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In the tropical rain forests of the Congo during the dry season, from June to September 1987, carboxylic acid partial pressures (P gas) in the air above the canopy, at ground level, and at the boundary layer, were estimated from water samples such as fog and rainwater. The concentrations of these acids were also measured in the sap of tree leaves. Tree leaves act as a sink or as a source if the acid P gas is greater of lower than the acid concentrations in molecular form in sap. For each of these soluble gases, there is a value of P gas where the exchange is nul. This is called the compensation point. Values of the compensation point for some tree leaves were evaluated according to Henry's law. Henry's law coefficients at ppm levels were redetermined for formic (HCOOH), acetic (CH3COOH), propionic (CH3CH2COOH), and isobutyric (CH3CH(CH3)COOH) acids.By comparison of P gas and compensation points, it is concluded that the forest was a potential source for these acids. The soil-or the litter-acts as a significant source of a carboxylic acid of C3 or C4 atoms in the aliphatic chain. This carboxylic acid, not yet fully characterized, could play an important role in the rain acidity in forested zones of the equatorial areas.The direct emission of these carboxylic acids by vegetation was the main source in the boundary layer above the forest. The average emissions were 3.1×109, 7.8×109, and 8.4×109 molecules cm-2 s-1 for HCOOH, CH3COOH, and CH3CH2COOH, respectively. The savanna is an exogenous source of HCOOH and CH3CH2COOH during moderately rainy days for 30% of the time. The ozonolysis of isoprene seems to be a small source of HCOOH.  相似文献   
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We report partial pressure of CO2 (pCO2) and ancillary data in three rivers (Bia, Tanoé, and Comoé) and five lagoons (Tendo, Aby, Ebrié, Potou, and Grand-Lahou) in Ivory Coast (West Africa), during four cruises covering the main climatic seasons. The three rivers were oversaturated in CO2 with respect to atmospheric equilibrium, and the seasonal variability of pCO2 was due to dilution during the flooding period. Surface waters of the Potou, Ebrié, and Grand-Lahou lagoons were oversaturated in CO2 during all seasons. These lagoons behaved similarly to the oligohaline regions of macrotidal estuaries that are CO2 sources to the atmosphere due to net ecosystem heterotrophy and inputs of riverine CO2 rich waters. The Aby and Tendo lagoons were undersaturated in CO2 with respect to the atmosphere because of their permanent haline stratification (unlike the other lagoons) that seemed to lead to higher phytoplankton production and export of organic carbon below the pycnocline.  相似文献   
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This study analyzes projected changes in seasonal extreme precipitation intensity and dry spell length in the investigation area (Côte d’Ivoire) under RCP4.5 and RCP8.5 forcing scenarios. To this end, a multi-model ensemble of fourteen CORDEX-Africa regional climate model simulations is used during the three stages of the West African Monsoon (WAM) season (April–June (AMJ), July–September (JAS), and October–December (OND)). The results indicate that Côte d’Ivoire is subject to a robust increase of cumulative intensity of precipitation associated with an amplification of extreme precipitation events during the WAM. In particular during JAS, a substantial increase in extreme precipitation reaching up to 50–60% compared to the reference mean value prevails in the western and coastal areas in the far future and under the RCP8.5 scenario. In addition, AMJ season is dominated by an increase in dry spell length of about 12% and 17% in the near future and 20% and 30% in the far future in the entire country under RCP4.5 and RCP8.5 scenarios, respectively, albeit considerable uncertainties. OND considered as the post-monsoon season is mostly characterized by a robust decrease in dry spell length more marked in the southwest in the RCP8.5 scenario during the far future. These results suggest that agricultural production and particularly cocoa plantations in the southwestern regions could be at the risk of flooding events and that water stress remains a threat for cocoa, coffee, and other cash crop plantations in the eastern regions.  相似文献   
