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Romain de Mesmay Pierre Metzger Vincent Grossi Sylvie Derenne 《Organic Geochemistry》2008,39(7):879-893
A mixture of C33–C37 botryococcenes and partially reduced derivatives was isolated from ca. 32,000 year old sediment from Lake Masoko, a freshwater crater lake in the Rungwe Range area (Tanzania). Botryococcenes and derivatives accounted for 246 μg/g dry sediment and for >92% of the hydrocarbon fraction; 1D and 2D nuclear magnetic resonance spectroscopy (NMR) and mass spectrometry allowed the structure of the dominant botryococcene (43% of hydrocarbon fraction) to be established, after purification using high performance liquid chromatography (HPLC). The compound is a novel tetraunsaturated dicyclic C34 botryococcene and is named C34 masokocene. Overall, the structures of six other novel botryococcenes and four partially reduced derivatives were tentatively assigned. The structures of the new biomarkers, three dicyclic C34–C36 botryococcenes (or masokocenes) and seven monocyclic C34–C37 analogues are discussed along with their biosynthetic relationship. The high abundance of such polyunsaturated compounds preserved in 32,000 year old sediment from the lake indicates an aquatic ecosystem dominated at the time by the green alga Botryococcus braunii, as well very good preservation of the organic matter. 相似文献
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Rivers, chemical weathering and Earth's climate 总被引:4,自引:0,他引:4
Bernard Dupr Cline Dessert Priscia Oliva Yves Goddris Jrme Viers Louis Franois Romain Millot Jrme Gaillardet 《Comptes Rendus Geoscience》2003,335(16):1141-1160
We detail the results of recent studies describing and quantifying the large-scale chemical weathering of the main types of continental silicate rocks: granites and basalts. These studies aim at establishing chemical weathering laws for these two lithologies, describing the dependence of chemical weathering on environmental parameters, such as climate and mechanical erosion. As shown within this contribution, such mathematical laws are of primary importance for numerical models calculating the evolution of the partial pressure of atmospheric CO2 and the Earth climate at geological timescales. The major results can be summarized as follow: (1) weathering of continental basaltic lithologies accounts for about 30% of the total consumption of atmospheric CO2 through weathering of continental silicate rocks. This is related to their high weatherability (about eight times greater than the granite weatherability); (2) a simple weathering law has been established for basaltic lithologies, giving the consumption of atmospheric CO2 as a function of regional continental runoff, and mean annual regional temperature; (3) no such simple weathering law can be proposed for granitic lithologies, since the effect of temperature can only be identified for regions displaying high continental runoff; (4) a general law relating mechanical erosion and chemical weathering has been validated on small and large catchments. The consequences of these major advances on the climatic evolution of the Earth are discussed. Particularly, the impacts of the onset of the Deccan trapps and the Himalayan orogeny on the global carbon cycle are reinvestigated. To cite this article: B. Dupré et al., C. R. Geoscience 335 (2003). 相似文献
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Adombi Adoubi Vincent De Paul Chesnaux Romain Boucher Marie-Amlie 《Hydrogeology Journal》2021,29(8):2671-2683
Hydrogeology Journal - Thanks to recent technological advances, hydrogeologists now have access to large amounts of data acquired in real time. Processing these data using traditional modelling... 相似文献
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ABSTRACT. Beekeeping has the potential to supplement incomes in rural southern Africa. In light of regional economic constraints, self-reliance strategies that draw on local knowledge and skills take on a renewed importance. We consider the advantages and disadvantages of beekeeping and examine appropriate forms of development support. A short case study from Zimbabwe illustrates these issues. 相似文献