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Ines Bamberger Brian Oney Dominik Brunner Stephan Henne Markus Leuenberger Nina Buchmann Werner Eugster 《Boundary-Layer Meteorology》2017,164(1):135-159
Mountain-top observations of greenhouse gas mixing ratios may be an alternative to tall-tower measurements for regional scale source and sink estimation. To investigate the equivalence or limitations of a mountain-top site as compared to a tall-tower site, we used the unique opportunity of comparing in situ measurements of methane (\(\hbox {CH}_{4}\)) and carbon dioxide (\(\hbox {CO}_{2}\)) mixing ratios at a mountain top (986 m above sea level, a.s.l.) with measurements from a nearby (distance 28.4 km) tall tower, sampled at almost the same elevation (1009 m a.s.l.). Special attention was given to, (i) how local wind statistics and greenhouse gas sources and sinks at the mountain top influence the observations, and (ii) whether mountain-top observations can be used as for those from a tall tower for constraining regional greenhouse gas emissions. Wind statistics at the mountain-top site are clearly more influenced by local flow systems than those at the tall-tower site. Differences in temporal patterns of the greenhouse gas mixing ratios observed at the two sites are mostly related to the influence of local sources and sinks at the mountain-top site. Major influences of local sources can be removed by applying a statistical filter (\(5{\mathrm{th}}\) percentile) or a filter that removes periods with unfavourable flow conditions. In the best case, the bias in mixing ratios between the mountain-top and the tall-tower sites after the application of the wind filter was \({-}0.0005\pm 0.0010\) ppm for methane (September, 0000–0400 UTC) and \(0.11\pm 0.18\) ppm for \(\hbox {CO}_{2}\) (February, 1200–1600 UTC). Temporal fluctuations of atmospheric \(\hbox {CH}_{4}\) and \(\hbox {CO}_{2}\) mixing ratios at both stations also showed good agreement (apart from \(\hbox {CO}_{2}\) during summertime) as determined by moving bi-weekly Pearson correlation coefficients (up to 0.96 for \(\hbox {CO}_{2}\) and 0.97 for \(\hbox {CH}_{4}\)). When only comparing mixing ratios minimally influenced by local sources (low bias and high correlation coefficients), our measurements indicate that mountain-top observations are comparable to tall-tower observations. 相似文献
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Martina Bisculm Daniele Colombaroli Elisa Vescovi Jacqueline F. N. van Leeuwen Paul D. Henne Julian Rothen Giovanni Procacci Salvatore Pasta Tommaso La Mantia Willy Tinner 《第四纪科学杂志》2012,27(7):687-698
High‐resolution pollen, macrofossil and charcoal data, combined with accelerator mass spectrometry 14C dating and multivariate analysis, were used to reconstruct Holocene vegetation and fire dynamics at Urio Quattrocchi, a small lake in the supra‐mediterranean belt in the Nebrodi Mountains of Sicily (Italy). The data suggest that after 10 000 cal a BP increasing moisture availability supported closed forests with deciduous (Quercus cerris, Fagus sylvatica and Fraxinus spp.) and evergreen (Quercus ilex) species. Species‐rich closed forest persisted until 6850 cal a BP, when Neolithic activities caused a forest decline and affected plant diversity. Secondary forest with abundant Ilex aquifolium recovered between 6650 and 6000 cal a BP, indicating moist conditions. From 5000 cal a BP, agriculture and pastoralism led to the currently fragmented landscape with sparse deciduous forests (Quercus cerris). The study suggests that evergreen broadleaved species were more important at elevations above 1000 m a.s.l. before ca. 5000 cal a BP than subsequently, which might reflect less human impact or warmer‐than‐today climatic conditions between 10 000 and 5000 cal a BP. Despite land use since Neolithic times, deciduous supra‐mediterranean forests were never completely displaced from the Nebrodi Mountains, because of favourable moist conditions that persisted throughout the Holocene. Reconstructed vegetation dynamics document the absence of any pronounced mid‐ or late‐Holocene ‘aridification’ trend at the site, an issue which is controversially debated in Italy and the Mediterranean region. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
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Willy Tinner Jacqueline F.N. van Leeuwen Daniele Colombaroli Elisa Vescovi W.O. van der Knaap Paul D. Henne Salvatore Pasta Stefania D'Angelo Tommaso La Mantia 《Quaternary Science Reviews》2009,28(15-16):1498-1510
