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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff 下载免费PDF全文
We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
2.
海岩的长篇小说《河流如血》再创出版高记录,但作家仍局限于特有的小说叙述模式,这部作品设能做到相应的创新。概言之,模式第一面是“刑侦+恋爱”;模式第二面是“财子+佳人”;模式第三面是“道德+法制”。文学创作需要不断创新,创新的过程也是对创作模式的不断突破过程。作家应该警惕的是,不要让模式成为创作的桎梏。 相似文献
3.
Tidal effects on temperature front in the Yellow Sea 总被引:5,自引:0,他引:5
Temperature front (TF) is one of the important features in the Yellow Sea, which forms in spring, thrives in summer, and fades
in autumn as thermocline declines. TF intensity ⋎S
T
⋎ is defined to describe the distribution of TF. Based on the MASNUM wave-tide-circulation coupled model, temperature distribution
in the Yellow Sea was simulated with and without tidal effects. Along 36°N, distribution of TF from the simulated results
are compared with the observations, and a quantitative analysis is introduced to evaluate the tidal effects on the forming
and maintaining processes of the TF. Tidal mixing and the circulation structure adapting to it are the main causes of the
TF.
Supported by the National Basic Research Program of China (No. G1999043809) and the National Science Foundation of China (No.
49736190). 相似文献
4.
5.
PALEOSOLSOFSANDYLANDSANDENVIRONMENTALCHANGESINTHEWESTERNPARTOFNORTHEASTPLAINOFCHINAWESTERNDURINGHOLOCENE¥QiuShanwen(裘善文)LiQus... 相似文献
6.
本文以爱黎-海斯卡宁均衡补偿假设模式为基础,利用圆模板编制了滇西北及邻区均衡重力异常图。分析了异常的基本特征与壳内构造的关系,并初步探讨了均衡重力异常和强震活动的相关性。 相似文献
7.
向文 《大地测量与地球动力学》1997,(2)
为了根据离散观测数据构制连续空间重力变化图像,分析和讨论了3种数值插值方法,计算结果表明多面函数方法插值精度最高。由于逐步回归分析筛选核函数中心点的计算繁琐,文中提出根据分形理论和Shannon取样定理来确定核函数中心点。对滇西试验场进行模拟试算,插值精度可达到4~5(10-8ms-2)。 相似文献
8.
In this paper, two factors — the redistribution of the density and the variation in the angular velocity of the Earth rotation, that affect the adopted value of the flattening for equidensity surface within the Earth, are discussed. The computational results show that the contribution of the redistribution of the density in the Earth interior (especially in the core) on the change of the flattening at the core-mantle boundary (CMB) is marginal, and that the calculated value of the flattening at the CMB can be in good agreement with the VLBI observed value so long as the fact that the angular velocity of the Earth rotation has undergone the tidal evolution is taken into account. As a result, this paper presents a set of recommended values of the dynamical parameters of the Earth (see Table III) for computing Earth's forced nutation series. 相似文献
9.
Profiles of spectral lines emitted from an accretion ring around an object with strong gravitational field should be affected by Doppler shift, gravitational redshift, and deflection of light. Taking these effects into account, precise line profile of a Keplerian ring around a Kerr black hole for a distant observer is obtained by solving the kinetic equation of photons. 相似文献
10.
VPN技术在浙江省气象网络中的应用 总被引:2,自引:0,他引:2
随着浙江省气象业务的不断发展,网络数据交换日益增多,同时更多基于网络的气象业务的增加,如网络视频会商、自动站数据传输等,使目前浙江省气象系统专线网络运行已达到极限,所以需要建立VPN网以对现有的网络作链路上的备份,而VPN的建立同时还可以实现移动办公,领导能在远程调用内网的资料进行远程决策服务和汇报工作。主要介绍VPN技术并叙述VPN技术在浙江省气象系统网络中的具体应用。 相似文献