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1.
李映葵  曹建劲  陈杰  易杰 《岩石学报》2017,33(3):831-842
为探讨上升气流微粒与深部隐伏矿体之间关系,在广西清明山铜镍硫化物矿床上方土壤中采集上升气流微粒,并采用透射电子显微镜(TEM)对微粒的形貌、大小、聚合状态、化学组分及结构等进行分析。结果表明,微粒主要由Cu、Co、Zn、Fe、Ca、Si、S等元素组成,其中成矿元素Cu、Co以自然Cu-Fe-Co、Zn-Fe-Co及Fe-Co合金微粒的形式存在,其余如Fe、Ca、Si、S等元素则以氢氧化物、氧化物及碳酸盐微粒形式存在。微粒可分为微粒聚合体及单个微粒,微粒的大小为50~500nm,微粒的形状多为不规则状、近椭圆形、近球状、水滴状和近长方体等。微粒中高含量的Cu、Co、Zn来源于深部隐伏矿体,含Fe、S微粒来源于矿床中金属硫化物矿物。此外,高价态的微粒组分指示微粒处于相对氧化的环境。清明山铜镍硫化物矿床的上升气流微粒组分与矿床矿物组分间存在着较好的对应性,本研究为隐伏铜镍硫化物矿床提供了新的找矿方法。  相似文献   
2.
细颗粒物(PM2.5)即粒径小于2.5μm的可吸入颗粒物[1],是当今中国城市大气污染的首要污染物。本研究以北京市为例,选取北京市2010年至2012年三年内采暖期与非采暖期两个不同时期的细颗粒物(PM0.3,PM0.5,PM1)实测数据,及同时期北京市患呼吸系统疾病人数数据,运用地统计的空间分析方法,对获取数据进行空间化及插值研究。通过偏相关分析法对北京市细颗粒物浓度与患呼吸系统疾病人数数据进行相关分析。得出以下主要结论:①细颗粒物的空间变化明显,2010年、2011年及2012年细颗粒物浓度整体呈上升趋势,2012年三种粒径细颗粒物浓度整体高于2010年与2011年。②不同粒径的细颗粒物,对呼吸疾病的影响程度不同:在0.3μm,0.5μm与1μm三种粒径的细颗粒物中,PM1对呼吸系统疾病影响最大,偏相关系数达到0.785。  相似文献   
3.
The statistics of the horizontal component of the water particle velocity vector under random waves are considered. A spread in the directions of travel of the component wave trains does not affect the rms value of the modulus r but it affects the shape of its probability distribution in such a way that the pr3bability of extreme values is reduced. For small and moderate directional spreads the modulus for a given probability of exceedance is reduced by a factor which tends to Fs as the probability of exceedance tends to zero, where Fs is the spread factor (which is typically 0.9 in temperate storms). However, the convergence on this asymptote is not complete for probabilities of engineering importance, particularly for wide directional spreads. The standard deviation of the probability distribution of the direction of the vector is reduced roughly in inverse proportion to r. The same conclusions apply to particle accelerations.  相似文献   
4.
东胜区污染状况分析   总被引:1,自引:0,他引:1  
文章利用东胜区主要污染源排放情况以及2005年9月1日-2007年8月31日每日SO2、NO2、PM10浓度监测值和2005-2007年SO2、NO2、PM10平均值,分析了东胜区主要污染类型、污染物来源以及东胜区近3年SO2、NO2、PM10监测值日、月、季、年分布特征和变化规律;提出了消减大气污染物排放的对策。  相似文献   
5.
The contribution of emissions from agricultural facilities is rapidly becoming a major concern for local and regional air quality. Characterization of particle properties such as physical size distribution and chemical composition can be valuable in understanding the processes contributing to emissions and ultimate fate of particulate matter from agricultural facilities. A measurement campaign was conducted at an Iowa, deep-pit, three-barn swine finishing facility to characterize near-source ambient particulate matter. Size-specific mass concentrations were determined using minivol samplers, with additional size distribution information obtain using optical particle counters. Particulate composition was determined via ion chromatographic analysis of the collected filters. A thermal-CO2 elemental/organic carbon analyzer measured particulate carbon. The chemical composition and size distribution of sub-micron particles were determined via real-time aerosol mass spectrometry. Primary particulate was not found to be a major emission from the examined facility, with filter-based impactor samples showing average near-source increases (~15–50 m) in ambient PM10 of 5.8 ± 2.9 μg m−3 above background levels. PM2.5 also showed contribution attributable to the facility (1.7 ± 1.1 μg m−3). Optical particle counter analysis of the numerical size distributions showed bimodal distributions for both the upwind and downwind conditions, with maximums around 2.5 μm and below the minimum quantified diameter of 0.3 μm. The distributions showed increased numbers of coarse particles (PM10) during periods when wind transport came from the barns, but the differences were not statistically significant at the 95% confidence level. The PM10 aerosols showed statistically increased concentrations of sulfate, nitrate, ammonium, calcium, organic carbon, and elemental carbon when the samplers were downwind from the pig barns. Organic carbon was the major constituent of the barn-impacted particulate matter in both sub-micron (54%) and coarse size (20%) ranges. The AMS PM1 chemical speciation showed similar species increases, with the exception of and Ca+2, the latter not quantified by the AMS.  相似文献   
6.
