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1.
Multiple sulfur isotope system is a powerful new tracer for atmospheric, volcanic, and biological influences on sulfur cycles in the anoxic early Earth. Here, we report high-precision quadruple sulfur isotope analyses (32S/33S/34S/36S) of barite, pyrite in barite, and sulfides in related hydrothermal and igneous rocks occurring in the ca. 3.5 Ga Dresser Formation, Western Australia. Our results indicate that observed isotopic variations are mainly controlled by mixing of mass-dependently (MD) and non-mass-dependently fractionated (non-MD) sulfur reservoirs. Based on the quadruple sulfur isotope systematics (δ34S-Δ33S-Δ36S) for these minerals, four end-member sulfur reservoirs have been recognized: (1) non-MD sulfate (δ34S = −5 ± 2‰; Δ33S = −3 ± 1‰); (2) MD sulfate (δ34S = +10 ± 3‰); (3) non-MD sulfur (δ34S > +6‰; Δ33S > +4‰); and (4) igneous MD sulfur (δ34S = Δ33S = 0‰). The first and third components show a clear non-MD signatures, thus probably represent sulfate and sulfur aerosol inputs. The MD sulfate component (2) is enriched in 34S (+10 ± 3‰) and may have originated from microbial and/or abiotic disproportionation of volcanic S or SO2. Our results reconfirm that the Dresser barites contain small amounts of pyrite depleted in 34S by 15-22‰ relative to the host barite. These barite-pyrite pairs exhibit a mass-dependent relationship of δ33S/δ34S with slope less than 0.512, which is consistent with that expected for microbial sulfate reduction and is significantly different from that of equilibrium fractionation (0.515). The barite-pyrite pairs also show up to 1‰ difference in Δ36S values and steep Δ36S/Δ33S slopes, which deviate from the main Archean array (Δ36S/Δ33S = −0.9) and are comparable to isotope effects exhibited by sulfate reducing microbes (Δ36S/Δ33S = −5 to −11). These new lines of evidence support the existence of sulfate reducers at ca. 3.5 Ga, whereas microbial sulfur disproportionation may have been more limited than recently suggested. 相似文献
2.
State Estimation of the North Pacific Ocean by a Four-Dimensional Variational Data Assimilation Experiment 总被引:1,自引:0,他引:1
Toshiyuki Awaji Shuhei Masuda Yoichi Ishikawa Nozomi Sugiura Takahiro Toyoda Tomohiro Nakamura 《Journal of Oceanography》2003,59(6):931-943
A four-dimensional variational data assimilation system has been applied to an experiment to describe the dynamic state of
the North Pacific Ocean. A synthesis of available observational records and a sophisticated ocean general circulation model
produces a dynamically consistent dataset, which, in contrast to the nudging approach, provides realistic features of the
seasonally-varying ocean circulation with no artificial sources/sinks for temperature and salinity fields. This new dataset
enables us to estimate heat and water mass transports in addition to the qualification of water mass formation and movement
processes. A sensitivity experiment on our assimilation system reveals that the origin of the North Pacific Intermediate Water
can be traced back to the Sea of Okhotsk and the Bering Sea in the subarctic region and to the subtropical Kuroshio region
further south. These results demonstrate that our data assimilation system is a very powerful tool for the identification
and characterization of ocean variabilities and for our understanding of the dynamic state of ocean circulation.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
3.
