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D. Arcay  M.-P. Doin  E. Tric  R. Bousquet   《Tectonophysics》2007,441(1-4):27-45
At continental subduction initiation, the continental crust buoyancy may induce, first, a convergence slowdown, and second, a compressive stress increase that could lead to the forearc lithosphere rupture. Both processes could influence the slab surface P–T conditions, favoring on one side crust partial melting or on the opposite the formation of ultra-high pressure/low temperature (UHP-LT) mineral. We quantify these two effects by performing numerical simulations of subduction. Water transfers are computed as a function of slab dehydration/overlying mantle hydration reactions, and a strength decrease is imposed for hydrated mantle rocks. The model starts with an old oceanic plate ( 100 Ma) subducting for 145.5 Myr with a 5 cm/yr convergence rate. The arc lithosphere is thermally thinned between 100 km and 310 km away from the trench, due to small-scale convection occuring in the water-saturated mantle wedge. We test the influence of convergence slowdown by carrying on subduction with a decreased convergence rate (≤ 2 cm/yr). Surprisingly, the subduction slowdown yields not only a strong slab warming at great depth (> 80 km), but also a significant cooling of the forearc lithosphere at shallower depth. The convergence slowdown increases the subducted crust temperature at 90 km depth to 705 ± 62 °C, depending on the convergence rate reduction, and might thus favor the oceanic crust partial melting in presence of water. For subduction velocities ≤ 1 cm/yr, slab breakoff is triggered 20–32 Myr after slowdown onset, due to a drastic slab thermal weakening in the vicinity of the interplate plane base. At last, the rupture of the weakened forearc is simulated by imposing in the thinnest part of the overlying lithosphere a dipping weakness plane. For convergence with rates ≥ 1 cm/yr, the thinned forearc first shortens, then starts subducting along the slab surface. The forearc lithosphere subduction stops the slab surface warming by hot asthenosphere corner flow, and decreases in a first stage the slab surface temperature to 630 ± 20 °C at 80 km depth, in agreement with P–T range inferred from natural records of UHP-LT metamorphism. The subducted crust temperature is further reduced to 405 ± 10 °C for the crust directly buried below the subducting forearc. Such a cold thermal state at great depth has never been sampled in collision zones, suggesting that forearc subduction might not be always required to explain UHP-LT metamorphsim.  相似文献   
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An integrated study combining facies analysis, multiple group biostratigraphy, identification of depositional sequences and mapping has been conducted on the Miocene Molasse Basin of the external Alps (southeastern France). The filling of the basin is described as resulting from a succession of fluvial incisions subsequently filled during marine transgressions. The major incision is dated as Latest Burdigalian and the major transgression as Langhian. This revised interpretation of the Miocene physiographic evolution of the Molasse Basin implies a re-examination of previous stratigraphic correlations within the basin. To cite this article: D. Besson et al., C. R. Geoscience 337 (2005).  相似文献   
5.
Graphitic cherts are interbedded within terrigenous sediments in the Cadomian orogenic belt of end-Proterozoic age. In the Armorican Massif (NW France), the graphitic cherts are of two types: massive cherts essentially composed of quartz (SiO2 > 96%) and with rare sedimentary structures; laminated cherts containing up to 3·4% Al2O3 and 92–98% SiO2. Sedimentary structures observed in the laminated cherts are indicative of a restricted hypersaline tidal or supratidal environment. The origins of both types of chert are to be found in the diagenetic processes of silification of terrigenous and mixed terrigenous-evaporitic facies. These processes, which could be mediated by the presence of organic matter, were controlled by the migration of the freshwater/saltwater mixing zone during periods of relative sea-level change. The proposed diagenetic origin for the cherts places a number of constraints on their use in the establishment of stratigraphic correlations.  相似文献   
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Based on a decade of research on cloud processes, a new version of the LMDZ atmospheric general circulation model has been developed that corresponds to a complete recasting of the parameterization of turbulence, convection and clouds. This LMDZ5B version includes a mass-flux representation of the thermal plumes or rolls of the convective boundary layer, coupled to a bi-Gaussian statistical cloud scheme, as well as a parameterization of the cold pools generated below cumulonimbus by re-evaporation of convective precipitation. The triggering and closure of deep convection are now controlled by lifting processes in the sub-cloud layer. An available lifting energy and lifting power are provided both by the thermal plumes and by the spread of cold pools. The individual parameterizations were carefully validated against the results of explicit high resolution simulations. Here we present the work done to go from those new concepts and developments to a full 3D atmospheric model, used in particular for climate change projections with the IPSL-CM5B coupled model. Based on a series of sensitivity experiments, we document the differences with the previous LMDZ5A version distinguishing the role of parameterization changes from that of model tuning. Improvements found previously in single-column simulations of case studies are confirmed in the 3D model: (1) the convective boundary layer and cumulus clouds are better represented and (2) the diurnal cycle of convective rainfall over continents is delayed by several hours, solving a longstanding problem in climate modeling. The variability of tropical rainfall is also larger in LMDZ5B at intraseasonal time-scales. Significant biases of the LMDZ5A model however remain, or are even sometimes amplified. The paper emphasizes the importance of parameterization improvements and model tuning in the frame of climate change studies as well as the new paradigm that represents the improvement of 3D climate models under the control of single-column case studies simulations.  相似文献   
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Recently, a new conceptual framework for deep convection scheme triggering and closure has been developed and implemented in the LMDZ5B general circulation model, based on the idea that deep convection is controlled by sub-cloud lifting processes. Such processes include boundary-layer thermals and evaporatively-driven cold pools (wakes), which provide an available lifting energy that is compared to the convective inhibition to trigger deep convection, and an available lifting power (ALP) at cloud base, which is used to compute the convective mass flux assuming the updraft vertical velocity at the level of free convection. While the ALP closure was shown to delay the local hour of maximum precipitation over land in better agreement with observations, it results in an underestimation of the convection intensity over the tropical ocean both in the 1D and 3D configurations of the model. The specification of the updraft vertical velocity at the level of free convection appears to be a key aspect of the closure formulation, as it is weaker over tropical ocean than over land and weaker in moist mid-latitudes than semi-arid regions. We propose a formulation making this velocity increase with the level of free convection, so that the ALP closure is adapted to various environments. Cloud-resolving model simulations of observed oceanic and continental case studies are used to evaluate the representation of lifting processes and test the assumptions at the basis of the ALP closure formulation. Results favor closures based on the lifting power of sub-grid sub-cloud processes rather than those involving quasi-equilibrium with the large-scale environment. The new version of the model including boundary-layer thermals and cold pools coupled together with the deep convection scheme via the ALP closure significantly improves the representation of various observed case studies in 1D mode. It also substantially modifies precipitation patterns in the full 3D version of the model, including seasonal means, diurnal cycle and intraseasonal variability.  相似文献   
8.
