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Thallium diagenesis in lacustrine sediments 总被引：1，自引：0，他引：1
Dated sediment cores and porewaters from two Canadian Shield lakes, located 40 km from Québec City (L. Tantaré) and 25 km downwind from an important smelter in northwestern Québec (L. Vose), were analyzed for thallium and other geochemical variables. Atmospheric deposition is the only source of anthropogenic Tl to these lakes. The porewater Tl concentration profiles in L. Tantaré display a peak below the sediment-water interface that suggests post-depositional Tl remobilization and transport to the overlying water and deeper sediments; such a dissolved Tl peak occurs just above the sediment-water interface in L. Vose. Modeling the porewater Tl profiles with a diagenetic reaction-transport equation reveals a zone of dissolved Tl production lying above a zone of Tl consumption in L. Tantaré sediments. In contrast, in L. Vose, Tl diffuses across the sediment-water interface from the anoxic hypolimnion and is fixed to the surficial sediments. The localization of the consumption zones, the shape of the dissolved Tl, sulfide and iron profiles, as well as calculations of saturation states are all consistent with the removal of Tl from porewater by co-precipitation with and/or adsorption to Fe sulfides. The concentrations of Tl removed from or added to sediments after their deposition (i.e., diagenetic Tl) amount to up to 36% of measured sediment Tl concentrations. Comparison of the reconstructed historical Tl records with those of polycyclic aromatic hydrocarbons (PAHs) and of Pb originating from coal burning or from smelting activities indicate that coal combustion is the major source of atmospheric Tl to L. Tantaré and that an additional important Tl source to L. Vose is the nearby smelter. 相似文献
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Lucie Juřičková Jitka Horáčková Vojen Ložek Michal Horsák 《Boreas: An International Journal of Quaternary Research》2013,42(4):932-946
Analyses of fossil mollusc successions have rarely been used to study the development of floodplain forests during the Holocene. The Oh?e River, located in a prehistorically settled chernozem area in the Czech Republic, is partly situated in Cretaceous marlstones, yielding sediments suitable for fossilization directly in floodplain deposits. We analysed five fossil mollusc successions situated in the lower stretch of the Oh?e River and compared the results with recent mollusc assemblages studied along the entire 256 km of the river. Fossil samples were composed mostly of open‐country species throughout the Holocene or the whole preserved succession. Only some samples also contained woodland assemblages, but these were always greatly impoverished, with a very low frequency of strictly woodland species. Although the natural‐looking appearance of the present‐day floodplain forests of the lower river stretch has resulted in its being declared a nature reserve, modern floodplain forest mollusc assemblages there are also impoverished. This reduction in the distribution of strictly woodland species compared with modern assemblages in the upper stretch of the river seems to be the result of an ancient human settlement and continuous disturbances of the floodplain forest development since the Neolithic. Thus, fully developed floodplain forest assemblages occur recently only in the upper non‐impacted stretch of the river. Based on the studied fossil successions we can conclude that the lower Oh?e River floodplain was probably a mosaic of open and disturbed forest habitats throughout the Holocene. This area is part of a central European landscape island, where forests probably never fully developed and open patches from the early Holocene continually developed into an agricultural landscape. 相似文献
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Abstract Trends in Canadian temperature and precipitation during the 20th century are analyzed using recently updated and adjusted station data. Six elements, maximum, minimum and mean temperatures along with diurnal temperature range (DTR), precipitation totals and ratio of snowfall to total precipitation are investigated. Anomalies from the 1961–1990 reference period were first obtained at individual stations, and were then used to generate gridded datasets for subsequent trend analyses. Trends were computed for 1900–1998 for southern Canada (south of 60°N), and separately for 1950–1998 for the entire country, due to insufficient data in the high arctic prior