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1.
Casey Saenger Thomas M. Cronin Debra Willard Jeffrey Halka Randy Kerhin 《Estuaries and Coasts》2008,31(3):492-500
We calculated Chesapeake Bay (CB) sediment and carbon fluxes before and after major anthropogenic land clearance using robust monitoring, modeling and sedimentary data. Four distinct fluxes in the estuarine system were considered including (1) the flux of eroded material from the watershed to streams, (2) the flux of suspended sediment at river fall lines, (3) the burial flux in tributary sediments, and (4) the burial flux in main CB sediments. The sedimentary maximum in Ambrosia (ragweed) pollen marked peak land clearance (~1900 a.d.). Rivers feeding CB had a total organic carbon (TOC)/total suspended solids of 0.24?±?0.12, and we used this observation to calculate TOC fluxes from sediment fluxes. Sediment and carbon fluxes increased by 138–269% across all four regions after land clearance. Our results demonstrate that sediment delivery to CB is subject to significant lags and that excess post-land clearance sediment loads have not reached the ocean. Post-land clearance increases in erosional flux from watersheds, and burial in estuaries are important processes that must be considered to calculate accurate global sediment and carbon budgets. 相似文献
2.
Stanislav FRANCISKOVIC-BILINSKI Halka BILINSKI Delko BARISIC Nada HORVATINCIC Institute Ruder BoSkovi POB HR- Zagre Croati E-mail: francis@rudjer.irb.hrand YUAN Daoxian Institute of Karst Geology Guilin Guangxi China 《《地质学报》英文版》2003,77(2):267-275
The paper presents an analysis of characteristic karst tufa from Guangxi, China, which has not been studied before. A comparison with tufa from Dinaric Karst of Croatia is discussed in view of the C-type climate. The major mineral is calcite. Minor minerals are quartz and dolomite, depending on location. The content of calcium carbonate varies from 65% to 92%, and that of magnesium carbonate from 0.03% to 1.77%. Among other elements, the most abundant are Fe, from 0.02% to 1.50%, and Ti, from 0.15% to 0.27%. Many other trace elements (V, Cr, Mn, Ni, Cu, Zn, As, Se, Br, Rb, Sr, Y, Zr, Hg and Pb) are also present. Specific activity of radionuclides 40K, 232Th, 137Cs, 226Ra and 238U varies from sample to sample. Concentration of U in tufa is close to that reported for sedimentary carbonate. Low concentration of 137Cs indicates that this part of the world was not exposed to nuclear explosions. The concentration of 226Ra is the highest in Mashan County. The ratio 238U/226Ra (0.21-0.71) in tufa from Mashan Co 相似文献
3.
A series of cruises was carried out in the estuarine turbidity maximum (ETM) region of Chesapeake Bay in 1996 to examine physical and biological variability and dynamics. A large flood event in late January shifted the salinity structure of the upper Bay towards that of a salt wedge, but most of the massive sediment load delivered by the Susquehanna River appeared to bypass the ETM zone. In contrast, suspended sediments delivered during a flood event in late October were trapped very efficiently in the ETM. The difference in sediment trapping appeared to be due to increases in particle settling speed from January to October, suggesting that the fate of sediments delivered during large events may depend on the season in which they occur. The ETM roughly tracked the limit of salt (defined as the intersection of the 1 psu isohaline with the bottom) throughout the year, but it was often separated significantly from the limit of salt with the direction of separation unrelated to the phase of the tide. This was due to a lag of ETM sediment resuspension and transport behind rapid meteorologically induced or river flow induced motion of the salt limit. Examination of detailed time series of salt, suspended sediment, and velocity collected near the limit of salt, combined with other indications, led to the conclusion that the convergence of the estuarine circulation at the limit of salt is not the primary mechanism of particle trapping in the Chesapeake Bay ETM. This convergence and its associated salinity structure contribute to strong tidal asymmetries in sediment resuspension and transport that collect and maintain a resuspendable pool of rapidly settling particles near the salt limit. Without tidal resuspension and transport, the ETM would either not exist or be greatly weakened. In spite of this repeated resuspension, sedimentation is the ultimate fate of most terrigenous material delivered to the Chesapeake Bay ETM. Sedimentation rates in the ETM channel are at least an order of magnitude greater than on the adjacent shoals, probably due to focusing mechanisms that are poorly understood. 相似文献
4.
Deposits of dredged cohesive sediments were monitored for changes in volume, bulk characteristics, and susceptibility to resuspension
and erosion at disposal sites in Chesapeake Bay. There is a 23–48% volume reduction during the first six months, with correspondingly
greater changes over longer time periods. A bulk density increase from 1.15 to 1.3 g/cm3 due to dewatering and compaction accounts for the majority of the volume change. Tidal current induced resuspension is a
minor process. The observed suspended sediment load can be accounted for by erosion of only a fraction of a millimeter of
sediment on each tidal cycle. 相似文献
5.
The solubilities of PbCO3(s), 2PbCO2·Pb(OH)2(s), and of 3PbCO3 2Pb(OH)2(s) have been studied at 25°C ± 0.1°C in solutions of the constant ionic strength I = 0.3 mol/dm3, consisting primarily of sodium perchlorate. A few experiments with hydrocerussite were performed in solutions of 0.1 M KNO3. The concentrations of lead and hydrogen ions have been determined in solution in contact with the solid phase. From experimental data the following values for equilibrium constants are obtained: log [Pb2+]·pCO2·[H+]?2 = 5.20log [Pb2+]·pCO0.672·[H+]?2 = 6.80log [Pb2+]3·[CO2?3]2·[OH?]2 = ?44.08 (and ?44.8 forI = 0.1 M)log [PbCO03]·[Pb2+]?1·[CO2?3]?1 = 5.40log [Pb(CO3)2?2]·[Pb2+]?1·[CO2?3]?2 = 8.86 The data indicate that hydrocerussite is the most stable solid phase in natural waters. Comparison with the literature and needs for further research are also presented. 相似文献
6.
