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David L. Naftz Gregory T. Carling Cory Angeroth Michael Freeman Ryan Rowland Eddy Pazmiño 《Aquatic Geochemistry》2014,20(6):547-571
Density stratification in saline and hypersaline water bodies from throughout the world can have large impacts on the internal cycling and loading of salinity, nutrients, and trace elements. High temporal resolution hydroacoustic and physical/chemical data were collected at two sites in Great Salt Lake (GSL), a saline lake in the western USA, to understand how density stratification may influence salinity and mercury (Hg) distributions. The first study site was in a causeway breach where saline water from GSL exchanges with less saline water from a flow restricted bay. Near-surface-specific conductance values measured in water at the breach displayed a good relationship with both flow and wind direction. No diurnal variations in the concentration of dissolved (<0.45 μm) methylmercury (MeHg) were observed during the 24-h sampling period; however, the highest proportion of particulate Hgtotal and MeHg loadings was observed during periods of elevated salinity. The second study site was located on the bottom of GSL where movement of a high-salinity water layer, referred to as the deep brine layer (DBL), is restricted to a naturally occurring 1.5-km-wide “spillway” structure. During selected time periods in April/May, 2012, wind-induced flow reversals in a railroad causeway breach, separating Gunnison and Gilbert Bays, were coupled with high-velocity flow pulses (up to 55 cm/s) in the DBL at the spillway site. These flow pulses were likely driven by a pressure response of highly saline water from Gunnison Bay flowing into the north basin of Gilbert Bay. Short-term flow reversal events measured at the railroad causeway breach have the ability to move measurable amounts of salt and Hg from Gunnison Bay into the DBL. Future disturbance to the steady state conditions currently imposed by the railroad causeway infrastructure could result in changes to the existing chemical balance between Gunnison and Gilbert Bays. Monitoring instruments were installed at six additional sites in the DBL during October 2012 to assess impacts from any future modifications to the railroad causeway. 相似文献
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Glaciological investigations of the Upper Fremont Glacier in the Wind River Range of Wyoming were conducted during 1990–1991. The glaciological data will provide baseline information for monitoring future changes to the glacier and support ongoing research utilizing glacial-ice-core composition to reconstruct paleoenvironmental records. Ice thickness, determined by radio-echo sounding, ranged from 60 to 172 m in the upper half of the glacier. Radio-echo sounding of ice thickness at one point was confirmed by drilling 159.7 m to bedrock. The difference between radio-echo sounding depth and measured drilling depth was about 4 m. Annual ablation (including snow, firn, and ice) measured for the 1990–1991 period averaged about 0.93 m/a. Densification proceeds rapidly on Upper Fremont Glacier. Measured densities in the near-surface parts of the glacier ranged from 4.4 x 105 g/m3 at the surface to larger than 8.5 x 105 g/m3 at depths exceeding 14 m. Surface ice velocity and direction were monitored from July 1990 to August 1991. Ice velocity decreased in a downslope direction. The largest measured velocity was about 3.1 m/a and the smallest was 0.8 m/a. The yearly mean air temperature of the study site during the period from July 11, 1990 to July 10, 1991 was -6.9°. Borehole temperatures from 10-m depths are 0 ± 0.4°. The warmer borehole temperatures relative to the yearly mean air temperature may be caused by the latent heat of freezing, as meltwater from the surface percolates into the glacier and refreezes. [Key words: glaciers, Wyoming, Wind River Range, ice thickness, ablation rates.] 相似文献
3.
Ice-core samples from Upper Fremont Glacier (UFG), Wyoming, were used as proxy records for the chemical composition of atmospheric
deposition. Results of analysis of the ice-core samples for stable isotopes of nitrogen (δ15N, ) and sulfur (δ34S, ), as well as and deposition rates from the late-1940s thru the early-1990s, were used to enhance and extend existing National Atmospheric
Deposition Program/National Trends Network (NADP/NTN) data in western Wyoming. The most enriched δ34S value in the UFG ice-core samples coincided with snow deposited during the 1980 eruption of Mt. St. Helens, Washington.
