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1.
M.D. Morrison 《Planetary and Space Science》1985,33(1):135-139
Laboratory measurements of the Å (3s' 3D° → 2p41D, 3s' 3D° → 2p43P) branching ratio have been made with a value of 1.5 × 10t-4 indicated. This value makes the branching transition at 1173 Å an order of magnitude stronger than the branch at 7990 Å (3s' 3D° → 3p 3P). The 1173 Å branching loss is still too weak a loss process for multiply scattered 989 Å photons to resolve the 989 Å intensity problem in the dayglow. 相似文献
2.
John Hardy Steven Kiesser Liam Antrim Alan Stubin Richard Kocan John Strand 《Marine environmental research》1987,23(4)
The sea surface is an important habitat for the developmental stages (eggs and larvae) of many fish and invertebrates; it is also a concentration point for anthropogenic contaminants entering the sea. Studies were conducted to determine the extent to which the sea surface of Puget Sound was toxic to the early life history stages of fish. Three urban bays with suspected contamination, a rural reference bay, and a Central Sound site were compared. Surface-dwelling eggs and organisms (zooneuston) were collected with a surface-skimming neuston net and their densities enumerated. Sand sole (Psettichthys melanostictus) embryos were exposed in the field and laboratory to the sea-surface microlayer. To develop a useful year-round approach to monitoring sea-surface toxicity, larval development of anchovies, kelp bass, and sea urchins was also evaluated as an indication of sea-surface microlayer toxicity.During the spawning season (February and March), urban boys in Puget Sound had lower concentrations of sand sole eggs and neustonic organisms on the sea surface than did the rural bayor Central Sound reference sites. Compared to the reference sites, laboratory exposure to surface microlayer samples collected from urban bay sites generally resulted in more chromsomal aberrations in developing sole embryos, reduced hatching success of sole larvae, and reduced growth in trout cell cultures. In situ hatching success of sole eggs was reduced by half or more in urban bays compared to reference sites.Toxicity was associated with visible surface slicks and, in urban bays, increased with increasing surface pressure (dynes cm−1). Results to be reported separately (Part II) indicate that toxicity is strongly correlated with the presence of high concentrations of polycyclic aromatic hydrocarbons and metals in the sea-surface microlayer. The toxicity of SMIC samples was similar when evaluated by sole, anchovy, kelp bass, or sea urchin tests. A sea-surface monitoring program could use sea urchin embryos to evaluate site-specific sea-surface toxicity throughout the year. 相似文献
3.
4.
Jeffrey N. Cross John T. Hardy Jo Ellen Hose G.Patrick Hershelman Liam D. Antrim Richard W. Gossett Eric A. Crecelius 《Marine environmental research》1987,23(4)
Sea-surface microlayer samples were collected from six nearshore areas receiving different amounts of anthropogenic inputs. The samples were analyzed for selected trace metals, chlorinated hydrocarbons, and polycyclic aromatic hydrocarbons. The relative toxicities of the samples were determined with fish embryo bioassays.Contaminant concentrations generally increased from offshore to the inshore stations. Contaminant concentrations were several orders of magnitude higher in microlayer samples from the highly industrialized Los Angeles and Long Beach harbors compared to samples from a site 15km offshore. Microlayer samples from the inshore stations were significantly more toxic, and induced significantly more developmental abnormalities and chromosome aberrations, than samples from the offshore stations. 相似文献
5.
Aquatic surface microlayer contamination in chesapeake bay 总被引:1,自引:0,他引:1
John T. Hardy Eric A. Crecelius Liam D. Antrim Steven L. Kiesser Virginia L. Broadhurst 《Marine Chemistry》1990,28(4)
The aquatic surface microlayer (SMIC), 50 μm thick, serves as a concentration point for metal and organic contaminants that have low water solubility or are associated with floatable particles. Also, the eggs and larvae of many fish and shellfish species float on, or come in contact with, the water surface throughout their early development. The objectives of this study were (1) to determine the present degree of aquatic surface microlayer pollution at selected sites in Chesapeake Bay, and (2) to provide a preliminary evaluation of sources contributing to any observed contamination.Twelve stations located in urban bays, major rivers, and the north central bay were sampled three times, each at 5-day intervals during May 1986. Samples of 1.4–4.1 each were collected from the upper 30–60-μm water surface (surface microlayer, SMIC) using a Teflon-coated rotating drum microlayer sampler. One sample of subsurface water was collected in the central bay.At all stations, concentrations of metals, alkanes, and aromatic hydrocarbons in the SMIC were high compared with one bulk-water sample and with typical concentrations in water of Chesapeake Bay and elsewhere. SMIC contamination varied greatly among the three sampling times, but high mean contaminant levels (total polycyclic aromatic hydrocarbons, 1.9–6.2 μg 1−1; Pb, 4.9–24 μg 1−1; Cu, 4–16 μg 1−1; and Zn, 34–59 μg 1−1) were found at the upper Potomac and northern bay sites. Three separate areas were identified on the basis of relative concentrations of different aromatic hydrocarbons in SMIC samples - the northern bay, the Potomac River, and the cleaner southern and eastern portions of the sampling area.Suspected sources of surface contamination include gasoline and diesel fuel combustion, coal combustion, and petroleum product releases. Concentrations of metals and hydrocarbons, at approximately half the stations sampled, are sufficient to pose a threat to the reproductive stages of some fish and shellfish. Sampling and analysis of the surface microlayer provides a sensitive tool for source identification and monitoring of potentially harmful aquatic pollution. 相似文献
6.
