Effects of Solid Organic Wastes on Soil Particulate Organic Carbon Structure Under Different Water Conditions     

Xiaojing Qu  Jinggui Wu  Jinghong Zhao  Jianming Li  Juan Hu  Opoku‐Kwanowaa Yaa 《洁净——土壤、空气、水》2019,47(8)

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Heavy metals in particulate and colloidal matter from atmospheric deposition of urban Guangzhou,South China     

Wen Huang  Dandan Duan  Yulong Zhang  Hefa Cheng  Yong Ran 《Marine pollution bulletin》2014

Suspended particulate matter (SPM) and colloidal matter (COM) in annual dry and wet deposition samples in urban Guangzhou were for the first time collected, and their trace metals were investigated by using inductively coupled plasma mass spectrometry (ICP-MS). The deposition flux of SPM and of metal elements varied largely among the investigated seasons, and reached the maximum in spring. The correlation analysis indicated that significant correlations existed among some of the metal elements in the deposition samples. The enrichment factors (EF) of metals in COM in the deposition ranging from 79.66 to 130,000 were much higher than those of SPM ranging from 1.65 to 286.48, indicating the important role of COM. The factor analysis showed that emissions from street dust, non-ferrous metal production, and heavy fuel oil were major sources of the trace metals. Positive matrix factorization (PMF) model was used to quantitatively estimate anthropogenic source.  相似文献   

Combining two filter paper‐based analytical methods to monitor temporal variations in the geochemical properties of fluvial suspended particulate matter          下载免费PDF全文

R. J. Cooper  B. G. Rawlins  B. Lézé  T. Krueger  K. M. Hiscock 《水文研究》2014,28(13):4042-4056

Many of the commonly used analytical techniques for assessing the properties of fluvial suspended particulate matter (SPM) are neither cost effective nor time efficient, making them prohibitive to long‐term high‐resolution monitoring. We present an in‐depth methodology utilizing two types of spectroscopy which, when combined with automatic water samplers, can generate accurate, high‐temporal resolution SPM geochemistry data, inexpensively and semi‐destructively, directly from sediment covered filter papers. A combined X‐ray fluorescence spectroscopy and diffuse reflectance infrared Fourier transform spectroscopy approach is developed to estimate concentrations for a range of elements (Al, Ca, Ce, Fe, K, Mg, Mn, Na, P, Si, Ti) and compounds (organic carbon, Al_dithionate, Al_oxalate, Fe_dithionate, and Fe_oxalate) within SPM trapped on quartz fibre filters at masses as low as 3 mg. Calibration models with small prediction errors are derived, along with mass correction factor models to account for variations in retained SPM mass. Spectral pre‐processing methods are shown to enhance the reproducibility of results for some compounds, and the importance of filter paper selection and homogeneous sample preparation in minimizing spectral interference is emphasized. The geochemical signal from sediment covered filter papers is demonstrated to be time stable enabling samples to be stored for several weeks prior to analysis. Example results obtained during a heavy precipitation event in October 2012 demonstrate the methodology presented here has considerable potential to be utilized for high‐resolution monitoring of SPM geochemistry under a range of in‐stream hydrological conditions. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

安徽省大气颗粒物污染特征分析     

易明建  邓淑梅  汪水兵  卫尤文  戴海夏 《地球化学》2021,50(1):36-45

对2016年全年颗粒物监测浓度数据进行统计分析,得到了安徽省颗粒物污染的空间分布、浓度和粒径,以及污染传输特征。结果表明,淮河以北、沿江和江淮之间、长江以南和皖南山区城市颗粒物污染随地理位置不同表现出明显的区域化特征,污染程度由北向南减轻,污染过程明显表现出由北向南逐步扩散传输的规律,污染程度越重,污染深入南方的范围越广,持续时间也越长。冬季污染较重的城市,上午出现明显的高浓度时段,全天变化为“双峰双谷”型。夏、秋季节夜间细颗粒物(PM2.5)浓度贡献比增加。PM2.5与PM10(可吸入颗粒物)质量浓度比值冬季最高,春季较低。污染重的城市冬季PM2.5占比高。  相似文献   