to the 1950s. From 1900–1998, the annual mean temperature has increased between 0.5 and 1.5°C in the south. The warming is greater in minimum temperature than in maximum temperature in the first half of the century, resulting in a decrease of DTR. The greatest warming occurred in the west, with statistically significant increases mostly seen during spring and summer periods. Annual precipitation has also increased from 5% to 35% in southern Canada over the same period. In general, the ratio of snowfall to total precipitation has been increasing due mostly to the increase in winter precipitation which generally falls as snow and an increase of ratio in autumn. Negative trends were identified in some southern regions during spring. From 1950–1998, the pattern of temperature change is distinct: warming in the south and west and cooling in the northeast, with similar magnitudes in both maximum and minimum temperatures. This pattern is mostly evident in winter and spring. Across Canada, precipitation has increased by 5% to 35%, with significant negative trends found in southern regions during winter. Overall, the ratio of snowfall to total precipitation has increased, with significant negative trends occurring mostly in southern Canada during spring. Indices of abnormal climate conditions are also examined. These indices were defined as areas of Canada for 1950–1998, or southern Canada for 1900–1998, with temperature or precipitation anomalies above the 66th or below the 34th percentiles in their relevant time series. These confirmed the above findings and showed that climate has been becoming gradually wetter and warmer in southern Canada throughout the entire century, and in all of Canada during the latter half of the century. 相似文献
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Huth Radan Mládek Richard Metelka Ladislav Sedlák Pavel Huthová Zuzana Kliegrová Stanislava Kyselý Jan Pokorná Lucie Halenka Tomáš Janoušek Martin 《Studia Geophysica et Geodaetica》2003,47(4):863-873
This note summarizes results of the first integration of regional numerical weather prediction model ALADIN in a climate mode. The ALADIN model, developed in an international cooperation led by Météo France, is operationally used for weather prediction. The grid step of the model is 12 km; the integration domain covers a major part of Europe. A one-month-long run has been performed with this model on observed boundary conditions (represented by assimilations by the global model ARPEGE). It is demonstrated that no excessive error is generated and accumulated in the model during the integration; hence the model is integrable for extended time periods and may serve a basis for a development towards a regional climate model. 相似文献
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Heat waves and dry spells are analyzed (i) at eightstations in south Moravia (Czech Republic), (ii) inthe control ECHAM3 GCM run at the gridpoint closest tothe study area, and (iii) in the ECHAM3 GCM run fordoubled CO2 concentrations (scenario A) at thesame gridpoint (heat waves only). The GCM outputs arevalidated both against individual station data andareally representative values. In the control run, theheat waves are too long, appear later in the year,peak at higher temperatures and their numbers areunder- (over-) estimated in June and July (in August).The simulated dry spells are too long, and the annualcycle of their occurrence is distorted.Mid-tropospheric circulation, and heat waves and dryspells are linked much less tightly in the controlclimate than in the observed. Since mid-troposphericcirculation is simulated fairly successfully, wesuggest the hypothesis that either the air-masstransformation and local processes are too strong inthe model or the simulated advection is too weak. Inthe scenario A climate, the heat waves become a commonphenomenon: warming of 4.5 °C in summer(difference between scenario A and control climates)induces a five-fold increase in the frequency oftropical days and an immense enhancement of extremityof heat waves. The results of the study underline theneed for (i) a proper validation of the GCM outputbefore a climate impact study is conducted and (ii)translation of large-scale information from GCMs intolocal scales using downscaling and stochasticmodelling techniques in order to reduce GCMs' biases. 相似文献