The surface compositions of 110 asteroids are analyzed from statistically representative data sets of polarimetry as a function of phase angle, broad-band radiometry near 10 and 20 μm, and visible and near-infrared spectrophotometry. A comparison of albedos and diameters determined by polarimetry and radiometry shows that a modest upward revision of the radiometric albedo scale is needed and that a single law relating the slope of the polarization-phase curve to geometric albedo may not hold for very dark asteroids. We present reliable adopted albedos and diameters for 56 objects. Roughdi ameters for 52 additional objects are obtained from spectrophotometry using a correlation between albedo and color. Corrections for sampling bias permit investigation of asteroid compositions as a function of diameter, orbit, and other parameters.More than 90% of the minor planets fall into two broad compositional groups, defined by several optical parameters, designated by the symbols C and S. Comparisons with meteorite spectral albedo curves suggest that the two groups are compositionally similar to carbonaceous and stony-metallic meteorites, respectively. C-type asteroids predominate in the belt, especially in the outer half. An unusual distribution of compositions is found between 2.77 and 3.0 AU. Many S-type objects have diameters of 100–200 km; C-type objects are much more common at both larger and smaller sizes. Vesta is unique, being apparently the only differentiated asteroid remaining intact in the belt. The largest C-type objects are compositionally distinct from smaller ones and possibly are metamorphosed. We sketch some implications for meteoritics and for the early history of the solar system and point to the need for further systematic sampling of smaller and fainter objects by these three observational techniques. 相似文献
7.
Material is ejected from impact craters in ballastic trajectories; it impacts first near the crater rim and then at progressively greater ranges. Ejecta from craters smaller than approximately 1 km is laid predominantly on top of the surrounding surface. With increasing crater size, however, more and more surrounding surface will be penetrated by secondary cratering action and these preexisting materials will be mixed with primary crater ejecta. Ejecta from large craters and especially basin forming events not only excavate preexisting, local materials, but also are capable of moving large amounts of material away from the crater. Thus mixing and lateral transport give rise to continuous deposits that contain materials from within and outside the primary crater. As a consequence ejecta of basins and large highland craters have eroded and mixed highland materials throughout geologic time and deposited them in depressions inside and between older crater structures.Because lunar mare surfaces contain few large craters, the mare regolith is built up by successive layers of predominantly primary ejecta. In contrast, the lunar highlands are dominated by the effects of large scale craters formed early in lunar history. These effects lead to thick fragmental deposits which are a mixture of primary crater material and local components. These deposits may also properly be named regolith though the term has been traditionally applied only to the relatively thin fine grained surficial deposit on mare and highland terranes generated during the past few billion year. We believe that the surficial highland regolith - generated over long periods of time - rests on massive fragmental units that have been produced during the early lunar history. 相似文献
8.
Gerold Morrison Edward T. Sherwood Richard Boler Joe Barron 《Estuaries and Coasts》2006,29(6):926-931
In the Tampa Bay region of Florida, extreme levels of annual and seasonal rainfall are often associated with tropical cyclones and strong El Niño episodes. We used stepwise multiple regression models to describe associations between annual and seasonal rainfall levels and annual, bay-segment mean water clarity (as Secchi depth [m]), chlorophylla (μg I?1), color (pcu), and turbidity (ntu) over a 20-yr period (1985–2004) during which estimated nutrient loadings have been dominated by non-point sources. For most bay segments, variations in annual mean water clarity were associated with variations in chlorophylla concentrations, which were associated in turn with annual or seasonal rainfall. In two bay segments these associations with annual rainfall were superimposed on significant long-term declining trends in chlorophylla. Color was significantly associated with annual rainfall in all bay segments, and in one segment variations in color were the best predictors of variations in water clarity. Turbidity showed a declining trend over time in all bay segments and no association with annual rainfall, and was significantly associated with variations in water clarity in only one bay segment. While chlorophylla, color, and turbidity a affected water clarity to varying degrees, the effects of extreme rainfall events (El Niño events in 1998 and 2003, and multiple tropical cyclone events in 2004) on water clarity were relatively short-lived, persisting for periods of months rather than years. During the 20-yr period addressed in these analyses, declining temporal trends in chlorophylla and turbidity, produced in part by a long-term watershed management program that has focused on curtailing annual loadings of nitrogen and other pollutants, may have helped to prevent the bay as a whole from responding more adversely to the high rainfall periods that occurred in 1998 and 2003–2004. 相似文献
9.