乌鲁木齐市PM10,PM2.5和PM1.0浓度及分布变化特征研究     

韩茜  魏文寿  刘新春  钟玉婷 《沙漠与绿洲气象(新疆气象)》2015,9(1):32-38

利用GRIMM180气溶胶粒谱分析仪采集乌鲁木齐市PM10、PM2.5和PM1.0数据,研究表明:乌鲁木齐市气溶胶颗粒物质量浓度在进入采暖季后急剧增加,冬季颗粒物中细粒子含量最高,PM2.5/PM10可达77.6%,PM2.5/PM10,PM1.0/PM10,PM1.0/PM2.5三比值体现了颗粒物的分布特征,四季污染程度越高,细粒子含量越高。四季无降水日PM10、PM2.5、PM1.0的质量浓度和分布的日变化基本呈三峰三谷型,出现早—午—晚峰值,上午—下午—午夜后谷值,各季节峰谷值具体出现时间略有差别,由于冬季逆温层顶盖等因素的影响,冬季质量浓度和分布的日变化在此基础上多了两次波动。降水的发生对冬、春季质量浓度的影响大于夏、秋季,对不同粒径段粒子的分布影响有一定差别。  相似文献   

Distribution of suspended particulate matter in the northern Bohai Bay in summer and its relation with thermocline     

L.L. Qiao  Y.Z. Wang  G.X. Li  S.G. Deng  Y. Liu  L. Mu 《Estuarine, Coastal and Shelf Science》2011

Field observations of suspended particulate matter (SPM) in the Bohai Bay, China have not been widely reported. The aim of this paper is to describe the horizontal and vertical distribution of mass and volume concentrations of SPM, respectively, based on observed data at 312 stations in the northern Bohai Bay during summer of 2006. A numerical model ECOMSED coupled with a sediment transport module was also established to further discuss the mechanism of the thermocline effect on the vertical distribution of SPM. The mass concentrations of SPM exhibited high inshore values and low offshore values in the horizontal distribution; while in the vertical direction, characteristics of the volume concentration of SPM can be divided into two types: one with a sharp peak at depth of 10–15 m and another without. The peak value at the depth of the thermocline was resulted from concentrated phytoplankton. A numerical experiment further displayed that the thermocline can also prevent particles from being resuspended upward.  相似文献   

Origin and biochemical cycling of particulate nitrogen in the Mandovi estuary   总被引：2，自引：0，他引：2  

Loreta Fernandes 《Estuarine, Coastal and Shelf Science》2011,94(3):291-298

Mandovi estuary is a tropical estuary strongly influenced by the southwest monsoon. In order to understand, sources and fate of particulate organic nitrogen, suspended particulate matter (SPM) collected from various locations, was analyzed for particulate organic carbon (POC) and particulate organic nitrogen (PON), δ¹³C_POC, total hydrolysable amino acid enantiomers (l- and d- amino acids) concentration and composition. δ¹³C_POC values were depleted (−32 to −25‰) during the monsoon and enriched (−29.6 to −21‰) in the pre-monsoon season implying that OM was derived from terrestrial and marine sources during the former and latter season, respectively. The biological indicators such as C/N ratio, d-amino acids, THAA yields and degradation indices (DI) indicate that the particulate organic matter (POM) was relatively more degraded during the monsoon season. Conversely, during the pre-monsoon, the biological indicators indicated the presence of relatively fresh and labile POM derived from autochthonous sources. Amino acids such as alanine, aspartic acid, leucine, serine, arginine, and threonine in monsoon and glutamic acid, glycine, valine, lysine, and isoleucine in pre-monsoon were relatively abundant. Presence of bacterial biomarker, d-amino acids in the SPM of the estuary during both the seasons signifies important contribution of bacteria to the estuarine detrital ON pool. Based on d-amino acid yields, bacterial OM accounted for 16-34% (23.0 ± 6.7%) of POC and 29-75% (47.9 ± 18.7%) of PON in monsoon, and 30-78% (50.0 ± 15%) of POC and 34-79% (51.2 ± 13.3%) of the PON in pre-monsoon in the estuary. Substantial contribution of bacterial-N to PON indicates nitrogen (N) enrichment on terrestrial POM during the monsoon season. Transport of terrestrial POM enriched with bacterial OM to the coastal waters is expected to influence coastal productivity and ecosystem functioning during the monsoon season.  相似文献   