The remaining δ34S values were similar to the isotopic composition of coal from southern Wyoming. The δ15N values in ice-core samples representing a similar period of snow deposition were negative, ranging from -5.9 to -3.2 ‰ and
all fall within the δ15N values expected from vehicle emissions. Ice-core nitrate and sulfate deposition data reflect the sharply increasing U.S.
emissions data from 1950 to the mid-1970s. 相似文献
4.
David L. Naftz Frank J. Millero Blair F. Jones W. Reed Green 《Aquatic Geochemistry》2011,17(6):809-820
Great Salt Lake (GSL) is one of the largest and most saline lakes in the world. In order to accurately model limnological
processes in GSL, hydrodynamic calculations require the precise estimation of water density (ρ) under a variety of environmental conditions. An equation of state was developed with water samples collected from GSL to
estimate density as a function of salinity and water temperature. The ρ of water samples from the south arm of GSL was measured as a function of temperature ranging from 278 to 323 degrees Kelvin
(oK) and conductivity salinities ranging from 23 to 182 g L−1 using an Anton Paar density meter. These results have been used to develop the following equation of state for GSL (σ = ± 0.32 kg m−3):
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r- r0 = 184.0 10 6 2 + 1.0 4 70 8*\textS - 1. 2 10 6 1*\textT + 3. 1 4 7 2 1 \textE - 4*\textS 2 + 0.00 1 9 9 \textT 2 - 0.00 1 1 2*\textS*\textT, \rho - \rho^{0} = { 184}.0 10 6 2 { } + { 1}.0 4 70 8*{\text{S}} - 1. 2 10 6 1*{\text{T }} + { 3}. 1 4 7 2 1 {\text{E}} - 4*{\text{S}}^{ 2} + \, 0.00 1 9 9 {\text{T}}^{ 2} - 0.00 1 1 2*{\text{S}}*{\text{T}}, 相似文献
5.
北秦岭西段冥古宙锆石(4.1～3.9Ga)年代学新进展 总被引：15，自引：13，他引：2
2007年王洪亮等报道在北秦岭西段火山岩中获得一粒年龄为4079±5Ma的冥古宙捕虏锆石。之后,对这一发现开展了深入的调查研究,我们除利用SHIMP技术方法对原4079Ma的锆石进行验证外,新获得了两粒~(207)Pb/~(206)Pb年龄为4007±29Ma和3908±45Ma捕获的变质成因锆石,表明早在4.0Ga已经有变质作用的发生,这或许说明在冥古宙时期地球已经具有相当规模和厚度的地壳。同时开展的岩石学研究表明,蕴含古老锆石的母岩属于火山碎屑熔岩类而不是火山熔岩。 相似文献
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Ximena Diaz William P. Johnson Diego Fernandez David L. Naftz 《Applied Geochemistry》2009,24(9):1653-1665
The characterization of trace elements in terms of their apportionment among dissolved, macromolecular, nano- and micro-particulate phases in the water column of the Great Salt Lake carries implications for the potential entry of toxins into the food web of the lake. Samples from the anoxic deep and oxic shallow brine layers of the lake were fractionated using asymmetric flow field-flow fractionation (AF4). The associated trace elements were measured via online collision cell inductively-coupled plasma mass spectrometry (CC-ICP-MS). Results showed that of the total (dissolved + particulate) trace element mass, the percent associated with particulates varied from negligible (e.g. Sb), to greater than 50% (e.g. Al, Fe, Pb). Elements such as Cu, Zn, Mn, Co, Au, Hg, and U were associated with nanoparticles, as well as being present as dissolved species. Particulate-associated trace elements were predominantly associated with particulates larger than 450 nm in size. Among the smaller nanoparticulates (<450 nm), some trace elements (Ni, Zn, Au and Pb) showed higher percent mass (associated with nanoparticles) in the 0.9–7.5 nm size range relative to the 10–250 nm size range. The apparent nanoparticle size distributions were similar between the two brine layers; whereas, important differences in elemental associations to nanoparticles were discerned between the two layers. Elements such as Zn, Cu, Pb and Mo showed increasing signal intensities from oxic shallow to anoxic deep brine, suggesting the formation of sulfide nanoparticles, although this may also reflect association with dissolved organic matter. Aluminum and Fe showed greatly increased concentration with depth and equivalent size distributions that differed from those of Zn, Cu, Pb and Mo. Other elements (e.g. Mn, Ni, and Co) showed no significant change in signal intensity with depth. Arsenic was associated with <2 nm nanoparticles, and showed no increase in concentration with depth, possibly indicating dissolved arsenite. Mercury was associated with <2 nm nanoparticles, and showed greatly increased concentration with depth, possibly indicating association with dissolved organic matter. 相似文献
