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1.
Biomass burning in the tropical savannas of Ivory Coast: An overview of the field experiment Fire of Savannas (FOS/DECAFE 91) 总被引:1,自引:0,他引:1
J. P. Lacaux J. M. Brustet R. Delmas J. C. Menaut L. Abbadie B. Bonsang H. Cachier J. Baudet M. O. Andreae G. Helas 《Journal of Atmospheric Chemistry》1995,22(1-2):195-216
FOS/DECAFE 91 (Fire of Savannas/Dynamique et Chimie Atmosphérique en Forêt Equatoriale) was the first multidisciplinary experiment organized in Africa to determine gas and aerosol emissions by prescribed savanna fires. The humid savanna of Lamto in Ivory Coast was chosen for its ecological characteristics representative of savannas with a high biomass density (900 g m–2 dry matter). Moreover the vegetation and the climate of Lamto have been studied for more than twenty years. The emission ratios (X/CO2) of the carbon compounds (CO2, CO, NMHC, CH4, PAH, organic acids and aerosols), nitrogen compounds (NOx, N2O, NH3 and soluble aerosols) and sulfur compounds (SO2, COS and aerosols) were experimentally determined by ground and aircraft measurements. To perform this experiment, 4 small plots (100×100 m) and 2 large areas (10×10 km) were prepared and burnt in January 1991 during the period of maximum occurrence of fires in this type of savanna. The detailed ecological study shows that the carbon content of the vegetation is constant within 1% (42 g C for 100 g of vegetal dry matter), the nitrogen content (0.29 g N for 100 g of dry matter) may vary by 10% and the sulfur content (0.05 g S/100 d.m.) by 20%. These variations of the biomass chemical content do not constitute an important factor in the variation of the gas and particle emission levels. With the emission ratios characteristic of humid savanna and flaming conditions (CO/CO2 of 6.1% at the ground and 8% for airborne measurements), we propose a set of new emission factors, taking into account the burning efficiency which is about 80%: 74.4% of the carbon content of the savanna biomass is released to the atmosphere in the form of CO2, 4.6% as CO, 0.2% as CH4, 0.5% as NMHC and 0.7% as aerosols. 17.2% of the nitrogen content of the biomass is released as NOx, 3.5% as N2O, 0.6% as NH3 and 0.5% as soluble aerosols. 相似文献
2.
Günter Helas Jürgen Lobert Dieter Scharffe Luise Schäfer Johann Goldammer Jean Baudet Brou Ahoua Ayité-Lô Ajavon Jean-Pierre Lacaux Robert Delmas Meinrat O. Andreae 《Journal of Atmospheric Chemistry》1995,22(1-2):163-174
Ozone has been observed in elevated concentrations by satellites over areas previously believed to be background. There is meteorological evidence, that these ozone plumes found over the Atlantic Ocean originate from vegetation fires on the African continent.In a previous study (DECAFE-88), we have investigated ozone and assumed precursor compounds over African tropical forest regions. Our measurements revealed large photosmog layers at altitudes from 1.5 to 4 km. Both chemical and meteorological evidence point to savanna fires up to several thousand km upwind as sources.Here we describe ozone mixing ratios observed over western Africa and compare ozone production ratios from different field measurement campaigns related to vegetation burning. We find that air masses containing photosmog ingredients require several days to develop their oxidation potential, similar to what is known from air polluted by emissions from fossil fuel burning. Finally, we estimate the global ozone production due to vegetation fires and conclude that this source is comparable in strength to the stratospheric input. 相似文献
3.
4.
B. Tapley J. Ries S. Bettadpur D. Chambers M. Cheng F. Condi B. Gunter Z. Kang P. Nagel R. Pastor T. Pekker S. Poole F. Wang 《Journal of Geodesy》2005,79(8):467-478
A new generation of Earth gravity field models called GGM02 are derived using approximately 14 months of data spanning from
April 2002 to December 2003 from the Gravity Recovery And Climate Experiment (GRACE). Relative to the preceding generation,
GGM01, there have been improvements to the data products, the gravity estimation methods and the background models. Based
on the calibrated covariances, GGM02 (both the GRACE-only model GGM02S and the combination model GGM02C) represents an improvement
greater than a factor of two over the previous GGM01 models. Error estimates indicate a cumulative error less than 1 cm geoid
height to spherical harmonic degree 70, which can be said to have met the GRACE minimum mission goals.
Electronic Supplementary Material Supplementary material is available in the online version of this article at 相似文献
5.
The equilibrium water content of cordierite has been measured for 31 samples synthesized at pressures of 1000 and 2000 bars
and temperatures from 600 to 750° C using the cold-seal hydrothermal technique. Ten data points are presented for pure magnesian
cordierite, 11 data points for intermediate iron/magnesium ratios from 0.25 to 0.65 and 10 data points for pure iron cordierite.
