H+加入量的变化对可交换性酸量的影响不大。 相似文献