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Vertical profiles of total sulfur and organic carbon have been measured in two deep-sea piston cores from the southwestern Japan Sea where sulfate reduction is proceeding within the sediments. The content of total sulfur, most of which is present as pyrite, increases gradually with increasing depth, showing several peaks. The amount of diagenetically deposited sulfide-sulfur is estimated using a steady-state model that considers vertical change in the diffusion coefficient. It is suggested that two-thirds to three-fourths of the observed total sulfur content has been deposited diagenetically. 相似文献
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We have developed an analytical treatment for the wave-induced response of a seabed with inhomogeneous permeability, by employing the boundary layer approximation. By assuming an exponential function for vertically distributed permeability, the inhomogeneous consolidation equation was formulated as Bessel's differential equation. Subsequently, we proposed some representative quantities for examining the effects of inhomogeneity of permeability. The main effects of inhomogeneity are that the boundary layer becomes thinner and the phase delay in the direction of depth becomes larger as the inhomogeneity becomes significant. In addition, it was shown that the boundary layer is properly evaluated by using the averaged permeability. 相似文献
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Norimichi Takenaka Tohru Daimon Akihiro Ueda Keiichi Sato Masaru Kitano Hiroshi Bandow Yasuaki Maeda 《Journal of Atmospheric Chemistry》1998,29(2):135-150
Nitrite oxidation in the tropospheric aqueous phase by freezing was evaluated by freezing a field sample. Nitrite oxidation by dissolved oxygen in the freezing process is much faster than by other oxidation processes, such as reactions with ozone, hydrogen peroxide or dissolved oxygen in an aqueous solution at pHs 3 to –6. At pH 4.5 and 25°C, the lifetime of nitrite in the aqueous phase is ca. 1 hr in oxidation by ozone (6×10-10 mol dm-3), ca. 10 hr in oxidation by H2O2 (2×10-4 mol dm-3), and 7.5 hr (Fischer and Warneck, 1996) in photodissociation at midday in summer. Under the same conditions at a temperature below 0°C, the lifetime of nitrite in the freezing process is estimated as ca. 2 sec when the droplets are frozen within a second. The reaction by freezing is affected by the presence of salts, such as NaCl or KCl, or orgnaic compounds, such as methanol or acetone. The results of freezing a field rain or fog sample showed that nitrite oxidation proceeds below pH 6, and the conversion ratio of nitrate from nitrite increases with decreasing pH. The oxidation of nitrite by freezing was also observed in freezing fog particles generated by an ultrasonic humidifier. The ratios of the concentrations of ions in the winter sample to those in the summer sample (or those in the fog sample) were almost the same values. However, the concentration of nitrite in the winter sample was lower than that estimated by the ratios of other ions. From the present study, it seems that the freezing process plays an important role in the nitrite sink process in the tropospheric aqueous phase. 相似文献
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This study investigates stem waves, propagating along a vertical wall, due to obliquely incident random waves through laboratory experiments and numerical simulations. Attention is paid to the difference or similarity between the stem waves due to periodic waves and random waves, the nonlinear and linear characteristics, and the effect of wave breaking on the evolution of stem waves. The following were found from this study: as the incident angle of waves become large or the nonlinearity of the incident waves become small, the significant stem wave height, normalized by the incident significant wave height, becomes large. This tendency is the same as that generated by the Stokes waves or cnoidal waves. However, regardless of the nonlinearity of incident waves, the width of stem waves is almost the same. This is a different point between the stem waves due to periodic and random waves. The wave breaking suppresses the growth of the stem waves. 相似文献
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The reversibility of the temperature effect on the chemical composition of interstitial waters of three deep-sea sediment samples was examined between 2 and 25°C for Cl, Na, K, Mg, Ca, Si, B, Mn and alkalinity. When the temperature of sediment samples was returned from 25°C to the initial value of 2°C, most chemical species gave nearly their initial concentrations. However, for alkalinity and in one case for magnesium, it took another three to four hours to reach their initial concentrations. 相似文献