We used a new sedimentary record to reconstruct the Holocene vegetation and fire history of Gorgo Basso, a coastal lake in south-western Sicily (Italy). Pollen and charcoal data suggest a fire-prone open grassland near the site until ca 10,000 cal yr BP (8050 cal BC), when Pistacia shrubland expanded and fire activity declined, probably in response to increased moisture availability. Evergreen Olea europaea woods expanded ca 8400 to decline abruptly at 8200 cal yr BP, when climatic conditions became drier at other sites in the Mediterranean region. Around 7000 cal yr BP evergreen broadleaved forests (Quercus ilex, Quercus suber and O. europaea) expanded at the cost of open communities. The expansion of evergreen broadleaved forests was associated with a decline of fire and of local Neolithic (Ficus carica–Cerealia based) agriculture that had initiated ca 500 years earlier. Vegetational, fire and land-use changes ca 7000 cal yr BP were probably caused by increased precipitation that resulted from (insolation-forced) weakening of the monsoon and Hadley circulation ca 8000–6000 cal yr BP. Low fire activity and dense coastal evergreen forests persisted until renewed human activity (probably Greek, respectively Roman colonists) disrupted the forest ca 2700 cal yr BP (750 BC) and 2100 cal yr BP (150 BC) to gain open land for agriculture. The intense use of fire for this purpose induced the expansion of open maquis, garrigue, and grassland-prairie environments (with an increasing abundance of the native palm Chamaerops humilis). Prehistoric land-use phases after the Bronze Age seem synchronous with those at other sites in southern and central Europe, possibly as a result of climatic forcing. Considering the response of vegetation to Holocene climatic variability as well as human impact we conclude that under (semi-)natural conditions evergreen broadleaved Q. ilex–O. europaea (s.l.) forests would still dominate near Gorgo Basso. However, forecasted climate change and aridification may lead to a situation similar to that before 7000 cal yr BP and thus trigger a rapid collapse of the few relict evergreen broadleaved woodlands in coastal Sicily and elsewhere in the southern Mediterranean region. 相似文献
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The Macraes orogenic gold deposit is hosted by a graphitic micaceous schist containing auriferous porphyroblastic sulphides. The host rock resembles zones of unmineralised micaceous graphitic pyritic schists, derived from argillaceous protoliths, that occur locally in background pelitic Otago Schist metasediments. This study was aimed at determining the relationship between these similar rock types, and whether the relationship had implications for ore formation. Argillites in the protolith turbidites of the Otago Schist metamorphic belt contain minor amounts of detrital organic matter (<0.1 wt.%) and diagenetic pyrite (<0.3 wt.% S). The detrital organic carbon was mobilised by metamorphic–hydrothermal fluids and redeposited as graphite in low-grade metaturbidites (pumpellyite–actinolite and greenschist facies). This carbon mobility occurred through >50 million years of evolution of the metamorphic belt, from development of sheared argillite in the Jurassic, to postmetamorphic ductile extension in the Cretaceous. Introduced graphite is structurally controlled and occurs with metamorphic muscovite and chlorite as veins and slicken-sided shears, with some veins having >50% noncarbonate carbon. Graphitic foliation seams in low-grade micaceous schist and metamorphic quartz veins contain equant graphite porphyroblasts up to 2 mm across that are composed of crystallographically homogeneous graphite crystals. Graphite reflectance is anisotropic and ranges from ~1% to ~8% (green light). Texturally similar porphyroblastic pyrite has grown in micaceous schist (up to 10 wt.% S), metamorphic quartz veins and associated muscovite-rich shears. These pyritic schists are weakly enriched in arsenic (up to 60 ppm). The low-grade metamorphic mobility and concentration of graphite in micaceous schists is interpreted to be a precursor process that structurally and geochemically prepared parts of the Otago Schist belt for later (more restricted) gold mineralisation. Economic amounts of gold, and associated arsenic, were subsequently introduced to carbonaceous sulphidic schists in the Macraes gold deposit by a separate metamorphic fluid derived from high-grade metaturbidites. Fluid flow at all stages in these processes occurred at metamorphic rates (mm/year), and fluids were broadly in equilibrium with the rocks through which they were passing. 相似文献
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Katharopoulos Ioannis Brunner Dominik Emmenegger Lukas Leuenberger Markus Henne Stephan 《Boundary-Layer Meteorology》2022,185(1):129-160
Boundary-Layer Meteorology - Lagrangian particle dispersion models (LPDMs) are frequently used for regional-scale inversions of greenhouse gas emissions. However, the turbulence parameterizations... 相似文献
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