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1.
Atmospheric dust is an integral component of the Earth system with major implications for the climate, biosphere and public health. In this context, identifying and quantifying the provenance and the processes generating the various types of dust found in the atmosphere is paramount. Isotopic signatures of Pb, Nd, Sr, Zn, Cu and Fe are commonly used as sensitive geochemical tracers. However, their combined use is limited by the lack of (a) a dedicated chromatographic protocol to separate the six elements of interest for low‐mass samples and (b) specific reference materials for dust. Indeed, our work shows that USGS rock reference materials BHVO‐2, AGV‐2 and G‐2 are not applicable as substitute reference materials for dust. We characterised the isotopic signatures of these six elements in dust reference materials ATD and BCR‐723, representatives of natural and urban environments, respectively. To achieve this, we developed a specific procedure for dust, applicable in the 4–25 mg mass range, to separate the six elements using a multi‐column ion‐exchange chromatographic method and MC‐ICP‐MS measurements.  相似文献   
2.
Dust, as a source of trace metal elements, affects the health of society. The spatial and temporal concentrations of dust‐bound trace metals (Cd, Pb, Ni, Zn, Cu, and Mn) in Kuhdasht watershed (456 km2), Lorestan Province, Iran, is investigated. Dust is collected using glass traps placed in ten research stations in the region. The spatial and temporal distribution of dust trace metals are plotted using ARC‐GIS. The highest and the lowest concentrations of Zn (9751150 mg kg?1), Pb (46.352.9 mg kg?1), and Cd (2.443.30 mg kg?1) are obtained in winter, of Ni (98110 mg kg?1) and Cu in autumn (16.053.5 mg kg?1), and of Mn in summer (385505 mg kg?1). The spatial concentrations of dust‐bound trace metals indicate all, except Cu, show a decreasing trend from the mountains toward the plains, similar to that of soil and of dust, except for Zn, which shows higher concentrations in dust than in soil. The potential sources of dust‐bound trace metals and their rate of contamination are also investigated using the enrichment and contamination factors. The major sources of Cd and Zn in the dust of watershed are due to anthropogenic activities or from activities outside the borders.  相似文献   
3.
叶翔  李靖  王爱军 《海洋学报》2018,40(7):79-89
滨海湿地作为人类活动和全球变化反应最为敏感的区域,其沉积记录可以反映出周边地区环境变化及人类活动信息。珠江口淇澳岛滨海湿地钻孔分析结果表明,在中全新世期间淇澳岛附近海域为河口湾环境,在风化层以上开始出现淤积,但在4 200 a BP前后受极冷气候的影响,沉积物粗化;自2 500 a BP以来,沉积环境相对稳定,在小冰期期间略有变化。沉积速率计算结果显示:淇澳岛附近海域自中全新世高海面以来的平均沉积速率为0.29 cm/a,4 160~2 500 a BP、2 500 a BP-1488年、1488-1893年、1893-1986年、1990-2007年期间的平均沉积速率分别为:0.17 cm/a、0.23 cm/a、0.35 cm/a、1.37 cm/a和5.94 cm/a,沉积速率逐渐增大,反映了珠江三角洲演化过程中沉积相与沉积环境的变化;1986-1990年期间的海堤建造极大地扰动了该钻孔上部的沉积过程,在工程施工期间共沉积了厚度约112 cm的沉积层,而在海堤建成后,沉积速率也显著增大。沉积物总有机碳、总氮和C/N值的垂向分布表明,在4 160~2 500 a BP期间受海洋环境影响较大,沉积物中有机碳以海源为主,2 500 a BP以来沉积物中碳、氮含量明显增大,C/N也相应变大,有机碳主要来源于陆源输入,但在小冰期期间海源有机碳贡献略有所增大;近百年来由于受人类活动影响显著,陆源有机碳的贡献快速增加。  相似文献   
4.
