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Marek Tulej Andreas Riedo Maike B. Neuland Stefan Meyer Peter Wurz Nicolas Thomas Valentine Grimaudo Pavel Moreno‐García Peter Broekmann Anna Neubeck Magnus Ivarsson 《Geostandards and Geoanalytical Research》2014,38(4):441-466
Performance studies of a microscope‐camera system (MCS) and a laser ablation/ionisation mass spectrometer (LIMS) instrument (referred to here as a laser mass spectrometer or LMS) are presented. These two instruments were designed independently for in situ analysis of solids on planetary surfaces and will be combined to a single miniature instrument suite for in situ chemical and morphological analysis of surface materials on planetary bodies. LMS can perform sensitive chemical (elemental, isotope and molecular) analyses with spatial resolution close to micrometre‐sized grains. It allows for studies with mass resolution (M/ΔM) up to 800 in ablation mode (elemental composition) and up to 1500 in desorption mode (molecular analysis). With an effective dynamic range of at least eight orders of magnitude, sensitive and quantitative measurements can be conducted of almost all elements and isotopes with a concentration larger than a few ppb atoms. Hence, in addition to the major element composition, which is important for the determination of mineralogical constituents of surface materials, trace elements can also be measured to provide information on mineral formation processes. Highly accurate isotope ratio measurements can be used to determine in situ geochronology of sample material and for investigations of various isotope fractionation processes. MCS can conduct optical imagery of mm‐sized objects at several wavelengths with micrometre spatial resolution for the characterisation of morphological surface details and to provide insight into surface mineralogy. Furthermore, MCS can help in the selection of sample surface areas for further mass spectrometric analysis of the chemical composition. Surface auto‐fluorescence measurements and images in polarised light are additional capabilities of the MCS, to identify either fluorescing minerals or organic materials, if present on the analysed surface, for further investigation by LMS. The results obtained by investigations of NIST reference materials, amino acid films and a natural graphite sample embedded in silicate rock are presented to illustrate the performance of the instruments and their potential to deliver chemical information for mineral and organic phases in their geological context. 相似文献
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Annette Eicker Maike Schumacher Jürgen Kusche Petra Döll Hannes Müller Schmied 《Surveys in Geophysics》2014,35(6):1285-1309
We introduce a new ensemble-based Kalman filter approach to assimilate GRACE satellite gravity data into the WaterGAP Global Hydrology Model. The approach (1) enables the use of the spatial resolution provided by GRACE by including the satellite observations as a gridded data product, (2) accounts for the complex spatial GRACE error correlation pattern by rigorous error propagation from the monthly GRACE solutions, and (3) allows us to integrate model parameter calibration and data assimilation within a unified framework. We investigate the formal contribution of GRACE observations to the Kalman filter update by analysis of the Kalman gain matrix. We then present first model runs, calibrated via data assimilation, for two different experiments: the first one assimilates GRACE basin averages of total water storage and the second one introduces gridded GRACE data at \(5^\circ\) resolution into the assimilation. We finally validate the assimilated model by running it in free mode (i.e., without adding any further GRACE information) for a period of 3 years following the assimilation phase and comparing the results to the GRACE observations available for this period. 相似文献
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Maike Groeschke Theresa Frommen Thomas Taute Michael Schneider 《Hydrogeology Journal》2017,25(7):2185-2197
The groundwater abstracted at a well field near the Yamuna River in Central Delhi, India, has elevated ammonium (NH4 +) concentrations up to 35 mg/L and arsenic (As) concentrations up to 0.146 mg/L, constituting a problem with the provision of safe drinking and irrigation water. Infiltrating sewage-contaminated river water is the primary source of the NH4 + contamination in the aquifer, leading to reducing conditions which probably trigger the release of geogenic As. These conclusions are based on the evaluation of six 8–27-m deep drillings, and 13 surface-water and 69 groundwater samples collected during seven field campaigns (2012–2013). Results indicate that losing stream conditions prevail and the river water infiltrates into the shallow floodplain aquifer (up to 16 m thickness), which consists of a 1–2-m thick layer of calcareous nodules (locally known as kankar) overlain by medium sand. Because of its higher hydraulic conductivity (3.7 × 10?3 m/s, as opposed to 3.5 × 10?4 m/s in the sand), the kankar layer serves as the main pathway for the infiltrating water. However, the NH4 + plume front advances more rapidly in the sand layer because of its significantly lower cation exchange capacity. Elevated As concentrations were only observed within the NH4 + plume indicating a causal connection with the infiltrating reducing river water. 相似文献
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Nicole Kowalski Olaf Dellwig Melanie Beck Maik Grunwald Sibylle Fischer Maike Piepho Thomas Riedel Holger Freund Hans-Jürgen Brumsack Michael E. Böttcher 《Ocean Dynamics》2009,59(2):333-350
Tidal and seasonal behaviour of the redox-sensitive trace metals Mn, Fe, Mo, U, and V have been investigated in the open-water
column and shallow pore waters of the backbarrier tidal flats of the island of Spiekeroog (Southern North Sea) in 2002 and