By representing the contribution of H2O to the heat capacity of cordierite as steam at the same temperature and pressure, it is possible to calculate a standard
enthalpy and entropy of reaction at 298.18° K and 1 bar for,
(Mg,Fe)2Al4Si5O18+H2O ⇄ (Fe,Mg)2Al4Si5O18.H2O
Combining the 31 new data points with 89 previously published experimental measurements gives: ΔH
°
r
=–37141±3520 J and ΔS
°
r
=–99.2±4 J/degree. This enthalpy of reaction is within experimental uncertainty of calorimetric data. The enthalpy and entropy
of hydration derived separately for magnesian cordierite (–34400±3016 J, –96.5±3.4 J/degree) and iron cordierite (–39613±2475,
–99.5±2.5 J/degree) cannot be distinguished within the present experimental uncertainty. The water content as a function of
temperature, T(K), and water fugacity, f(bars), is given by n
H2O=1/[1+1/(K ⋅ f
H2O)] where the equilibrium constant for the hydration reaction as written above is, ln K=4466.4/T–11.906 with the standard state for H2O as the gas at 1 bar and T, and for cordierite components, the hydrous and anhydrous endmembers at P and T.
Received: 2 August 1994/Accepted: 7 February 1996 相似文献
6.
Norbert I. K 《冰川冻土》2004,26(Z1):310-318
The exploration of ice sheets by melting vertical holes into the ground has some tradition in terrestrial glaciology. Such probes have been used since the 1960's to investigate the vertical structure of the ice in Greenland and Antarctica and in alpine glaciers. In this paper we look into the possibility to develop similar devices for use on extraterrestrial icy bodies, like e.g. the polar areas on Mars or the icy satellites of the outer solar system. We report on some basic experiments performed in the cryo-vacuum laboratory of the Space Research Institute of the Austrian Academy of Sciences, Graz. In these experiments the penetration of a simple melting probe into compact and porous water ice (with a snow-like texture) was monitored, both under vacuum conditions and under air pressure. The observed penetration speeds for a given power supply are compared with a simple mathematical model. We conclude that a miniature melting probe with small overall dimensions and a reasonable power demand could well be part of the payload of a future planetary mission, for example to the poles of Mars. Such missions are currently under discussion in several space agencies. Moreover such probes could also e? ectively be used in terrestrial environments. A possible design is presented at the end of the paper. 相似文献
7.
Olga Didova Brian Gunter Riccardo Riva Roland Klees Lutz Roese-Koerner 《Journal of Geodesy》2016,90(11):1207-1221
8.
Two procedures for the calibration of an electron capture detector (ECD) for peroxyacetyl nitrate (PAN) are discussed. One is based on the first-order decay rate of the the PAN mixing ratio in conditioned glass storage vessels. The other method makes use of the photochemical generation of PAN in mixtures of acetone and NO2 in air. For this purpose a Penray Hg lamp was inserted into a glass vessel filled with 1 atmosphere of air containing 10 ppm NO2 and 1% acetone. After 3 min of irradiation, the average PAN mixing ratio formed was 8.87±0.25 ppmv as determined in six separate runs. 相似文献
9.
D. Perner U. Platt M. Trainer G. Hübler J. Drummond W. Junkermann J. Rudolph B. Schubert A. Volz D. H. Ehhalt K. J. Rumpel G. Helas 《Journal of Atmospheric Chemistry》1987,5(2):185-216
Using long path UV absorption spectroscopy we have measured OH concentrations close to the earth's surface. The OH values observed at two locations in Germany during 1980 through 1983 range from 0.7×106 to 3.2×106 cm-3. Simultaneously we measured the concentrations of O3, H2O, NO, NO2, CH4, CO, and the light non methane hydrocarbons. We also determined the photolysis rates of O3 and NO2. This allows calculations of OH using a zero dimensional time depdendent model. The modelled OH concentrations significantly exceed the measured values for low NO
x
concentrations. It is argued that additional, so far unidentified. HO
x
loss reactions must be responsible for that discrepancy. 相似文献
10.
Fourteen core samples of Precambrian granitic gneisses from a well drilled in the Green Township, Scioto County, Ohio were studied to determine the origin of alkali feldspar in these rocks. The well intersected the basement at a depth of 1,700 m and penetrated 11.3m of Precambrian crystalline rocks. Petrographically the samples in the upper 6.4 m of the basement core show evidence of severe alteration by the presence of hematite, limonite and chlorite and by the absence of plagioclase. Alkali feldspars from this part of the core are turbid, have a low 2 V of about 10°, are highly enriched in K, have low Na and Rb concentrations, lack cathode luminescence, and form a straight line on a Rb-Sr isochron diagram yielding a date of 599±69 Ma. Core samples from below 6.4 m appear relatively fresh and unaltered. Alkali feldspar from this portion of the core is orthoclase, shows uniform blue luminescence and gives a Rb-Sr date of 1,162±11 Ma. These results indicate that feldspars in the lowest part of the core are primary minerals that crystallized during the Grenville Orogeny, whereas the K-feldspar in the top of the core is of low-temperature secondary origin. The formation of this feldspar is explained as a consequence of chemical weathering of primary feldspar during late Precambrian time to clay minerals that were later reconstituted under low-temperature hydrothermal conditions as K-feldspar (adularia) by reactions with brines derived from the overlying Mt. Simon Formation of Cambrian age.Laboratory for Isotope Geology and Geochemistry (Isotopia), Contribution No. 68 相似文献