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《Applied Geochemistry》2003,18(10):1507-1515
Adsorption studies have been conducted at pH 4, 6 and 8 to assess the effect of fulvic acid on arsenate adsorption to ferrihydrite and gibbsite. The studies compared the adsorption of arsenate on the mineral surfaces in the absence of fulvic acid, to those cases where increasing concentrations of fulvic acid (0.3–60 μM) were added to the mineral–arsenate suspensions. Experiments where arsenate was added to mineral–fulvate suspensions were also conducted. The results suggest that arsenate adsorption on both gibbsite and ferrihydrite decreases with increasing concentrations of fulvic acid. This effect was highest at pH 4, and decreased at pH 6 and 8. Ferrous ion concentrations were very low during the ferrihydrite experiments and support the view that fulvic acid can both displace arsenate from and inhibited its adsorption to mineral surfaces. The experiments also indicated that the amount of arsenate adsorbed was lower if fulvic acid was added before rather than after arsenate. This may reflect the relative size of arsenate and fulvic acid molecules and their ability to penetrate the crystal matrices of the minerals. 相似文献
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Despite important progress on Amazonian floodplain research, the flooded forest of the Negro River “igapó” has been little investigated. In particular, no study has previously focused the linkage between fluvial geomorphology and the floristic variation across the course of the river. In this paper we describe and interpret relations between igapó forest, fluvial geomorphology and the spatial evolution of the igapó forest through the Holocene. Therefore, we investigate the effect of geomorphological units of the floodplain and channel patterns on tree diversity, composition and structural parameters of the late-successional igapó forest. Our results show that sites sharing almost identical flooding regime, exhibit variable tree assemblages, species richness and structural parameters such as basal area, tree density and tree heights, indicating a trend in which the geomorphologic styles seem to partially control the organization of igapó's tree communities. This can be also explained by the high variability of well-developed geomorphologic units in short distances and concentrated in small areas. In this dynamic the inputs from the species pool of tributary rivers play a crucial role, but also the depositional and erosional processes associated with the evolution of the floodplain during the Holocene may control floristic and structural components of the igapó forests. These results suggest that a comprehensive approach integrating floristic and geomorphologic methods is needed to understand the distribution of the complex vegetation patterns in complex floodplains such as the igapó of the Negro River. This combination of approaches may introduce a better comprehension of the temporal and spatial evolutionary analysis and a logic rationale to understand the vegetation distribution and variability in function of major landforms, soil distributions and hydrology. Thus, by integrating the past into macroecological analyses will sharpen our understanding of the underlying forces for contemporary floristic patterns along the inundation forests of the Negro River. 相似文献
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How freezing and thawing processes affect black-soil aggregate stability in northeastern China 总被引：2，自引：0，他引：2
Laboratory experiments were carried out to investigate the effect of freezing and thawing processes on wet aggregate stability （WAS） of black soil. Wet aggregate stability was determined by different aggregate size groups, different water contents, various freeze-thaw cycles, and various freezing temperatures. The results showed that, when at suitable water content, aggregate stability was enhanced, aggregate sta-bility will be disrupted when moisture content is too high or too low, especially higher water content. Temperature also had a significant ef-fect, but moisture content determined the suitable freezing temperatures for a given soil. Water-stable aggregate （WSA〉0.5）, the total aggre-gate content, and mean weight diameter decreasing with the freeze-thaw cycles increase, reached to 5 percent significance level. The reason for crumbing aggregates is the water and air conflict, thus raising the hypothesis that water content affects the aggregate stability in the process of freezing and thawing. 相似文献
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不同水生植物对富营养化水体无机氮吸收动力学特征 总被引：3，自引：2，他引：1
采用浓度梯度法,研究了鸢尾(Iris louisiana)、狐尾藻(Myriophyllum verticillatum)、茭白(Zizania latifolia)和水芹(Oenanthe clecumbens)对硝态氮(NO3--N)和铵态氮(NH4+-N)吸收动力学特征.结果表明:4种水生植物对水体NO3--N和NH4+-N吸收可用Michaelis-Menten酶动力学方程描述,随溶液NO3--N和NH4+-N浓度增加,植物吸收NO3--N和NH4+-N速率增加,当溶液NO3--N和NH4+-N浓度接近于2.0 mmol/L时,吸收速率增加趋缓;4种水生植物对NO3--N和NH4+-N的Vmax值大小为水芹 >茭白 >鸢尾 >狐尾藻,对NO3--N的Km值大小为水芹 >鸢尾=茭白=狐尾藻,对NH4+-N的Km值大小为水芹 >狐尾藻 >茭白=鸢尾.根据吸收动力学参数(Vmax,Km)判断水芹适宜于净化NO3--N和NH4+-N浓度较高的水体,茭白、鸢尾和狐尾藻适合净化NO3--N和NH4+-N浓度较低水体;4种水生植物对NO3--N、NH4+-N表现出不同的吸收偏好性,鸢尾吸收NO3--N的潜力大于吸收NH4+-N的,但对NH4+-N的亲和力大于NO3--N,表明能在NO3--N浓度较高环境中优先吸收NH4+-N.狐尾藻和水芹对NO3--N和NH4+-N能均衡吸收.茭白对NH4+-N具有较高的吸收潜力与亲和力. 相似文献
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