Sulfur isotope studies of post-Archean terrestrial materials have focused on the ratio 34S/32S because additional isotopes, 33S and 36S, were thought to carry little information beyond the well-known mass-dependent relationship among multiple-isotope ratios. We report high-precision analyses of Δ33S and Δ36S values, defined as deviations of 33S and 36S from ideal mass-dependent relationships, for international reference materials and sedimentary sulfides of Phanerozoic age by using a fluorination technique with a dual-inlet isotope ratio mass spectrometer. Measured variations in Δ33S and Δ36S are explained as resulting from processes involve branching reactions (two or more reservoirs formed) or mixing. Irreversible processes in closed systems (Rayleigh distillation) amplify the isotope effect. We outline how this new isotope proxy can be used to gain new insights into fundamental aspects of the sulfur biogeochemical cycle, including additional constraints on seawater sulfate budget and processes in sedimentary sulfide formation. The isotope systematics discussed here cannot explain the much larger variation of Δ33S and Δ36S observed in Archean rock records. Furthermore, Phanerozoic samples we have studied show a characteristic Δ33S and Δ36S relationship that differs from those measured in Archean rocks and laboratory photolysis experiments. Thus, high precision analysis of Δ33S and Δ36S can be used to distinguish small non-zero Δ33S and Δ36S produced by mass-dependent processes from those produced by mass-independent processes in Archean rocks and extraterrestrial materials. 相似文献
4.
Yukio Isozaki Shinji Yamamoto Shuhei Sakata Hideyuki Obayashi Takafumi Hirata Ken-ichi Obori Toshinori Maebayashi Satoshi Takeshima Toshikazu Ebisuzaki Shigenori Maruyama 《地学前缘(英文版)》2018,9(4):1073-1083
Despite the recent development in radiometric dating of numerous zircons by LA-ICPMS, mineral separation still remains a major obstacle, particularly in the search for the oldest material on Earth. To improve the efficiency in zircon separation by an order of magnitude, we have designed/developed a new machine-an automatic zircon separator(AZS). This is designed particularly for automatic pick-up of100 μm-sized zircon grains out of a heavy mineral fraction after conventional separation procedures. The AZS operates in three modes:(1) image processing to choose targeted individual zircon grains out of all heavy minerals spread on a tray,(2) automatic capturing of the individual zircon grains with microtweezers, and(3) placing them one-by-one in a coordinated alignment on a receiving tray. The automatic capturing was designed/created for continuous mineral selecting without human presence for many hours. This software also enables the registration of each separated zircon grain for dating, by recording digital photo-image, optical(color) indices, and coordinates on a receiving tray. We developed two new approaches for the dating; i.e.(1) direct dating of zircons selected by LA-ICPMS without conventional resin-mounting/polishing,(2) high speed U-Pb dating, combined with conventional sample preparation procedures using the new equipment with multiple-ion counting detectors(LA-MIC-ICPMS).With the first approach, Pb-Pb ages obtained from the surface of a mineral were crosschecked with the interior of the same grain after resin-mounting/polishing. With the second approach, the amount of time required for dating one zircon grain is ca. 20 s, and a sample throughput of 150 grains per hour can be achieved with sufficient precision(ca. 0.5%).We tested the practical efficiency of the AZS, by analyzing an Archean Jack Hills conglomerate in Western Australia with the known oldest(4.3 Ga) zircon on Earth. Preliminary results are positive; we were able to obtain more than 194 zircons that are over 4.0 Ga out of ca. 3800 checked grains, and 9 grains were over 4300 Ma with the oldest at 4371 ± 7 Ma. This separation system by AZS, combined with the new approaches, guarantees much higher yield in the hunt for old zircons. 相似文献
5.
Reciprocity theorem to compute the static deformation due to a point dislocation buried in a spherically symmetric earth 总被引:4,自引:0,他引:4
Shuhei Okubo 《Geophysical Journal International》1993,115(3):921-928
Intriguing reciprocity relations exist between the static deformation excited by a point dislocation in a SNREI earth and those generated by external forces, such as tidal force, surface loading and surface shear forces. Coseismic deformations can be rewritten as follows: (1) potential change in terms of the tide deformation field, (2) radial displacement in terms of the load and tidal deformation fields, and (3) tangential displacement in terms of shear and torsional deformation fields. The relations greatly reduce the effort to compute the coseismic crustal deformation in a spherically symmetric earth. 相似文献
6.