长江口跨越锋面颗粒磷季节分布变化特征及影响因素   总被引：1，自引：0，他引：1  

刘希真  李宏亮  陈建芳  金海燕  王文亮  刘际弟  王奎  庄燕培 《海洋学研究》2011,(3):88-98

根据2006年夏、冬季以及2007年春、秋季“海监49号”科学考察船的调查数据,分析了长江口跨越锋面区域(31.00°～31.78°N、121.04°～123.99°E)颗粒总磷(PP),颗粒无机磷(PIP),颗粒有机磷(POP)的季节变化和空间分布特征.结果表明,PIP是水体颗粒磷的主要存在形式;受长江径流输沙量的影...  相似文献   

塔克拉玛干沙漠腹地沙尘暴过程大气颗粒物浓度及影响因素分析   总被引：1，自引：0，他引：1  

刘新春  钟玉婷  何清  艾力·买买提明 《中国沙漠》2011,31(6):1548-1553

 利用Grimm1.108、Thermo RP 1400a、TSP以及CAWS-600等仪器,对2008年4月17日至23日发生在塔克拉玛干沙漠腹地的1次强沙尘暴过程的颗粒物质量浓度进行连续观测,结合天气资料分析得出:①Grimm1.108颗粒物分析仪监测结果表明,日平均浓度出现两个峰值区,主峰值出现在20日,次峰值出现在18日,而小时平均浓度高值区主要集中4月19日至20日,21日中午存在1个峰值区,其他时段浓度相对较低。②强沙尘暴发生时的分钟观测数据表明,随着风速的逐渐增强,沙尘暴强度逐渐增强,不同粒径颗粒物浓度达到最大值,>0.23 μm颗粒物总浓度为39 496.5 μg·m-3,>20.0 μm颗粒物总浓度为5 390.7 μg·m-3,随后浓度逐渐下降。③PM10和TSP的浓度变化同样反映沙尘天气的过程和强度,沙尘暴前期大气中颗粒物浓度远低于强沙尘暴期间,随沙尘天气减弱,颗粒物浓度明显下降。④沙尘天气过程中大气颗粒物浓度变化具有以下规律：晴天<浮尘天气<浮尘、扬沙天气<沙尘暴天气。风速大小直接影响大气中颗粒物浓度,风速越大颗粒物浓度越高。气温、相对湿度和气压是影响沙尘暴强度的重要因素,也间接影响大气中颗粒物浓度的变化。  相似文献   

太湖流域昆承湖春季颗粒物和有色可溶性有机物吸收特性   总被引：4，自引：1，他引：3  

柳彩霞  郭子祺  张宝钢  雷霞  马茵驰 《湖泊科学》2011,23(5):773-782

利用2010年4月23日在昆承湖采集的水体吸收系数数据,对总悬浮物颗粒物、浮游植物色素颗粒物、非色素颗粒物和有色可溶性有机物的吸收特征进行研究.结果表明,春季昆承湖水体除675 nm附近具有叶绿素吸收峰的红光波段外,非色素颗粒物吸收系数大于浮游植物色素颗粒物吸收系数,总颗粒物吸收系数光谱分布与非色素颗粒物的吸收光谱类似...  相似文献