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Carsten Blindauer Vladimir Rozanov John Philip Burrows 《Journal of Atmospheric Chemistry》1996,24(1):1-21
The accurate radiative transfer model GOMETRAN, initially designed to yield radiances at TOA in the wavelength range 240–790 nm, has been extended to allow for the computation of actinic fluxes down to 175 nm and for the calculation of photolysis frequencies in the atmosphere. The capability of the extended model PHOTOGT (PHOTOGOMETRAN) is demonstrated in a number of successful comparison studies both with recent experiments (ground-based, balloonborne, airborne) and model calculations of radiances, actinic fluxes and photolysis frequencies in the stratosphere and troposphere. In an atmospheric case study, the impact of new quantum yield data for the O3 » O2+O(1
d) photodissociation channel on the photolytic production of O(1
d) atoms in the lower atmosphere has been quantified. 相似文献
4.
M. Krämer Ri. Müller H. Bovensmann J. Burrows J. Brinkmann E. P. Röth J.-U. Grooß Ro. Müller Th. Woyke R. Ruhnke G. Günther J. Hendricks E. Lippert K. S. Carslaw Th. Peter A. Zieger Ch. Brühl B. Steil R. Lehmann D. S. McKenna 《Journal of Atmospheric Chemistry》2003,45(1):51-77
Several stratospheric chemistry modules from box, 2-D or 3-D models, have been intercompared. The intercomparison was focused on the ozone loss and associated reactive species under the conditions found in the cold, wintertime Arctic and Antarctic vortices. Comparisons of both gas phase and heterogeneous chemistry modules show excellent agreement between the models under constrained conditions for photolysis and the microphysics of polar stratospheric clouds. While the mean integral ozone loss ranges from 4–80% for different 30–50 days long air parcel trajectories, the mean scatter of model results around these values is only about ±1.5%. In a case study, where the models employed their standard photolysis and microphysical schemes, the variation around the mean percentage ozone loss increases to about ±7%. This increased scatter of model results is mainly due to the different treatment of the PSC microphysics and heterogeneous chemistry in the models, whereby the most unrealistic assumptions about PSC processes consequently lead to the least representative ozone chemistry. Furthermore, for this case study the model results for the ozone mixing ratios at different altitudes were compared with a measured ozone profile to investigate the extent to which models reproduce the stratospheric ozone losses. It was found that mainly in the height range of strong ozone depletion all models underestimate the ozone loss by about a factor of two. This finding corroborates earlier studies and implies a general deficiency in our understanding of the stratospheric ozone loss chemistry rather than a specific problem related to a particular model simulation. 相似文献
5.
Erodibility of low‐compaction steep‐sloped reclaimed surface mine lands in the southern Appalachian region,USA 下载免费PDF全文
The use of loose spoils on steep slopes for surface coal mining reclamation sites has been promoted by the US Department of Interior, Office of Surface Mining for the establishment of native forest, as prescribed by the Forest Reclamation Approach (FRA). Although low‐compaction spoils improve tree survival and growth, erodibility on steep slopes was suspected to increase. This study quantified a combined KC factor (combining the effects of the soil erodibility K factor and cover management C) for low compaction, steep‐sloped (>20°) reclaimed mine lands in the Appalachian region, USA. The combined KC factor was used because standard Unit Plot conditions required to separate these factors, per Revised Universal Soil Loss Equation (RUSLE) experimental protocols, were not followed explicitly. Three active coal mining sites in the Appalachian region of East Tennessee, each containing four replicate field plots, were monitored for rainfall and sediment yields during a 14‐month period beginning June 2009. Average cumulative erosivity for the study sites during the monitoring period was measured as 5248.9 MJ·mm·ha?1·h?1. The KC ranged between 0.001 and 0.05 t·ha·h·ha?1·MJ?1·mm?1, with the highest values occurring immediately following reclamation site construction as rills developed (June – August 2009). The KC for two study sites with about an 18–20 mm spoil D84 were above 0.01 t·ha·h·ha?1·MJ?1·mm?1 during rill development, and below 0.003 t·ha·h·ha?1·MJ?1·mm?1 after August 2009 for the post‐rill development period. The KC values for one site with a 40 mm spoil D84 were never above 0.008 t·ha·h·ha?1·MJ?1·mm?1 and also on average were lower, being more similar to the other two sites after the rill development period. Based on an initial KC factor (Ke) measured during the first few storm events, the average C factor (Ce) was estimated as 0.58 for the rill development period and 0.13 for the post‐rill development period. It appears that larger size fractions of spoils influence KC and Ce factors on low‐compaction steep slopes reclamation sites. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献
6.
A hand-operated, tubular-coring device developed for use in biogeochemical sampling of succulent and pulpy plants is described. The sampler weighs about 500 g (1.1 lb); and if 25 × 175 mm (1 × 7 in) screw-top test tubes are used as sample containers, the complete sampling equipment kit is easily portable, having both moderate bulk and weight. 相似文献
7.