张涵  黎夏  石洪  刘晓娟 《地理学报》2021,76(3):680-693
科学地评估自然保护区缓解人类活动压力的效果,对于有效的自然保护至关重要。目前中国国家尺度下的这方面研究,仅将保护区内、外的人类活动压力进行对比,其缺陷是样本选择性偏差会导致评估结果的不合理。本文选择了倾向得分匹配(Propensity Score Matching)方法来克服保护区评价中的样本选择性偏差问题。首先耦合多源数据构建了2013年、2015年、2017年的人类活动压力指数,然后采用倾向得分匹配方法对自然保护区内、外的随机点进行匹配,使两个对比组的观测变量尽可能相似。最后通过相对有效性指标和面板模型从不同层面评估了中国680个自然保护区在2013—2017年间缓解人类活动压力的效果。研究结果表明:① 2013—2017年,全国86.72%的自然保护区内人类活动压力指数呈现上升趋势,其面积占保护区总面积的43.80%。② 69.85%的自然保护区在缓解人类活动压力方面的效果较好。其中,除了海洋海岸、野生植物、野生动物类的保护区以外,其余保护区类型都表现出较好的缓解人类活动压力的效果,且保护区级别越高,保护效果越好。③ 中国自然保护区建设在2013—2017年间能缓解22.90%的人类活动压力,且保护区缓解人类活动压力的能力存在区域性差别。本文研究结果可为中国自然保护区监测、评估和管理提供更科学的参考依据。  相似文献   
5.
长江口扁担沙动力地貌变化过程研究   总被引:1,自引:0,他引:1  
河口浅滩不仅为人类提供宝贵湿地资源,而且是调控河势演变的重要因素。研究河口浅滩动力地貌演变规律对航道整治、湿地生态开发及岸堤防护等具有重要价值。本文利用最近150多年的长江口历史海图资料、实测水深与水文泥沙数据,分析长江口南支最大的浅滩—扁担沙动力地貌演变格局及其变化机制。结果表明:(1) 1860?2016年期间,扁担沙反复历经淤积?冲刷?淤积,浅滩由最初水下阴滩发育出露而形成纺锤状沙体,随后演变为细长扁担状,沙尾切滩成爪状沙体,下扁担沙则伴随爪状缝隙被不断填充而淤长;(2)自1954年洪水到目前,扁担沙?2 m、?5 m等深线包络的面积与体积整体上均呈现增长态势,其中面积年均增长率分别为0.88 km2/a和0.81 km2/a,体积年均增长率分别为1.3×106 m3/a和5×106 m3/a;扁担沙浅滩在不同时期冲淤变化不同,其中1998年出现大幅度冲刷,平均冲刷厚度达到1.4 m;(3)扁担沙体积变化和长江入海泥沙的增减无直接联系,但与入海径流量的变化密切相关;(4)白茆沙“南强北弱”的河势、南北港分流工程以及东风西沙水库的建立导致扁担沙向北推移。  相似文献   
6.
The release of excessive anthropogenic nitrogen contributes to global climate change, biodiversity loss, and the degradation of ecosystem services. Despite being an urgent global problem, the excess nitrogen is not governed globally. This paper considers possible governance options for dealing with excessive nitrogen through target setting, which is an approach commonly adopted to address global environmental problems. The articulation of the nitrogen problem and the numerous international institutions dealing with it, provide evidence of a nitrogen regime characterised by limited coordination and targets covering sources and impacts only partially. This calls for improving the nitrogen governance in the direction of more integrated approaches at the global scale. In this vein, the paper investigates two opposite governance options – here labelled as ‘holistic’ and ‘origin-based’ – and evaluates them for their capability to define solutions and targets for human-induced nitrogen. From the analysis, it emerges that origin-based solutions can be preferable to holistic solutions as they can be more specific and potentially have greater immediate results. Independent from which governance arrangement is chosen, what matters most is the speed at which an arrangement can deploy solutions to combat (fast-growing) nitrogen pollution.  相似文献   
7.
为减少不同气候模式评估气溶胶气候效应的差异,第六次耦合模式比较计划(Coupled Model Intercomparison Project Phase 6,CMIP6)直接给定了人为气溶胶强迫数据。因此,有必要基于此强迫数据重新评估气溶胶气候效应。本研究首先将CMIP6给出的描述人为气溶胶强迫的模块引入南京信息工程大学(Nanjing University of Information Science and Technology,NUIST)的地球系统模式(The NUIST Earth System Model,NESM)。之后,利用NESM模式评估地球辐射收支平衡对此人为气溶胶强迫的响应,并分析模式模拟结果的不确定性。评估给出的人为气溶胶有效辐射强迫为-0. 45(±0. 28) W·m~(-2)。其中,气溶胶直接辐射效应为-0. 34(±0. 01) W·m~(-2),与第二次气溶胶比较计划(The second phase of Aerosol Comparisons between Observations and M odels,Aero ComⅡ)的评估结果基本一致;气溶胶对云辐射强迫的影响(包括半直接效应和间接效应)为-0. 10(±0. 30) W·m~(-2),明显受到模式内部变率的干扰,具有较大的不确定性。  相似文献   
8.
