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Molybdenum disulfide (MoS2), a layered transition-metal dichalcogenide, has been of special importance to the research community of geochemistry, materials
and environmental chemistry, and geotechnical engineering. Understanding the oxidation behavior and charge-transfer mechanisms
in MoS2 is important to gain better insight into the degradation of this mineral in the environment. In addition, understanding the
insertion of metals into molybdenite and evaluation of charge-transfer mechanism and dynamics is important to utilize these
minerals in technological applications. Furthermore, a detailed investigation of thermal oxidation behavior and metal-insertion
will provide a basis to further explore and model the mechanism of adsorption of metal ions onto geomedia. 相似文献
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BO Husφy 《极地研究(英文版)》2002,13(1)
1 ＩｎｔｒｏｄｕｃｔｉｏｎＡｔｌａｔｉｔｕｄｅｓａｒｏｕｎｄ 80°Ｎａｎｄｉｎｔｈｅｍｅｓｏｓｐｈｅｒｅ /ｌｏｗｅｒｔｈｅｒｍｏｓｐｈｅｒｅ (ＭＬＴ) ,ｔｈｅｒｅｈａｖｅｂｅｅｎｆｅｗｍｅａｓｕｒｅｍｅｎｔｓｏｆｎｅｕｔｒａｌｄｙｎａｍｉｃｓ.ＡｒｅｑｕｉｒｅｍｅｎｔｗａｓｓｅｅｎｆｏｒｌｏｎｇｔｅｒｍｃｏｎｔｉｎｕａｌｍｏｎｉｔｏｒｉｎｇａｎｄａＶＨＦｍｅｔｅｏｒｒａｄａｒｗａｓｉｄｅｎｔｉｆｉｅｄａｓｂｅｉｎｇａｍｏｓｔｓｕｉｔａｂｌｅｉｎｓｔｒｕｍｅｎｔ.ＲａｄａｒｓｌｉｋｅｔｈｅＥＩＳＣＡ… 相似文献
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Two sedimentary cores with pollen, charcoal and radiocarbon data are presented. These records document the Late‐glacial and Holocene dry forest vegetation, fire and environmental history of the southern Cauca Valley in Colombia (1020 m). Core Quilichao‐1 (640 cm; 3° 6′N, 76° 31′W) represents the periods of 13 150–7720 14C yr BP and, following a hiatus, from 2880 14C yr BP to modern. Core La Teta‐2 (250 cm; 3° 5′N, 76° 32′W) provides a continuous record from 8700 14C yr BP to modern. Around 13 150 14C yr BP core Quilichao‐1 shows an active Late‐glacial drainage system and presence of dry forest. From 11 465 to 10 520 14C yr BP dry forest consists mainly of Crotalaria, Moraceae/Urticaceae, Melastomataceae/Combretaceae, Piper and low stature trees, such as Acalypha, Alchornea, Cecropia and Celtis. At higher elevation Andean forest comprising Alnus, Hedyosmum, Quercus and Myrica was common. After 10 520 14C yr BP the floral composition of dry forest changed, with extensive open grass vegetation indicative of dry climatic conditions. This event may coincide with the change to cool and dry conditions in the second part of the El Abra stadial, an equivalent to the Younger Dryas. From 8850 14C yr BP the record from La Teta indicates dry climatic conditions relative to the present, these prevailing up to 2880 14C yr BP at Quilichao and to 2720 14C yr BP at La Teta. Severe dryness reached maxima at 7500 14C yr BP and 4300 14C yr BP, when dry forest reached maximum expansion. Dry forest was gradually replaced by grassy vegetation, reaching maximum expansion around 2300 14C yr BP. After 2300 14C yr BP grassy vegetation remains abundant. Presence of crop taxa (a.o. Zea mays), disturbance indicators (Cecropia) and an increase in charcoal point to the presence of pre‐Columbian people since 2300 14C yr BP. After 950 14C yr BP, expansion of secondary forest taxa may indicate depopulation and abandonment of previously cultivated land. After 400 14C yr BP, possibly related to the Spanish conquest, secondary forest expanded and charcoal concentrations increased, possibly indicating further reduction of cultivated land. During the past century, Heliotropium and Didymopanax became abundant in an increasingly degraded landscape. Copyright © 2002 John Wiley & Sons, Ltd. 相似文献
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I. Bejarano-Ramirez Jose M. Jurado R. Muñiz-Valencia Á. Alcázar Silvia G. Ceballos-Magaña A. Olivos-Ortiz O. Rangel 《International Journal of Environmental Science and Technology》2017,14(6):1333-1342
The contents of As, Cd, Cu, Cr, Mg, Mn, Ni, Pb and Zn have been determined in sediment and water samples from Valle de las Garzas estuary and Port Manzanillo (Colima, Mexico) using ICP-AES. The concentrations of these elements were used for a comparative study to determine the distribution of heavy metals and to evaluate which elements reflect natural or anthropogenic backgrounds. For this purpose, seven sampling points were selected: Four of them correspond to the lagoon, and three were situated in the port. Statistical analysis of the mineral content was assessed. Initially, data comparison was assessed by statistical tests for each variable. Principal component analysis was then applied considering the influence of all variables at the same time by obtaining the distribution of samples according to their scores in the principal component space. In this way, four studies were carried out: (1) study of sediments collected during the dry season; (2) study of sediments collected during the rainy season; (3) comparative study between sediments from rainy and dry season; and (4) study of water composition collected during rainy season. From the results of the performed analyses, it can be concluded that metals distribution pattern reflected natural and anthropogenic backgrounds (e.g., sediments from the lagoon, situated at the beginning of the rain channel, presented high contents of Zn and Cu, perhaps related to anthropogenic activities or the influence of igneous sediments). 相似文献