Burrows A Guillot T Hubbard WB Marley MS Saumon D Lunine JI Sudarsky D 《The Astrophysical journal》2000,534(1):L97-L100
The recent discovery that the close-in extrasolar giant planet HD 209458b transits its star has provided a first-of-its-kind measurement of the planet's radius and mass. In addition, there is a provocative detection of the light reflected off of the giant planet tau Bootis b. Including the effects of stellar irradiation, we estimate the general behavior of radius/age trajectories for such planets and interpret the large measured radii of HD 209458b and tau Boo b in that context. We find that HD 209458b must be a hydrogen-rich gas giant. Furthermore, the large radius of a close-in gas giant is not due to the thermal expansion of its atmosphere but to the high residual entropy that remains throughout its bulk by dint of its early proximity to a luminous primary. The large stellar flux does not inflate the planet but retards its otherwise inexorable contraction from a more extended configuration at birth. This implies either that such a planet was formed near its current orbital distance or that it migrated in from larger distances (>/=0.5 AU), no later than a few times 107 yr of birth. 相似文献
8.
We present results from the first light observations of the Cassiopeia A supernova remnant (SNR) by the Chandra X-Ray Observatory. Based on representative spectra from four selected regions, we investigate the processes of nucleosynthesis and mixing in Cas A. We make the first unequivocal identification of iron-rich ejecta produced by explosive silicon burning in a young Galactic SNR. Elsewhere in the remnant, we see silicon-rich ejecta from explosive oxygen burning. The Fe-rich ejecta lie outside the Si-rich material, indicating that bulk motions were extensive and energetic enough in Cas A to cause a spatial inversion of a significant portion of the supernova core. It is likely that this inversion was caused by "Fe"-rich ejecta emerging in plumes from the rising bubbles in the neutrino-driven convection layer during the supernova explosion. In addition, the radioactive decay energy from 56Ni may have contributed to the subsequent evolution of the material. We have also discovered faint, well-defined filaments with featureless X-ray spectra that are possibly sites of cosmic-ray acceleration in Cas A. 相似文献
9.
The Global Ozone Monitoring Experiment (GOME) is the first of a series of European satellite instruments monitoring global ozone and other relevant trace constituents in the UV/visible spectral range. On 20 April 1995, the European Space Agency (ESA) launched the GOME from Kourou, French Guyana, aboard the second European Remote Sensing satellite (ERS-2). In order to obtain the geometric albedo from the backscattered terrestrial radiance measurements, a solar irradiance measurement sequence in the spectral range between 240 nm and 790 nm is carried out once every day. The GOME solar irradiance is recorded at a moderate spectral resolution (0.2–0.4 nm), thus providing an excellent opportunity to contribute to the long-term investigation of solar flux variation associated with the 11-year solar activity cycle from space, which started in 1978 with SBUV (Solar Backscatter UV Experiment) observations on Nimbus-7 and covers solar cycles 21 and 22. This paper briefly describes the GOME spectrometer and measurement mode which are relevant to the solar viewing. Preliminary results from the solar irradiance measurements between 1995 and 1997 and comparisons to SSBUV-8 (Shuttle SBUV) in January 1996 are presented. Solar activity indices used as proxies for solar flux variation are often used to find a correlation with observed variation in atmospheric quantities, for instance, total ozone. Initial results from the GOME Mgii (280 nm) and Caii K (393 nm) solar activity index calculation are presented and discussed. The coupling of solar irradiance variability to global change is a current source of scientific and public concern. This study shows that GOME/ERS-2 (1995–2001) and the next generation of European remote sensing instruments, SCIAMACHY and GOME/METOP, have the potential to provide continuity in the measurements of solar irradiance from space well into the next century. 相似文献
10.
R. Müller J.-U. Grooß D. S. McKenna P. J. Crutzen C. Brühl J. M. Russell III L. L. Gordley J. P. Burrows A. F. Tuck 《Annales Geophysicae》1998,17(1):101-114
Severe chemical ozone loss has been detected in the Arctic in the winter and spring of 1995–96 by a variety of methods. Extreme reductions in column ozone due to halogen catalysed chemistry were derived from measurements of the Halogen Occultation Experiment (HALOE) on board the Upper Atmosphere Research Satellite in the Arctic vortex. Here, we discuss further aspects of the HALOE observations in the Arctic over this period. Potential problems, both in the data themselves and in the methodology of the data analysis are considered and the reason for the differences between the Arctic ozone losses deduced from HALOE data version 17 and 18 is analysed. Moreover, it is shown that HALOE measurements in the Arctic in winter and spring 1995–96 compare well with observations by other ground-based and satellite instruments. 相似文献