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Simone Dell��Agnello Caterina Lops Giovanni O. Delle Monache Douglas G. Currie Manuele Martini Roberto Vittori Angioletta Coradini Cesare Dionisio Marco Garattini Alessandro Boni Claudio Cantone Riccardo March Giovanni Bellettini Roberto Tauraso Mauro Maiello Luca Porcelli Simone Berardi Nicola Intaglietta 《Experimental Astronomy》2011,32(1):19-35
MAGIA is a mission approved by the Italian Space Agency (ASI) for Phase A study. Using a single large-diameter laser retroreflector, a large laser retroreflector array and an atomic clock onboard MAGIA we propose to perform several fundamental physics and absolute positioning metrology experiments: VESPUCCI, an improved test of the gravitational redshift in the Earth?CMoon system predicted by General Relativity; MoonLIGHT-P, a precursor test of a second generation Lunar Laser Ranging (LLR) payload for precision gravity and lunar science measurements under development for NASA, ASI and robotic missions of the proposed International Lunar Network (ILN); Selenocenter (the center of mass of the Moon), the determination of the position of the Moon center of mass with respect to the International Terrestrial Reference Frame/System (ITRF/ITRS); this will be compared to the one from Apollo and Lunokhod retroreflectors on the surface; MapRef, the absolute referencing of MAGIA??s lunar altimetry, gravity and geochemical maps with respect to the ITRF/ITRS. The absolute positioning of MAGIA will be achieved thanks to: (1) the laboratory characterization of the retroreflector performance at INFN-LNF; (2) the precision tracking by the International Laser Ranging Service (ILRS), which gives two fundamental contributions to the ITRF/ITRS, i.e. the metrological definition of the geocenter (the Earth center of mass) and of the scale of length; (3) the radio science and accelerometer payloads; (4) support by the ASI Space Geodesy Center in Matera, Italy. Future ILN geodetic nodes equipped with MoonLIGHT and the Apollo/Lunokhod retroreflectors will become the first realization of the International Moon Reference Frame (IMRF), the lunar analog of the ITRF. 相似文献
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Report of the IAU Working Group on Cartographic Coordinates and Rotational Elements: 2009 总被引：5，自引：0，他引：5
B. A. Archinal M. F. A��Hearn E. Bowell A. Conrad G. J. Consolmagno R. Courtin T. Fukushima D. Hestroffer J. L. Hilton G. A. Krasinsky G. Neumann J. Oberst P. K. Seidelmann P. Stooke D. J. Tholen P. C. Thomas I. P. Williams 《Celestial Mechanics and Dynamical Astronomy》2011,109(2):101-135
Every three years the IAU Working Group on Cartographic Coordinates and Rotational Elements revises tables giving the directions of the poles of rotation and the prime meridians of the planets, satellites, minor planets, and comets. This report takes into account the IAU Working Group for Planetary System Nomenclature (WGPSN) and the IAU Committee on Small Body Nomenclature (CSBN) definition of dwarf planets, introduces improved values for the pole and rotation rate of Mercury, returns the rotation rate of Jupiter to a previous value, introduces improved values for the rotation of five satellites of Saturn, and adds the equatorial radius of the Sun for comparison. It also adds or updates size and shape information for the Earth, Mars?? satellites Deimos and Phobos, the four Galilean satellites of Jupiter, and 22 satellites of Saturn. Pole, rotation, and size information has been added for the asteroids (21) Lutetia, (511) Davida, and (2867) ?teins. Pole and rotation information has been added for (2) Pallas and (21) Lutetia. Pole and rotation and mean radius information has been added for (1) Ceres. Pole information has been updated for (4) Vesta. The high precision realization for the pole and rotation rate of the Moon is updated. Alternative orientation models for Mars, Jupiter, and Saturn are noted. The Working Group also reaffirms that once an observable feature at a defined longitude is chosen, a longitude definition origin should not change except under unusual circumstances. It is also noted that alternative coordinate systems may exist for various (e.g. dynamical) purposes, but specific cartographic coordinate system information continues to be recommended for each body. The Working Group elaborates on its purpose, and also announces its plans to occasionally provide limited updates to its recommendations via its website, in order to address community needs for some updates more often than every 3 years. Brief recommendations are also made to the general planetary community regarding the need for controlled products, and improved or consensus rotation models for Mars, Jupiter, and Saturn. 相似文献