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During a cruise aboard the R/V Hakuho-maru in the northwestern North Pacific in the summer of 1998 the particle number concentrations
and the major ionic components of size fractionated aerosols were measured to investigate the aerosol produced by marine biological
activity. Continuous low concentrations of nitrate (<1.8 nmol m−3), similar to the marine air background level, were found over the northwestern North Pacific (40–45°N) and the Sea of Okhotsk
(44–45°N). Over the Sea of Okhotsk, a high concentration of chlorophyll-a (5.4 mg m−3) in seawater was observed, and atmospheric concentrations of non sea-salt (nss-) sulfate (44 nmol m−3), methane sulfonic acid (MSA) (1.8 nmol m−3) and particle number in the size range of 0.1 < D < 0.5 μm (199 cm−3) were found to be 9, 7, and 2 times, respectively, higher than those in the background marine air. The increase in particle
number concentrations mainly in the size range of 0.2 < D < 0.3 μm was likely caused by the increase of biogenic sulfate over the high productive region of the Sea of Okhotsk. In
humid air conditions (R.H. > 96%), the increased biogenic sulfate that condensed the large amount of water vapor would not
have sufficient solute mass to activate as cloud condensation nuclei (CNN) and would remain as aerosol particles in the marine
air with frequent sea-fogs over the high productive region. Biogenic sulfate originating from dimethyl sulfide (DMS) would
gradually grow into the CCN size and continuously supply a great number of CCN to the marine air in the northwestern North
Pacific.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
3.
Francesco Canganella Giovanna Bianconi Agata Gambacorta Chiaki Kato Katsuyuki Uematsu 《Marine Ecology》2002,23(S1):1-10
Abstract. Hydrothermal vent ecosystems have been extensively investigated during the last 20 years; shallow water hot springs (typically found below 50 m depth) have also been studied, and from these ecosystems many thermophilic and hyperthermophilic organisms were isolated and described.
The submarine caves of Cape Palinuro were discovered long ago, but only during the last decades were geological and biological investigations carried out, yielding a large number of reports on this fascinating environment. During the last two years, several samples of water, mud, and/or bacterial mat were collected within the "Grotta Azzurra", and enrichment experiments were performed using peptone, starch, glucose or pullulan as main organic nutrients. Many heterotrophic strains were isolated and most of them grew optimally between 37 and 43 ° C with the addition of 0-2 % NaCl. Growth was usually observed between 10 and 50 ° C the range of growth pH was 4 to 9, and NaCl concentrations up to 10–12 % were tolerated in most cases.
The analysis of 16S rDNA performed with the most representative isolates showed a close phylogenetic relationship with the genera Bacillus, Vibrio, Citrobacter and Escherichia. Moreover, an isolate showing morphological and physiological similarities with the genus Enterococcus was characterised and taxonomically described based on the 16S rDNA sequence. 相似文献
The submarine caves of Cape Palinuro were discovered long ago, but only during the last decades were geological and biological investigations carried out, yielding a large number of reports on this fascinating environment. During the last two years, several samples of water, mud, and/or bacterial mat were collected within the "Grotta Azzurra", and enrichment experiments were performed using peptone, starch, glucose or pullulan as main organic nutrients. Many heterotrophic strains were isolated and most of them grew optimally between 37 and 43 ° C with the addition of 0-2 % NaCl. Growth was usually observed between 10 and 50 ° C the range of growth pH was 4 to 9, and NaCl concentrations up to 10–12 % were tolerated in most cases.
The analysis of 16S rDNA performed with the most representative isolates showed a close phylogenetic relationship with the genera Bacillus, Vibrio, Citrobacter and Escherichia. Moreover, an isolate showing morphological and physiological similarities with the genus Enterococcus was characterised and taxonomically described based on the 16S rDNA sequence. 相似文献
4.
Mitsuo Uematsu 《Journal of Oceanography》1987,43(6):395-401
I am deeply honored to have been selected as a recipient of the 1987 Okada Prize by the Oceanographical Society of Japan. The present paper reviews my work and recent studies of other investigators concerning mineral aerosol (dust) particles in the marine atmosphere over the Pacific Ocean. I would like to emphasize the importance of atmospheric deposition of continental substances to the ocean environment. From consecutive measurements of atmospheric dust concentrations and total deposition fluxes at 13 island stations in the Pacific Ocean, a strong seasonal transfort pattern of dust particles was found at most of the stations. High atmospheric dust concentrations occurred during the spring in both hemispheres. There was a latitudinal gradient in both the atmospheric dust concentration and flux, with the highest values observed at midlatitudes. When combined with observations of dust storms in Asia and isentropic trajectory analysis, it was clear that the dust over the central North Pacific was transported by the upper westerly winds from the arid desert regions in central and eastern Asia. Transport times were 1–2 weeks, and in some cases, atmospheric transport paths of over 10,000 km were observed. Infrequent short-term dust events contributed most of annual atmospheric dust flux to the open ocean. These sporadic inputs are major sources for both suspended mineral matter in the water column and the non-biogenic component of deep-sea sediments in the Pacific Ocean. The impact of atmospheric dust fluxes on chemical and biological processes in the water column remains to be determined. 相似文献
5.