The physical and chemical properties of aerosol particles were investigated at Plan d'Aups, one of the ESCOMPTE sites located in the St. Baume mountain area (700 m a.s.l.), 50 km east of Marseilles (France). The site is ideally located for assessing the vertical and horizontal extent of the pollution plume from the Marseilles–Berre area.Our study showed that polluted air masses from the Marseilles–Berre area are advected to Plan d'Aups in the early afternoon. Average daily concentration of particles reaches up to 40 μg m−3 while 1-h average particle number concentration is greater than 30,000 cm−3. Most of the particle mass is composed of SO42− and organic carbon (OC). The chemical properties of the particles revealed that an additional source, possibly from the industrial area of Gardanne, contributes to the aerosol mass. This last source is characterised by significant emissions of elements, such as Zn, V, Al and Si.In addition to transport, we found that gas-to-particle conversion takes place at the interface between the free troposphere and the boundary layer. We estimated that on average, 30% of the particle number is accounted for by direct nucleation. This is potentially a major aerosol source to the free troposphere.  相似文献   
7.
Hydrological processes are known to have a considerable effect on nutrient transport from agricultural land to watercourses. In cold temperate regions peak discharges are caused not only by storm conditions but also by melting of snow and frost. The objective of this work was to investigate the effects of snow and frost melt on concentrations of phosphorus and suspended solids. The samples were taken using flowweighted automatic sampling techniques from two agricultural drainage basins. During the beginning of the snowmelt period the concentration of suspended solids was rather low by comparison with the total phosphorus concentration and the discharge. The different behaviour compared with the relationships found during storm conditions was probably caused by continuous extraction of the soil surface by low ionic concentration melt water, and to some extent by leaching from plant residues. The gradual decrease of total phosphorus concentration during the frost thawing period could be attributed to the gradually increasing proportion of the subsurface and ground water discharge in the runoff.  相似文献   
8.
A new parameterisation for the threshold shear velocity to initiate deflation of dry and wet particles is presented. It is based on the balance of moments acting on particles at the instant of particle motion. The model hence includes a term for the aerodynamic forces, including the drag force, the lift force and the aerodynamic-moment force, and a term for the interparticle forces. The effect of gravitation is incorporated in both terms. Rather than using an implicit function for the effect of the aerodynamic forces as reported earlier in literature, a constant aerodynamic coefficient was introduced. From consideration of the van der Waals force between two particles, it was further shown that the effect of the interparticle cohesion force between two dry particles on the deflation threshold should be inversely proportional to the particle diameter squared. The interparticle force was further extended to include wet bonding forces. The latter were considered as the sum of capillary forces and adhesive forces. A model that expresses the capillary force as a function of particle diameter squared and the inverse of capillary potential was deduced from consideration of the well-known model of Fisher and the Young–Laplace equation. The adhesive force was assumed to be equal to tensile strength, and a function which is proportional to particle diameter squared and the inverse of the potential due to adhesive forces was derived. By combining the capillary-force model and the adhesive force model, the interparticle force due to wet bonding was simplified and written as a function of particle diameter squared and the inverse of matric potential. The latter was loglinearly related to the gravimetric moisture content, a relationship that is valid in the low-moisture content range that is important in the light of deflation of sediment by wind. By introducing a correction to force the relationship to converge to zero moisture content at oven dryness, the matric potential–moisture content relationship contained only one unknown model parameter, viz. moisture content at −1.5 MPa. Working out the model led to a rather simple parameterisation containing only three coefficients. Two parameters were incorporated in the term that applies to dry sediment and were determined by using experimental data as reported by Iversen and White [Sedimentology 29 (1982) 111]. The third parameter for the wet-sediment part of the model was determined from wind-tunnel experiments on prewetted sand and sandy loam aggregates. The model was validated using data from wind-tunnel experiments on the same but dry sediment, and on data obtained from simulations with the model of Chepil [Soil Sci. Soc. Am. Proc. 20 (1956) 288]. The experiments showed that soil aggregates should be treated as individual particles with a density equal to their bulk density. Furthermore, it was shown that the surface had to dry to a moisture content of about 75% of the moisture content at −1.5 MPa before deflation became sustained. The threshold shear velocities simulated with our model were found to be in good agreement with own observations and with simulations using Chepil's model.  相似文献   
9.
用欧亚大陆地面电离层垂测站资料考察1989年3月12~16日磁暴期间的电离层暴形态及其发展变化. 特强磁暴引发的电离层暴是全球性的,但自磁层沉降的高能粒子对热层低部的加热程度及区域分布不同,因而各经度链区域内电离层暴的特征也有所差异. 本文研究表明,与理论推断对照,欧洲地区内F2层最大电子密度NmaxF2(或f0F2)并不出现正暴现象,而负暴自高纬向低纬的发展则与典型的热层环流结果相符. 此外,此磁暴过程期间在中低纬区存在明显的波动过程. 在亚洲高纬地区,磁暴初期13日有约10 h的正暴,而负暴过程则与欧洲地区类似,但不太清晰;且无波动现象. 磁暴期间,同一经度链的中低纬地区,夜间常发生多站同时的h′F突增. 本文再次证实这是一般磁暴期间常出现的普遍现象.  相似文献   
10.
对流层平流层气溶胶粒子的形态和化学组成   总被引:13,自引:1,他引:12  
分析研究了1993年和1994年的8月、9月在香河地区上空采集的单个气溶胶粒子的形态及化学元素和化合物的组成。结果表明:1993年,在对流层大气中的气溶胶颗粒经常出现不规则形的粒子,可能是土壤粒子;而在平流层大气中的颗粒以具有“卫星”结构的硫酸粒子为主;硫酸铵粒子则经常出现在对流层的中、下部。香河地区上空颗粒物的化学元素组成比较复杂,单一化学元素组成的粒子较少,粒子主要含有Si,Fe,Al和S等元素。气溶胶的化合物有硫酸盐、硅酸盐、硝酸盐和磷酸盐等  相似文献   
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