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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff
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We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
2.
自从在活动星系核NGC4945的视线方向上发现第一个河外H2O超脉泽源以来,迄今为止已发现了19个河外H2O超脉泽源,对与活动星系核成协和河外H2O超脉泽源及分子谱线的观测和研究是探测和研究活动星系核核区中央源,拱核气体和尘埃环性质的非常有效的工具,主要评述对河外H2O超脉泽源及与其相关分子谱线的搜索,观测和理论研究现状。 相似文献
3.
ZHANGPing-yu MAYan-ji YUZhen-han 《中国地理科学(英文版)》2002,12(4):315-320
Manzhouli is the largest land port city on the Sino-Russia border, transit cargo through the land port amount-ed to 5.95 million tons, transit tourists were 304 500 in 2000. It stands at the joint place of China, Mongolia and Russi-a, faces to Siberia area of Russia, receives direct support from the Northeast China and Bohai Sea Rim Area, and possess-es priorities in geographical location, land port infrastructure, water resources, coal resources, tourist resources andgreat potentiality in economic cooperation with Russia. The future urban function is a key port on the First Eurasia Continen-tal Bridge. Manzhouli Port will keep its first place between China and Russia land transport, and it is forecasted that thetransit amount through Manzhouli Port will go up to 10 million tons in 2005 and 20 million tons in 2010. It will be construct-ed to be a trade center of the peripheral area extending to Russia and Mongolia, a key export-oriented processing industri-al zone supported by industries such as export processing industries, export agriculture, trade services, technology trad-ing and the other service industries. It keeps being a well-known touring city for trade, shopping, sightseeing, vocation,local food, recreation and cultural events. To build Manzhouli Export Processing Industry Zone will improve city econom-ic structure, and the main sectors are organic food processing, livestock products processing, garment and furniture indus-try. Moreover, Manzhouli Export Processing Industry Zone will eventually be upgraded to be a border free trade zone.The city functional transition will inevitably affect urban spatial restructure and its expansion. The city space transforma-tion will develop as such: one development axis of No. 301 highway paralleling with Bin - Zhou(Harbin - Manzhouli) rail-way which cuts through central part of Manzhouli City, and links Zhalainuocr District with central city; three urban unitsincluding central city, Zhalainuocr District and Manzhouli Interchange Trade Zone; cohesion with Aoerjin and Cuogangpastures; regional dual-nuclei structure of Hailaer City and Manhzouli City; and the Manzhouli-Zabaykalsk Free TradeZone. 相似文献
4.
Grid method is employed for sampling covering soil at the test field,which is reclamation area filled by coal mining wastes for cropland in the Fushun coal mine,Liaoning Province,the Northeast China.The soil samples are taken at different locations,including three kinds of covering soil,three different depths of soil layers and four different covering ages of covering soil.The spatial-temporal variation of heavy metal element content in reclamation soil is stud-ied.The results indicate that the content of heavy metal elements is decreasing year after year,the determinant reason why the content of heavy metal elements at 60cm depth layer is higher than that at 30cm depth layer and surface is fertiliz-er and manure application;the metal elements mainly come from external environment;there is no metal pollution coming from mother material (coal mining wastes)in plough layer of covering soil. 相似文献
5.
ENVIRONMENTAL SUSTAINABILITY AND SCENARIOS OF URBANIZATION IN ARID AREA——A Case Study in Wuwei City of Gansu Province 总被引:1,自引:0,他引:1
YOUFei LIYu DONGSuo-cheng 《中国地理科学(英文版)》2005,15(2):120-130
1IN T R O D U C T IO N The western China isfacinggrowing problems of eco- logicaland economic development. The disparitiebse- tween the socio-economy of the western and eastern China were enlarging, and the major ecologicalprob- lems stilelvolve as past(H… 相似文献
6.
Methyl-galactosides were oxidized at room temperature by galactose oxidase in a one-step reaction and afforded methyl-galactoaldehyde
in excellent yield and high purity. The resulting galactoaldehyde as a useful intermediate can be directly used in glycopeptide
synthesis. 相似文献
7.
本文通过对1980年以来长江上游10次洪涝过程的500hpa环流形势分析,并用车比雪夫多项式对500hpa高度场进行展开,研究了各类洪涝过程的中期演变特征,发现代表不同洪涝过程环流形势变化的不同的车氏系数值都有明显的特征变化,结合欧洲中心中期数值预告96小时500hpa高度场的车氏系数分析,可为洪涝暴雨的中期预报提供一种新的思路。 相似文献
8.
Baolin Tan Haisheng Ji Guangli Huang Tuanhui Zhou Qiwu Song Yu Huang 《Solar physics》2006,239(1-2):137-148
Using one-minute cadence vector magnetograms from Big Bear Solar Observatory (BBSO), we analyze the temporal behavior of derived
longitudinal electric currents associated with two flares on July 26, 2002. One of the events is an M1.0 flare which occurred
in active region NOAA 10044, while the other is an M8.7 flare in the adjacent region 10039. Rapid changes of magnetic fields
in the form of flux emergence are found to be associated with both of these events. However, the temporal behavior of electric
currents are very different. For the M1.0 flare, the longitudinal electric current density drops rapidly near the flaring
neutral line; while for the M8.7 flare, the current density rapidly increases, confirming the picture of the current-carrying
flux emergence. We offer a possible explanation for such a difference: magnetic reconnection at different heights for the
two events, near the photosphere for the M1.0 flare, and higher up for the M8.7 flare. 相似文献
9.
10.
Byurakan Astrophysical Observatory. Translated from Astrofizika, Vol. 33, No. 2, pp. 271–281, September–October, 1990. 相似文献