Dennis L. Savoie Joseph M. Prospero John T. Merrill Mitsuo Uematsu 《Journal of Atmospheric Chemistry》1989,8(4):391-415
Weekly bulk aerosol samples collected at Funafuti, Tuvalu (8°30S, 179°12E), American Samoa (14°15S, 170°35W), and Rarotonga (21°15S, 159°45W), from 1983 through most of 1987 have been analyzed for nitrate and other constituents. The mean nitrate concentration is about 0.11 g m–3 at each of these stations: 0.107±0.011 g m–3 at Funafuti; 0.116±0.008 at American Samoa; and 0.117±0.010 at Rarotonga. Previous measurements of mineral aerosol and trace metal concentrations at American Samoa are among the lowest ever recorded for the near-surface troposphere and indicate that this region is minimally affected by transport of soil material and pollutants from the continents. Consequently, the nitrate concentration of 0.11 g m–3 can be regarded as the natural level for the remote marine boundary layer of the tropical South Pacific Ocean. In contrast, over the tropical North Pacific which is significantly impacted by the transport of material from Asia and North America, the mean nitrate concentrations are about three times higher, 0.29 and 0.36 g m–3 at Midway and Oahu, respectively. The major sources of the nitrate over the tropical South Pacific are still very uncertain. A very significant correlation between the nitrate concentrations at American Samoa and the concentrations of 210Pb suggests that transport from continental sources might be important. This continental source could be lightning, which occurs most frequently over the tropical continents. A near-zero correlation with 7Be indicates that the stratosphere and upper troposphere are probably not the major sources. A significant biogenic source would be consistent with the higher mean nitrate concentrations, 0.16 to 0.17 g m–3, found over the equatorial Pacific at Fanning Island (3°55N, 159°20W) and Nauru (0°32S, 166°57E). The lack of correlation between nitrate and nss sulfate at American Samoa does not necessarily preclude an important role for marine biogenic sources. 相似文献
6.
The downward flux of Mn through the water column was directly measured using sediment traps. The Mn flux from the bottom sediment to the water column, and the removal rate of Mn in the bottom water were estimated from Mn gradients in the bottom water. The sediment traps were deployed more than ten times at the same station in Funka Bay, Japan. The trapped settling matter and filtered suspended matter samples were analyzed for Mn, Fe, Al and ignition loss. The observed downward flux of Mn through the water column in winter (1.3–2.8 μg/cm2 /day) was generally an order of magnitude larger than that in summer (0.13–0.45 μg/cm2 /day), and the Mn fluxes for both seasons were also greater than the accumulation rate of Mn in the bottom sediments (0.10 μg/cm 2/day). More Al was contained in the trapped settling matter than in the suspended matter, while Mn showed the opposite behavior. The Fe/Mn ratio of the residual fraction (obtained by subtracting the sediment component of the settling matter) was rather well correlated with the corresponding ratio in suspended matter. Settling particles are expected to scavenge suspended matter during their passage through the water column. The flux of Mn across the sediment—water interface was estimated from its vertical profiles in the water column to be 0.1–0.3 μg/cm2 day. The residence time of Mn in bottom water was about one to several months. These results suggest that Mn is actively recycled between the water column and the sediments of the coastal sea. 相似文献
7.
Suspended particles collected from surface seawater during the SEEDS II (Subarctic Iron Experiment for Ecosystem and Dynamics Study II) experiment were analyzed individually using an electron probe X-ray micro analyzer and characterized by size and elemental composition. Their numbers, relative abundances, and relative particle volume all showed clear differences between samples collected inside vs. outside the phytoplankton bloom that developed following the addition of iron. Throughout the study, Si-rich, Ca-rich and Organic particles were dominant and their number increased inside the fertilized patch; these particles accounted for 21%, 13% and 58% of the particles examined, respectively. Si-rich or Ca-rich particles commonly consisted of fragments of diatom frustules and coccolithophorids. There was consistently greater percentage of Ca-rich particles and lower percentage of Si-rich particles inside the patch than outside of it in number, but both types of these particles apparently occupied a larger volume inside the patch than outside of it. Organic particles, that showed having peaks in smaller diameter particles, increased apparently inside the patch with time after iron fertilization. The Organic particles had a more diverse mixture of both bio-related and crustal trace elements than the other types of particles. These results suggest that the increase in suspended particles following the iron enrichment was due to a combination of detrital material and live phytoplankton. 相似文献
8.
