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Unexpected chaotic features are found in time series of arrival time intervals of successive air showers with (E > 3 × 1014 eV). Over 99 % of air shower arrival time intervals obey the Poisson distribution law representing stochastic behaviors, but occasionally there are air showers showing real chaotic behaviors as distinguished from both random and colored noises. With two systems of the Kinki university installations, we found 13 cases showing chaotic time series in 3.36 yr with the system-1 and the 1.37 yr with the system-2. Five out of 10 chaotic air showers of the Kinki installation are detected during the same time zone also by the Osaka City university installation which is at 115 km distance from the Kinki one. In a remarkable example of September 19, 1991, the correlation dimension was observed to have dropped from about 4 to the minimum of 1.3 and recovered smoothly in about 38 h. The chaos structure in this case is detected in nearly the same time zone at the Ohya station of the Institute for Cosmic Ray Research, University of Tokyo, which is separated from the Kinki one by 460 km. Formation of chaos structure due to energetic cosmic ray dust particles is suggested. Progress of cosmic ray physics may be expected with the study of air showers marked with chaos.  相似文献   
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