7.
Scott A. Reinemann David F. Porinchu Mae Sexauer Gustin Bryan G. Mark 《Journal of Paleolimnology》2014,52(4):405-418
The geochemistry of lake sediments was used to identify anthropogenic factors influencing aquatic ecosystems of sub-alpine lakes in the western United States during the past century. Sediment cores were recovered from six high-elevation lakes in the central Great Basin of the United States. The proxies utilized to examine the degree of recent anthropogenic environmental change include spheroidal carbonaceous particle (SCP), mercury (Hg), and sediment organic content estimated using loss-on-ignition. Chronologies for the sediment cores, developed using 210Pb, indicate the cores span the twentieth century. Mercury flux varied between lakes but all exhibited increasing fluxes during the mid-twentieth century. The mean ratio of modern (post-A.D. 1985) to preindustrial (pre-A.D. 1880) Hg flux was 5.2, which is comparable to the results from previous studies conducted in western North America. Peak SCP flux for all lakes occurred between approximately A.D. 1940 and A.D. 1970, after which time the SCP flux was greatly reduced. The reduction in SCP input is likely due to better controls on combustion sources. Measured Hg concentrations and calculated sedimentation rates suggest atmospheric Hg flux increased in the early 1900s, from A.D. 1920 to A.D. 1990, and at present. Atmospheric deposition is the primary source of the anthropogenic inputs of Hg and SCPs to these high elevation lakes. The input of SCPs, which is largely driven by regional sources, has declined with the implementation of national pollution control regulations. Mercury deposition in the Great Basin has most likely been influenced more by regional inputs. 相似文献
8.
This paper treats the static spheroidal deformation of degree 1 in detail. We give a physical interpretation of the consistency relation imposed on it. the relation serves as a guiding principle to find out all of its members. Following Okubo & Saito, we derive the partial derivatives of the degree 1 Love numbers with respect to density, bulk modulus and rigidity. 相似文献
9.
Amit K. Pradhananga Mae A. Davenport David C. Fulton Geoffrey M. Maruyama Dean Current 《社会与自然资源》2017,30(2):212-227
This study applies an integrated moral obligation model to examine the role of environmental and cultural values, and beliefs in the activation of landowner conservation norms. Data for this study were collected through a self-administered survey of riparian landowners in two Minnesota watersheds: Sand Creek and Vermillion River watersheds. Study findings suggest that collectivistic and biospheric–altruistic values form the bases for the activation of personal norms. Further, beliefs about local responsibility and ability to act influence personal norms to protect water resources. Findings suggest that landowners’ personal norms of water conservation are more likely to be activated by conservation strategies that appeal to biospheric–altruistic and collectivistic values, emphasize adverse consequences of water pollution, highlight water resource protection as a local responsibility, and provide the resources needed to protect water resources. 相似文献
10.
Teresa Mae Lassak Allen K. McNamara Edward J. Garnero Shijie Zhong 《Earth and Planetary Science Letters》2010,289(1-2):232-241
The origin of large low shear-wave velocity provinces (LLSVPs) in the lowermost mantle beneath the central Pacific and Africa is not well constrained. We explore numerical convection calculations for two proposed hypotheses for these anomalies, namely, thermal upwellings (e.g., plume clusters) and large intrinsically dense piles of mantle material (e.g., thermochemical piles), each of which uniquely affects the topography on Earth's core–mantle boundary (CMB). The thermochemical pile models predict a relatively flat but elevated CMB beneath piles (presumed LLSVPs), with strong upwarping along LLSVP margins. The plume cluster models predict CMB upwarping beneath upwellings that are less geographically organized. Both models display CMB depressions beneath subduction related downwelling. While each of the two models produces a unique, characteristic style of CMB topography, we find that seismic models will require shorter length scales than are currently being employed in order to distinguish between the end-member dynamic models presented here. 相似文献