A.J. Gooday K. Uematsu H. Kitazato T. Toyofuku J.R. Young 《Deep Sea Research Part I: Oceanographic Research Papers》2010,57(2):239-247
We examined four multilocular agglutinated foraminiferan tests from the Challenger Deep, the deepest point in the world's oceans and well below the depth at which biogenic and most detrital minerals disappear from the sediment. The specimens represent undescribed species. Three are trochamminaceans in which imprints and other traces of dissolved agglutinated particles are visible in the orange or yellowish organic test lining. In Trochamminacean sp. A, a delicate meshwork of organic cement forms ridges between the grain impressions. The remnants of test particles include organic structures identifiable as moulds of coccoliths produced by the genus Helicosphaera. Their random alignment suggests that they were agglutinated individually rather than as fragments of a coccosphere. Trochamminacean sp. C incorporates discoidal structures with a central hole; these probably represent the proximal sides of isolated distal shields of another coccolith species, possibly Hayaster perplexus. Imprints of planktonic foraminiferan test fragments are also present in both these trochamminaceans. In Trochamminacean sp. B, the test surface is densely pitted with deep, often angular imprints ranging from roughly equidimensional to rod-shaped. The surfaces are either smooth, or have prominent longitudinal striations, probably made by cleavage traces. We presume these imprints represent mineral grains of various types that subsequently dissolved. X-ray microanalyses reveal strong peaks for Ca associated with grain impressions and coccolith remains in Trochamminacean sp. C. Minor peaks for this element are associated with coccolith remains and planktonic foraminiferan imprints in Trochamminacean sp. A. These Ca peaks possibly originate from traces of calcite remaining on the test surfaces. Agglutinated particles, presumably clay minerals, survive only in the fourth specimen (‘Textularia’ sp.). Here, the final 4–5 chambers comprise a pavement of small, irregularly shaped grains with flat surfaces and no obvious intervening cement. Our observations suggest that (1) small biogenic particles can reach the deepest parts of the ocean intact in rapidly sinking phytodetrital aggregates or faecal pellets and (2) some agglutinated foraminifera living at extreme hadal depths construct a test from biogenic or detrital particles, which subsequently dissolve, leaving imprints and other remnants in the organic matrix of the test. 相似文献
9.
Jinyoung?JungEmail author Hiroshi?Furutani Mitsuo?Uematsu 《Journal of Atmospheric Chemistry》2011,68(2):157-181
Aerosol and rain samples were collected between 48°N and 55°S during the KH-08-2 and MR08-06 cruises conducted over the North
and South Pacific Ocean in 2008 and 2009, to estimate dry and wet deposition fluxes of atmospheric inorganic nitrogen (N).
Inorganic N in aerosols was composed of ~68% NH4+ and ~32% NO3– (median values for all data), with ~81% and ~45% of each species being present on fine mode aerosol, respectively. Concentrations
of NH4+ and NO3− in rainwater ranged from 1.7–55 μmol L−1 and 0.16–18 μmol L−1, respectively, accounting for ~87% by NH4+ and ~13% by NO3− of total inorganic N (median values for all data). A significant correlation (r = 0.74, p < 0.05, n = 10) between NH4+ and methanesulfonic acid (MSA) was found in rainwater samples collected over the South Pacific, whereas no significant correlations
were found between NH4+ and MSA in rainwater collected over the subarctic (r = 0.42, p > 0.1, n = 6) and subtropical (r = 0.33, p > 0.5, n = 6) western North Pacific, suggesting that emissions of ammonia (NH3) by marine biological activity from the ocean could become a significant source of NH4+ over the South Pacific. While NO3− was the dominant inorganic N species in dry deposition, inorganic N supplied to surface waters by wet deposition was predominantly
by NH4+ (42–99% of the wet deposition fluxes for total inorganic N). We estimated mean total (dry + wet) deposition fluxes of atmospheric
total inorganic N in the Pacific Ocean to be 32–64 μmol m−2 d−1, with 66–99% of this by wet deposition, indicating that wet deposition plays a more important role in the supply of atmospheric
inorganic N than dry deposition. 相似文献
10.
Yuto Kurumada Shogo Aoki Kazumasa Aoki Daichi Kato Mototaka Saneyoshi Khishigjav Tsogtbaatar Brian F. Windley Shinobu Ishigaki 《地学学报》2020,32(4):246-252
To verify the usefulness of calcite U–Pb measurement for vertebrate‐bearing strata in the Eastern Gobi, Mongolia, we performed laser ablation‐inductively coupled plasma‐mass spectrometry calcite U–Pb and trace element analyses of three caliche (calcrete) of the Bayn Shire Formation. The trace element analysis demonstrates high concentration of U in the calcites. Two meaningful calcite U–Pb ages were obtained; 95.9 ± 6.0 and 89.6 ± 4.0 Ma, which are consistent with published ages from the Bayn Shire Formation. Our results demonstrate that the calcite U–Pb method can be powerful tool for age determination of vertebrate‐bearing strata in the Gobi that do not contain index fossils or beds, but do contain caliches. This would make it possible for a comparison of biostratigraphy between the Gobi and other areas yielding abundant vertebrate fossils in Asia, North America and Europe, based on chronological data. 相似文献