Kwokal Z Francisković-Bilinski S Bilinski H Branica M 《Marine pollution bulletin》2002,44(10):1152-1157
Anthropogenic mercury pollution was studied in Kastela Bay (Croatia), 10 years after chloralkaline plant (PVC) stopped production. The concentration of total mercury determined in sediments which are composed mainly of calcite and quartz, are in the range 14,280-30,400 ng/g. The values are higher than reported in the literature for Elbe and Seine estuaries and also above 25,000 ng/g used for criterion in remediation project in Minamata Bay. The concentration of methylmercury 6.05-36.74 ng/g are typical for slightly to highly contaminated estuarine sediments. The low ratio of methylmercury to total mercury found in sediments of Kastela Bay is in the range 0.04-0.18%. It can be explained that in this region predominate conditions which do not promote in-situ methylation. Sediments were found to be highly anoxic. Concentrations of total mercury in unfiltered surface waters are in the range 69-145 ng/l and in unfiltered bottom waters in the range 230-1,418 ngl(-1). High concentrations found in bottom waters suggest that either resuspension or partial dissolution of sediments takes place. An experiment performed on filtered and unfiltered waters showed that about 85% of total mercury in surface water and almost 100% in bottom water was retained on 45 microm filters. To demonstrate contrasts, two pristine estuaries from norths and south Europe were studied. Silicious sediments of Ore estuary (Sweden) and calcareous sediments of Krka estuary (Croatia) have total mercury concentrations close to accepted background level. The ratio of methylmercury to total mercury is < or = 1% in all samples with one exception. The highest observed ratio (2.70%) was in the surface sediment from E2 station in Krka estuary measured in March 2000. This location is suitable for studying methylmercury formation in pristine environment. 相似文献
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8.
Stanislav Frančišković-Bilinski Vlado Cuculić Halka Bilinski Hermann Häusler Philipp Stadler 《Chemie der Erde / Geochemistry》2013
Complementary geochemical and stable isotope investigations of the Gorski Kotar karst aquifer system in western Croatia were obtained for the first time, to answer the question whether both studied rivers drain the same aquifer system or not. The two main rivers, the Kupa and the Rje?ina, rise under the same mountain range, but belong to two different watersheds (Black Sea and Adriatic Sea). The karst aquifer of Gorski Kotar is a potentially important source of drinking water for two neighboring countries, Croatia and Slovenia (Central and South Europe), and is strongly influenced by both Mediterranean and continental weather conditions. It is a part of the Dinaric karst, which is “locus typicus” for karst worldwide and one of the most typical karst areas in the world. 相似文献
9.
Stanislav Frančišković-Bilinski Robert Scholger Halka Bilinski Darko Tibljaš 《Environmental Earth Sciences》2014,72(10):3939-3953
The aim of the present work was to investigate links between the low-field magnetic susceptibility (MS) and chemical and mineral composition of sediments from several Croatian and Slovenian rivers, as well as to determine possible anthropogenic influence on these sediments. MS measurements are a fast and simple method, which serves as a proxy for the estimation of pollution in different environmental systems. The investigated rivers are predominantly unpolluted rivers from Croatian and Slovenian karstic and flysch areas, which belong to the Adriatic or the Black Sea watersheds: the Dragonja, the Mirna, the Ra?a, the Ri?ana, the Reka, the Rak, the Cerkni?nica, the Unec and the Ljubljanica rivers. It was assumed that, due to their mostly unpolluted status, they could serve as a database for natural MS background values for this region. For comparison, several rivers and a lake from the Celje old metallurgic industrial area (Slovenia) were also investigated: the Savinja, the Hudinja, the Voglajna rivers and Slivni?ko Lake. They form a sub-basin of the Sava River drainage basin. Sediments of the clean karstic and flysch rivers showed extremely low MS values, with mass susceptibility values ranging from 0.58 × 10?7 to 5.11 × 10?7 m3/kg, and isothermal remanent magnetism (IRM) values ranging from 0.71 to 7.88 A/m. In the Celje industrial area, river sediments showed much higher MS values, with mass susceptibility values ranging from 1.31 × 10?7 to 38.3 × 10?7 m3/kg, and IRM values ranging from 0.91 to 100.42 A/m. The highest MS value was found in the Voglajna River at Teharje-?tore, a point which showed a significant number of anomalies of toxic metals in earlier investigations. Semiquantitative determination of relations between grain size and concentration of magnetite was performed using the Thompson-Oldfield method. X-ray diffraction (XRD) mineralogical analysis showed that sediments of the Celje area have mostly quartz as major mineral, with relatively small amount of carbonate minerals, while in sediments of karstic rivers carbonate minerals prevail. Statistically significant correlations were obtained between MS and Cr, Mn, Fe, Co, Ni, Cu, Zn, Cd and Ba in the Slovenian karstic region and between MS and Cr, Fe, Co, Ni and Zn in flysch drainage basins. On the contrary, no correlation of MS and Hg content was obtained. 相似文献
10.