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Kimberly R. Beisner Nicholas V. Paretti Fred D. Tillman David L. Naftz Donald J. Bills Katie Walton-Day Tanya J. Gallegos 《Hydrogeology Journal》2017,25(2):539-556
The processes that affect water chemistry as the water flows from recharge areas through breccia-pipe uranium deposits in the Grand Canyon region of the southwestern United States are not well understood. Pigeon Spring had elevated uranium in 1982 (44 μg/L), compared to other perched springs (2.7–18 μg/L), prior to mining operations at the nearby Pigeon Mine. Perched groundwater springs in an area around the Pigeon Mine were sampled between 2009 and 2015 and compared with material from the Pigeon Mine to better understand the geochemistry and hydrology of the area. Two general groups of perched groundwater springs were identified from this study; one group is characterized by calcium sulfate type water, low uranium activity ratio 234U/238U (UAR) values, and a mixture of water with some component of modern water, and the other group by calcium-magnesium sulfate type water, higher UAR values, and radiocarbon ages indicating recharge on the order of several thousand years ago. Multivariate statistical principal components analysis of Pigeon Mine and spring samples indicate Cu, Pb, As, Mn, and Cd concentrations distinguished mining-related leachates from perched groundwater springs. The groundwater potentiometric surface indicates that perched groundwater at Pigeon Mine would likely flow toward the northwest away from Pigeon Spring. The geochemical analysis of the water, sediment and rock samples collected from the Snake Gulch area indicate that the elevated uranium at Pigeon Spring is likely related to a natural source of uranium upgradient from the spring and not likely related to the Pigeon Mine. 相似文献
10.
James DL White 《Bulletin of Volcanology》1991,53(4):239-258
Remnants of an extensive maar-diatreme volcanic field are magnificently exposed at various depths of erosion in the Hopi Buttes volcanic field of northeastern Arizona. Field and petrographic studies of both the maar and diatreme elements of a selection of volcanoes within the field show that: (1) lower sections of the maar rim sequences are typically rich in sandy mudrock derived from the pre-eruptive Mio-Pliocene Bidahochi Formation, and the muddy Bidahochi sediment was soft and wet at the time of maar eruptions; (2) beds higher within the rims contain generally increased proportions of sandstone clasts from the Triassic Wingate Formation. In the diatremes, late-emplaced breccia has deeper-seated lithics than more marginal breccia emplaced earlier; and (3) many vents are topped by megacryst-enriched scoria and spatter, and deep-seated xenoliths are known only from upper diatreme and craterfilling tephra. These observations show that: (1) eruptions at Hopi Buttes involved interaction of magma with unconsolidated mudrock at shallow levels, and the phreatomagmatic processes that provided the bulk of the energy involved in the violent eruptions were driven by the interaction of magma and wet sediment; (2) the locus of explosive activity migrated downward as eruptions progressed; and (3) the closing stage of many eruptions was characterized by rapid magma rise and relative depletion of water. 相似文献
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