We simulated the impact of anthropogenic heat release (AHR) on the regional climate in three vast city agglomerations in China using the Weather Research and Forecasting model with nested high-resolution modeling.Based on energy consumption and high-quality land use data,we designed two scenarios to represent no-AHR and current-AHR conditions.By comparing the results of the two numerical experiments,changes of surface air temperature and precipitation due to AHR were quantified and analyzed.We concluded that AHR increases the temperature in these urbanized areas by about 0.5℃-1℃,and this increase is more pronounced in winter than in other seasons.The inclusion of AHR enhances the convergence of water vapor over urbanized areas.Together with the warming of the lower troposphere and the enhancement of ascending motions caused by AHR,the average convective available potential energy in urbanized areas is increased.Rainfall amounts in summer over urbanized areas are likely to increase and regional precipitation patterns to be altered to some extent.  相似文献   
9.
Distribution and sources of heavy metals in the sediment of Xiangshan Bay   总被引:2,自引:0,他引:2  
Heavy metals in the surface sediments and sediment core from the Xiangshan Bay, a mariculture base on the coast of the East China Sea, were determined by inductively coupled plasma mass spectrometry(ICP–MS) in order to evaluate their levels and sources. The results showed that the levels of Cu, Pb, Zn, and Cr in the sediments of the bay have been generally influenced by anthropogenic inputs since the founding of the People's Republic of China. In particular, Cu and Zn were polluted to some extent, as evidenced by high enrichment factors. Organic matter, grain size, wastewater discharge, and low energy hydrodynamic environment played dominant roles in the heavy metal enrichment in the sediments. The ratio of terrigenous source to marine biogenic deposit of trace metals in the sediments was calculated, revealing that terrigenous inputs were the main source of Cu, Pb, and Zn, while biological pellets contributed much more to the enrichment of Cr and Cd. Considering the influence of biological sources on the enrichment of Cd and Cr, and the fact that the sediment has been polluted by Cu and Zn, the development of mariculture and discharge of wastewater into the Bay should be restricted.  相似文献   
10.
This study has investigated the use of the artificial sweetener acesulfame and the magnetic resonance imaging contrast agent gadolinium as quantitative tracers for river water infiltration into shallow groundwater. The influence of a river on alluvial groundwater in a subalpine catchment in western Europe has been assessed using the ‘classical’ hydrochemical tracer chloride and the trace contaminants acesulfame and anthropogenic gadolinium. Mixing ratios for riverine bank filtrate with ambient groundwater and the uncertainties associated with the temporal and spatial tracer variability were calculated using acesulfame and gadolinium and compared with those obtained using chloride. The temporal variability of tracer concentrations in river water of gadolinium (standard deviation SD: 63%) and acesulfame (SD: 71%) both exceeded that of chloride (SD: 27%), and this was identified as the main source of uncertainty in the mixing analysis. Similar spatial distributions were detected in the groundwater for chloride and gadolinium, but not for acesulfame. Mixing analyses using acesulfame resulted in calculated mixing ratios that differed from those obtained using gadolinium and chloride by up to 83% and 92%, respectively. At the investigated site, which had oxic conditions and moderate temperatures, acesulfame was found to be a less reliable tracer than either gadolinium or chloride, probably because of natural attenuation and input from other sources. There was no statistically significant difference between the mixing ratios obtained using chloride or gadolinium, the mixing ratios obtained using gadolinium were 40–50% lower than those obtained using chloride. This is mainly due to a bias of the mean gadolinium concentration in river water towards higher values. In view of the uncertainties of the two tracers, neither could be preferred over the other for the quantification of bank filtrate in groundwater. At this specific site gadolinium was able to reliably identify river water infiltration and was a more precise tracer than chloride at low mixing ratios (<20%), because of the exclusive occurrence of gadolinium in river water and its high dynamic range. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   
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