2007. The purpose was to study the response of trace metal cycles on algae blooms, which are assumed to cause significant
changes in the redox state of the entire ecosystem. Trace metal data were complemented by measurements of nutrients and enumeration
of algae cells in 2007. Generally, Mn and V show a tidal cyclicity in the water column with maximum values during low tide
which is most pronounced in summer due to elevated microbial activity in the sediments. Mo and U behave almost conservatively
throughout the year with slightly increasing levels towards high tide. Exceptions are observed for both metals after summer
algae blooms. Thus, the seasonal behaviour of the trace metals appear to be significantly influenced by productivity in the
water column as the occurrence of algae blooms is associated with an intense release of organic matter (e.g. transparent exopolymer
particles, TEP) thereby forming larger organic-rich aggregates. Along with elevated temperatures in summer, the deposition
of such aggregates favours microbial activity within the surface sediments and release of DOC, nutrients and trace metals
(Mn, Mo and V) during the degradation of the aggregates. Additionally, pronounced reducing conditions lead to the reduction
of Mn(IV)-oxides and Fe(III)-(oxihydr)oxides, thereby releasing formerly scavenged compounds as V and phosphate. Therefore,
pore-water profiles show significant enrichments in trace metals especially from July to September. Finally, the trace metals
are released to the open water column via draining pore waters (esp. Mo, Mn, and V) and/or fixed in the sediment as sulphides
(Fe, Mo) and bound to organic matter (U). Non-conservative behaviour of Mo in oxygenated seawater, first observed in the investigation
area by Dellwig et al. (Geochim Cosmochim Acta 71:2745–2761, 2007a), was shown to be a recurrent phenomenon which is closely coupled to bacterial activity after the breakdown of algae blooms.
In addition to the postulated fixation of Mo in oxygen-depleted micro-zones of the aggregates or by freshly formed organic
matter, a direct removal of Mo from the water column by reduced sediment surfaces may also play an important role. 相似文献
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Maximilian Konzack Thomas McKetterick Tim Ophelders Maike Buchin Luca Giuggioli Jed Long 《International journal of geographical information science》2017,31(2):320-345
The analysis of interaction between movement trajectories is of interest for various domains when movement of multiple objects is concerned. Interaction often includes a delayed response, making it difficult to detect interaction with current methods that compare movement at specific time intervals. We propose analyses and visualizations, on a local and global scale, of delayed movement responses, where an action is followed by a reaction over time, on trajectories recorded simultaneously. We developed a novel approach to compute the global delay in subquadratic time using a fast Fourier transform (FFT). Central to our local analysis of delays is the computation of a matching between the trajectories in a so-called delay space. It encodes the similarities between all pairs of points of the trajectories. In the visualization, the edges of the matching are bundled into patches, such that shape and color of a patch help to encode changes in an interaction pattern. To evaluate our approach experimentally, we have implemented it as a prototype visual analytics tool and have applied the tool on three bidimensional data sets. For this we used various measures to compute the delay space, including the directional distance, a new similarity measure, which captures more complex interactions by combining directional and spatial characteristics. We compare matchings of various methods computing similarity between trajectories. We also compare various procedures to compute the matching in the delay space, specifically the Fréchet distance, dynamic time warping (DTW), and edit distance (ED). Finally, we demonstrate how to validate the consistency of pairwise matchings by computing matchings between more than two trajectories. 相似文献
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Witt Lilli M&#;ller Moritz J. Gr&#;schke Maike Post Vincent E. A. 《Hydrogeology Journal》2021,29(5):1733-1748
Hydrogeology Journal - Aquifer storage and recovery systems using multiple partially penetrating wells (MPPW-ASR) can form a viable solution to the problem of freshwater buoyancy when using... 相似文献
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Maike Didero Sonja Nebel Carmella Pfaffenbach 《Singapore journal of tropical geography》2019,40(3):361-386
Population growth, urban sprawl and a high degree of car dependency as well as slowly rising petrol prices contribute towards increasing challenges for everyday urban mobility in Muscat, Oman. Until now, only a few empirical studies have dealt with urban mobility in Oman. Therefore, this article draws mainly on our own empirical findings to answer the following questions: What do daily and weekly mobility patterns look like in Muscat? How do these practices differ depending on the social position of the household, i.e. their nationality, income and education? Which interdependent effects can be discerned between everyday mobility practices and the fragmented and segregated urban structures? Since our research questions focus on the interrelations between urban structures and individual mobility, we chose a mixed‐methods approach including methods derived both from social and spatial research. This article in particular draws on our quantitative survey covering 850 households and extensive mappings of three selected case study areas and secondary data analysis. 相似文献
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