The Archean Shawmere anorthosite lies within the granulite facies portion of the Kapuskasing Structural Zone (KSZ), Ontario,
and is crosscut by numerous linear alteration veins containing calcite + quartz ± dolomite ± zoisite ± clinozoisite ± margarite ±paragonite ± chlorite.
These veins roughly parallel the trend of the Ivanhoe Lake Cataclastic Zone. Equilibria involving clinozoisite + margarite + quartz ± calcite
± plagioclase show that the vein minerals were stable at T < 600 °C, XCO2 < 0.4 at P ≈ 6 kbar. The stabilities of margarite and paragonite in equilibrium with quartz are also consistent with T < 600 °C and XCO2 < 0.4 at 6 kbar. Additional assemblages consisting of calcite + clinochlore + quartz + talc + margarite indicate T < 500 °C with XCO2 > 0.9. Thus, vein formation, while clearly retrograde, spanned a range of temperatures, and fluid compositions evolved from
H2O-rich to CO2-rich. The calcite in the retrograde veins has δ18O values that range from 8.4 to 11.2‰ (average = +9.7 ± 0.9‰) and δ13C values that range from −3.9 to −1.6‰ (average = −3.1 ± 0.6‰). These values indicate that the fluids from which calcite precipitated
underwent extensive exchange with the anorthosite and other crustal lithologies. The fluids may have been initially derived
either from devolatilization of metamorphic rocks or crystallization of igneous rocks in the adjacent Abitibi subprovince.
Vein quartz contains CO2-rich fluid inclusions (final melting T = −57.0 to −58.7 °C) that range in size from 5 to 17 μm. Measured homogenization temperatures (T h) range from −44.0 to 14.5 °C, however for most inclusions (46 of S1), T h = −44.0 to −21.1 °C (ρCO2 ≈ 1.13 to 1.05 g/cm3). At 400 to 600 °C, these densities correspond to pressures of 3.5 to 7 kbar, which is the best estimate of pressures of
vein formation. It has been argued that some high density CO2-rich fluid inclusions found in the KSZ were formed during peak metamorphism and thus document the presence of a CO2-rich fluid during peak granulite facies metamorphism (Rudnick et al. 1984). The association of high density CO2-rich fluid inclusions with clearly retrograde veins documents the formation of similar composition and density inclusions
after the peak of metamorphism. Thus, the coincidence of entrapment pressures calculated from fluid inclusion density measurements
with peak metamorphic pressures alone should not be considered strong evidence for peak metamorphic inclusion entrapment.
All fluid inclusion results are consistent with an initially semi-isobaric retrograde P–T path.
Received: 2 April 1996 / Accepted: 15 November 1996 相似文献
10.
Fred Worrall Ross Morrison Chris Evans Joerg Kaduk Susan Page Alex Cumming Mark Rayment Nicholas Kettridge 《水文研究》2021,35(12):e14431
Whilst all ecosystems must obey the second law of thermodynamics, these physical bounds and controls on ecosystem evolution and development are largely ignored across the ecohydrological literature. To unravel the importance of these underlying restraints on ecosystem form and function, and their power to inform our scientific understanding, we have calculated the entropy budget of a range of peat ecosystems. We hypothesize that less disturbed peatlands are ‘near equilibrium’ with respect to the second law of thermodynamics and thus respond to change by minimizing entropy production. This ‘near equilibrium’ state is best achieved by limiting evaporative losses. Alternatively, peatlands ‘far-from-equilibrium’ respond to a change in energy inputs by maximizing entropy production which is best achieved by increasing evapotranspiration. To test these alternatives this study examined the energy balance time series from seven peatlands across a disturbance gradient. We estimate the entropy budgets for each and determine how a change in net radiation (ΔRn) was transferred to a change in latent heat flux (ΔλE). The study showed that: (i) The transfer of net radiation to latent heat differed significantly between peatlands. One group transferred up to 64% of the change in net radiation to a change in latent heat flux, while the second transferred as little as 27%. (ii) Sites that transferred the most energy to latent heat flux were those that produced the greatest entropy. The study shows that an ecosystem could be ‘near equilibrium’ rather than ‘far from equilibrium’. 相似文献