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Formation of Brominated Disinfection By-products after Chlorination of Water from Lake Constance Depending on Treatment Steps and Bromide Concentration The formation of halogenated disinfection by-products (DNP) (trihalomethanes (THM), haloacetic acids (HES), haloacetonitriles (HAN), haloketones (HKE) and chloropicrin (TCNM)) was studied after chlorination (0.5 mg/L) of raw water and drinking water from Lake Constance. The objectives of this study were to investigate the effect of bromide ion on the distribution of DNP-species resulting from chlorination and to draw up a bromide mass-balance. The treatment of water from Lake Constance with ozone decreased the formation of DNP about 35% and of total organic halogens (AOX) about 45%. This decline in DNP-formation is mainly due to the formation of chloroform, dichloro- and trichloroacetic acid. Though there is only a small amount of bromide (6.2 μg/L) in water from Lake Constance, about 32% of THM, 16% of HES, and 30% of HAN contained bromine after chlorination of treated water. The addition of bromide ion (up to 1 mg/L) shifted the DNP-composition to more brominated species. The distribution of the DNP-species depends on the initial molar bromide-to-chlorine ratio. A mathematic model showed the same pattern of DNP-species depending on the initial molar bromide-to-chlorine ratio that was observed experimentally in microstrained raw water and drinking water from Lake Constance. After chlorination of microstrained raw water, 27% of the bromide were incorporated in known DNP, 34% in unknown substances, and about 39% of bromide were not converted to organic bromine. After chlorination of treated water, only 16% of the bromide were incorporated in unknown substances, whereas 34% were found in known DNP. About 50% were found as bromide again. After addition of bromide (up to 25 μg/L) to ozonated and treated water from Lake Constance, between 60 and 72% of the bromide that had reacted after chlorination were found in analyzed low-molecular DNP. 相似文献
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Alcides Nobrega Sial Claudio Gaucher Marinho Alves da Silva Filho Valderez P. Ferreira Marcio M. Pimentel Luiz D. Lacerda Emmanoel V. Silva Filho Wilker Cezario 《Precambrian Research》2010
Two cap carbonates overlying glaciogenic diamictites crop out extensively in the eastern Vaza Barris Domain of the Sergipano Belt, northeastern Brazil. They are represented by carbonates of the Jacoca Formation, resting on top of diamictite of the Ribeiropolis Formation, and by the Olhos D’Agua Formation (carbonates, organic-rich towards the top), which overlies diamictite of the Palestina Formation. These two sequences were deformed and metamorphosed at sub-greenschist facies-conditions during the Brasiliano cycle (650–600 Ma). 相似文献
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