The Comblanchien limestone is a well-known building stone that deserves a quantitative characterization in order to be able to certify its origin. We compare petrographical and geochemical characteristics of limestones commercialized under the name of Comblanchien to those of one of their competitors (VATC, a Portuguese coated grain-bearing limestone). From macroscopic and microscopic observations, the distinction is somehow difficult but the coated grain-bearing Comblanchien samples have δ13C values (from +1.75 to +2.25‰) different from those of the VATC sample (negative δ13C value). As an example of application of these results, three samples from a building site near Paris are also studied in order to verify their provenance. We conclude that they do not come from quarries from the Comblanchien area, but likely from Portugal. The study shows that a detailed analysis of building limestones may provide a robust tool for discriminating between currently mined stones of different provenances, and thus open the possibility to attach to a given limestone a fingerprint, an identity card, and if required a commercial label.  相似文献   
9.
In tobacco plants, elimination of Zn and Cd via the production of Ca-containing grains at the top of leaf hairs, called trichomes, is a potent detoxification mechanism. This study examines how Cd is incorporated in these biominerals, and how calcium growth supplement modifies their nature. Scanning electron microscopy coupled with energy dispersive X-ray microanalysis (SEM-EDX), microfocused X-ray diffraction (μ-XRD), and microfocused X-ray absorption near edge structure (μ-XANES) spectroscopy were used to image the morphology of the grains, identify the crystallized mineral phases, and speciate Cd, respectively. The mineralogy of the grains and chemical form of Cd varied with the amount of Ca. When tobacco plants were grown in a nutrient solution containing 25 μM Cd and low Ca supplement (Ca/Cd = 11 mol ratio), most of the grains were oblong-shaped and low-Cd-substituted calcite. When exposed to the same amount of Cd and high Ca supplement (Ca/Cd = 131 mol ratio), grains were more abundant and diverse in compositions, and in total more Cd was eliminated. Most grains in the high Ca/Cd experiment were round-shaped and composed predominantly of Cd-substituted vaterite, a usually metastable calcium carbonate polymorph, and subordinate calcite. Calcium oxalate and a Ca amorphous phase were detected occasionally in the two treatments, but were devoid of Cd. The biomineralization of cadmium and implications of results for Cd exposure of smokers and phytoremediation are discussed.  相似文献   
10.
Dredging and disposal of sediments onto agricultural soils is a common practice in industrial and urban areas that can be hazardous to the environment when the sediments contain heavy metals. This chemical hazard can be assessed by evaluating the mobility and speciation of metals after sediment deposition. In this study, the speciation of Zn in the coarse (500 to 2000 μm) and fine (<2 μm) fractions of a contaminated sediment dredged from a ship canal in northern France and deposited on an agricultural soil was determined by physical analytical techniques on raw and chemically treated samples. Zn partitioning between coexisting mineral phases and its chemical associations were first determined by micro-particle-induced X-ray emission and micro-synchrotron-based X-ray radiation fluorescence. Zn-containing mineral species were then identified by X-ray diffraction and powder and polarized extended X-ray absorption fine structure spectroscopy (EXAFS). The number, nature, and proportion of Zn species were obtained by a coupled principal component analysis (PCA) and least squares fitting (LSF) procedure, applied herein for the first time to qualitatively (number and nature of species) and quantitatively (relative proportion of species) speciate a metal in a natural system.The coarse fraction consists of slag grains originating from nearby Zn smelters. In this fraction, Zn is primarily present as sphalerite (ZnS) and to a lesser extent as willemite (Zn2SiO4), Zn-containing ferric (oxyhydr)oxides, and zincite (ZnO). In the fine fraction, ZnS and Zn-containing Fe (oxyhydr)oxides are the major forms, and Zn-containing phyllosilicate is the minor species. Weathering of ZnS, Zn2SiO4, and ZnO under oxidizing conditions after the sediment disposal accounts for the uptake of Zn by Fe (oxyhydr)oxides and phyllosilicates. Two geochemical processes can explain the retention of Zn by secondary minerals: uptake on preexisting minerals and precipitation with dissolved Fe and Si. The second process likely occurs because dissolved Zn and Si are supersaturated with respect to Zn phyllosilicate. EXAFS spectroscopy, in combination with PCA and LSF, is shown to be a meaningful approach to quantitatively determining the speciation of trace elements in sediments and soils.  相似文献   
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