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The distribution of arsenic (As(III), As(V)) and iron (Fe(II), Fe(III)) species was monitored during 1 year in a borehole drilled in the Carnoulès tailings impoundment which contains As-rich pyrite. The concentrations of total As and Fe in subsurface waters exhibited strong variations over one year, which were controlled by dissolved oxygen concentrations. At high oxygen levels, extremely high As (up to 162 mM) and Fe (up to 364 mM) concentrations were reached in the borehole, with the oxidised species predominant. As and Fe concentrations decreased 10-fold under oxygen-deficient conditions, as a result of pH increase and subsequent precipitation of As(V) and Fe(III). From drill core sections, it appeared that at low dissolved oxygen levels, As(III) was primarily released into water by the oxidation of As-rich pyrite in the unsaturated zone. Subsequent As and Fe precipitation was promoted during transport to the saturated zone; this reaction resulted in As enrichments in the sediment below the water table compared to the original content in pyrite, together with the formation of As-rich (up to 35 wt% As) ferruginous material in the unsaturated zone. High amounts of As(V) were released from these secondary phases during leaching experiments with oxygenated acid sulfate-rich waters; this process is believed to contribute to As(V) enrichment in the subsurface waters of the Carnoulès tailings during periods of high dissolved oxygen level.  相似文献   
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Recent climatic trends in the tropical Atlantic   总被引：1，自引：1，他引：0  
A homogeneous monthly data set of sea surface temperature (SST) and pseudo wind stress based on in situ observations is used to investigate the climatic trends over the tropical Atlantic during the last five decades (1964–2012). After a decrease of SST by about 1 °C during 1964–1975, most apparent in the northern tropical region, the entire tropical basin warmed up. That warming was the most substantial (>1 °C) in the eastern tropical ocean and in the longitudinal band of the intertropical convergence zone. Surprisingly, the trade wind system also strengthened over the peirod 1964–2012. Complementary information extracted from other observational data sources confirms the simultaneity of SST warming and the strengthening of the surface winds. Examining data sets of surface heat flux during the last few decades for the same region, we find that the SST warming was not a consequence of atmospheric heat flux forcing. Conversely, we suggest that long-term SST warming drives changes in atmosphere parameters at the sea surface, most notably an increase in latent heat flux, and that an acceleration of the hydrological cycle induces a strengthening of the trade winds and an acceleration of the Hadley circulation. These trends are also accompanied by rising sea levels and upper ocean heat content over similar multi-decadal time scales in the tropical Atlantic. Though more work is needed to fully understand these long term trends, especially what happens from the mid-1970’s, it is likely that changes in ocean circulation involving some combination of the Atlantic meridional overtuning circulation and the subtropical cells are required to explain the observations.  相似文献   
7.
The Vea catchment, mainly underlain by crystalline basement rocks, is located in Northern Ghana. Hydrogeochemical studies were carried out in this area with the objective of identifying the geochemical processes influencing water quality and suitability of surface and groundwater for agricultural and domestic uses. Sixty-one groundwater and four surface water samples were collected from boreholes, dams and rivers and analysed for Ca2+, Mg2+, Na+, K+, HCO3 ?, Cl?, and SO4 2?, Fetot, PO4 3?, Mntot, NH4 +, NO3 ?, NO2 ?. In addition, pH, total dissolved solids, electrical conductivity, total hardness, turbidity, colour, salinity and dissolved oxygen were analysed. Chloro-alkaline indices 1 and 2, and characterization of weathering processes suggest that the chemistry of groundwater is dominated by the interaction between water and rocks. Cation exchange and silicate weathering are the dominant processes controlling the chemical composition of the groundwater in the area studied. Mineral saturation indices indicate the presence of at least three groups of groundwater in the Vea catchment with respect to residence time. The meteoric genesis index suggests that 86% of the water samples belong to the shallow meteoric water percolation type. The findings further suggest that the groundwater and surface water in the basin studied are mainly Ca–Mg–HCO3 water type, regardless of the geology. Compared to the water quality guidelines of WHO, the study results on sodium absorption ratio, sodium percentage, magnesium hazard, permeability index and residual sodium carbonate indicate that groundwater and surface water in the Vea catchment are generally suitable for drinking and irrigation purposes.  相似文献   
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