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Caio Vinícius Gabrig Turbay Rangel Marcos Tadeu D’Azeredo Orlando Cláudio De Morisson Valeriano Alexandre de Oliveira Chaves 《International Geology Review》2017,59(15):1966-1973
The Varre-Sai meteorite fell along the border of the states of Espirito Santo and Rio de Janeiro, Brazil; on 19 June 2010 at 5:40 pm. Petrography and X-ray powder diffraction (XRD) indicate that the rock is an L5 S4 chondrite, with blastoporphyritic texture that has not been previously described. Geochemical data based on major and rare-earth elements (REEs) show that Varre-Sai is highly similar to the other L chondrites. In Harker diagrams, Varre-Sai, L, and LL chondrites form a single group, suggesting no significant chemical differences between them and contributing to the long-standing debate of whether LL chondrites form a distinct group or whether they are a subset of the L group. Harker diagrams also define a trend from E to H and L/LL chondrites, similar to the cosmochemical trends suggested by other authors. The behaviour of Fe2O3t and NiO indicates a relationship with Fe-Ni alloys, and their trend in the diagram suggests some chemical differentiation in the ordinary chondrite parental bodies. The REE content in Varre-Sai, normalized to C chondrites, falls in the field of L chondrites and others, but with slight REE enrichment. The chemical differences in chondrites, mainly in REEs, Fe2O3t and NiO could be alternatively interpreted as variations in the inherited agglutinated materials as chondrules, Ca–Al-rich inclusions and Fe–Ni nodules. 相似文献
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In this work, we report diffusion-limited aggregation (DLA)-type Montecarlo computations of a stochastic model of displacement
of a viscous fluid by another that preferentially wets a porous medium, for the case when both fluids are immiscible in the
absence of buoyancy forces. The model has the aim to simulate cooperative invasion processes found in experiments of immiscible
wetting displacement. The model considers the nonlocal effects of the Laplacian pressure field and the capillary forces via hydrodynamic equations in the Darcy regime with a boundary
condition for the pressure at the interface. The boundary condition contains two different types of disorder: the capillary
term, which constitutes an additive random disorder, and a term containing an effective random surface tension, which couples
to a curvature (it constitutes a multiplicative random term that carries nonlocal information of the whole pressure). We generate
different displacement patterns for different setting of the parameters of the model. We analyze these patterns by studying
the scaling properties of the interface that separate the two fluids and calculating the fractal dimension of the interface.
The results show the existence of three distinct regimes of scaling. One regime at the smallest-length scales is due to the
multiplicative random disorder together with the nonlocal coupling; it reveals itself in a roughness exponent α ≈ 0.80. Additionally, we find a DLA-type scaling regime with a roughness exponent α ≈ 0.60 at the largest scales and intermediate scaling regime with α ≈ 0.70 corresponding to invasion percolation with trapping. Each regime has definite scaling ranges that depend on the capillary
number and the relative wetting tendency of the fluids. The behavior of the fractal dimensions of the interfaces of the aggregates
constitutes a further confirmation of the existence of three scaling regimes and the multi-self-affinity of the perimeter
of the interface boundaries. 相似文献
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白云鄂博碳酸岩的方解石-白云石地质温度计 总被引：6，自引：2，他引：4
利用方解石-白云石地质温度计对白云鄂博地区碳酸岩的平衡温度进行了测定。出露于东矿下盘的白云岩质火山岩和出露于尖山的方解石-白云石型火山岩获得了较高的温度,分别为681℃和648℃。这些样品中的方解石呈二十微米左右晶形较完整的小片,被稍大粒度的白云石颗粒包裹,未受交代作用影响,推测这种碳酸岩在快速冷却的情况下保存下了其岩浆侵位时的成分特点,从而指示出接近碳酸岩浆侵位时的温度。但本区多数碳酸岩的平衡温度在400～500℃之间,有下列三种情况:(1)具有自形-半自形中粗粒粒状变晶结构的碳酸岩最后的平衡温度为415～496℃;(2)产自东矿的其余样品(火山岩),所测最后平衡温度为431～485℃,在测温的微区范围内可见极细粒白云石方解石与稀土等矿物共生的现象;(3)为交代重结晶结构的碳酸岩明显受到后期热液流体的交代,在流体的作用下共生方解石和白云石在成分上达到新的平衡,平衡温度为432～507℃。本文所分析的样品多数结果(371～507℃)与用白云石(方解石)和磁铁矿氧同位素温度计对白云鄂博碳酸岩的计算结果(360～546℃)十分一致。虽然有研究者对方解石-白云石温度计用于火成碳酸岩表示过质疑,但本文资料表明火成碳酸岩最后的平衡温度是可以运用方解石-白云石温度计法来计算的。 相似文献
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安徽巢湖凤凰山剖面石炭系微相和层序地层特征 总被引：9，自引：1，他引：9
应用露头层序地层学基本原理和方法 ,对巢湖凤凰山石炭系剖面进行重新研究。巢湖凤凰山石炭系总厚度为79.0 2 m ,在这个剖面中可以识别出 6种主要岩相、18种微相和 11个三级沉积层序 ,其中六个三级沉积层序属于 I型沉积层序 ,三个属于 II型沉积层序 ,缺失第 9和第 10沉积层序。三级沉积层序在不同的古地理单元和不同的沉积环境中可以进行对比。根据各微相特征和成因 ,揭示了沉积间断面上存在的多期古岩溶现象。阐述了三级层序及其对应的三级海平面升降旋回的特征 相似文献