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Vertical distributions of sulfate, hydrogen sulfide, and iron (II) concentrations in interstitial waters and of sulfur content in sediment have been studied in a sediment core (73 cm long) from a meromictic lake, Lake Suigetsu, which changed from fresh-water to brackish conditions in 1664 A.D. The diatom assemblage of the sediment has also been analyzed. A boundary between high (>1.5%) and low (<0.2%) sulfur contents is found at a depth of 52 cm in the core. In the high sulfur layer (above 52 cm), the maximum sulfur content is 6.8% at 35 to 37 cm. The diatom assemblage, however, indicates that the boundary between fresh-water and brackish sediments lies at 40 cm. The hydrogen sulfide and iron (II) profiles in the interstitial waters indicate a sink for these chemical species near a depth of 40 cm. The discrepancy between the chemically-defined boundary at 52 cm and the paleontologically-defined boundary at 40 cm seems to be due to the downward migration of hydrogen sulfide and deposition of iron sulfide after the lake became brackish. 相似文献
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Diagenetic deposition of manganese in sediment of a historically meromictic lake,Lake Suigetsu,Japan
Vertical profiles of manganese concentration in interstitial waters and of manganese and iron contents in five chemically-separated fractions of sediments have been studied in a sediment core (73 cm long) from a meromictic lake, Lake Suigetsu, which changed from freshwater to brackish conditions in 1664 A.D. The interstitial waters show a minimum manganese concentration of 0.13 ppm near a depth of 10 cm and a maximum of 26 ppm near 65 cm in the core. A predominant amount of manganese, up to 0.17%, is found in the hydrogen peroxide-soluble fraction of sediments in layers above a depth of 52 cm. It is suggested that the manganese is included in stable iron sulfides such as pyrite. Manganese, which diffuses upward from the lower layer, is thought to be deposited along with stable iron sulfide during diagenetic formation of the latter near a depth of 10 cm in the core. 相似文献
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To understand the behavior of manganese in diagenetic processes in sediments of an enclosed bay which is similar to those
of an estuary, chemical analyses have been carried out on both sediment and interstitial water of a core sample collected
from Tokyo Bay. The results suggest that redistribution of manganese takes place within the sediment as a result of the dissolution
of buried manganese oxides and hydroxides under reducing condition, the downward diffusion of Mn2+ through the interstitial water toward lower layers and then the precipitation of carbonate. The carbonate formed in the sediment
contains managanese carbonate probably as a solid solution between calcitic calcium carbonate and manganese carbonate. 相似文献
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Effects of deposit feeder Stichopus japonicus on algal bloom and organic matter contents of bottom sediments of the enclosed sea 总被引：4，自引：0，他引：4
Michio K Kengo K Yasunori K Hitoshi M Takayuki Y Hideaki Y Hiroshi S 《Marine pollution bulletin》2003,47(1-6):118-125
Algae growing in an enclosed sea may inhibit eutrophication because they absorb nutrients in the water. However, dead algae often cause anaerobic conditions in the water just above and on sediment after they are deposited on the bottom. We found that Stichopus japonicus inhibited the anaerobic processes coupling water sulfite production in sediment. The present study investigates whether S. japonicus inhibits algal flourish and influences sediment properties such as organic matter contents. Aquarium experiments were carried out at Komatsushima port in Tokushima Prefecture, western Japan. The aquaria used in the experiments were supplied with water directly from the adjacent sea (6 L/min), laid with sand of 10 cm depths, and lighted at 12 h intervals. Six aquaria each containing a sea cucumber from Komatsushima port and six aquaria without any were used in the experiments. Water temperature ranged between 9 and 15 degrees C during December 2000 and April 2001. Salinity ranged between 32 per thousand and 34 per thousand. Algae began to cover the bottom of the aquaria without S. japonicus after 2 weeks, whereas no growth was evident in the aquaria containing sea cucumbers. Chlorophyll a concentration in the surface sediment of the aquaria with S. japonicus (6.1+/-3.6 microg/g, mean S.D.+/-standard deviation) was significantly lower than that without it (60+/-17 microg/g, U-test, p<0.05). Phaeophytin concentration in the surface sediment of the aquaria with S. japonicus (0.9+/-0.09 microg/g) was also significantly lower than that without it (4.5+/-1.0 microg/g, U-test, p<0.05). TOC concentration in the surface sediment of the aquaria with S. japonicus (2.6+/-1.3 microg/g) was slightly lower than that without it (4.0+/-1.2 microg/g). These results showed that algal biomass and organic matter concentration of the bottom were decreased in the presence of S. japonicus. Therefore, S. japonicus inhibits algal bloom and decrease the contents of organic matter deposited on the bottom of enclosed sea areas. 相似文献