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城市地区大气气溶胶颗粒的物理化学特性复杂,理清单颗粒精细的化学成分和混合状态对于大气污染溯源和精细治理具有重要意义。本研究利用被动式气溶胶采样器分别在山东省日照市城区和钢铁园区两个区域进行了定点采样,并利用智能扫描电镜环境颗粒物分析系统（IntelliSEM EPAS）对采集的大气单颗粒物样品进行分析。结果表明,日照市大气颗粒物主要由不规则碳质颗粒（C-rich）、含硫颗粒（Ca-S、Na-S-Ca）与矿物颗粒组成。其中,城区样品中C-rich颗粒数量贡献为53.5%,是钢铁园区样品的2.5倍,大于1 μm的颗粒物数量为9.0%,是钢铁园区样品的1.7倍,城区居民活动和工业过程是城市中大气颗粒物特别是二次细颗粒的主要来源。钢铁园区样品中含硫颗粒物数量贡献为72.9%,含硫颗粒物质量贡献为30.9%,富铁颗粒物质量贡献为5.3%,分别是城区样品的1.8倍、3.6倍和2.9倍,表明钢铁园区大气颗粒物的主要来源包括钢铁企业排放的一次污染物及其转化生成的二次细颗粒物。 相似文献
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A Leeway-Trace model was established for the traceability analysis of drifting objects at sea. The model was based on the Leeway model which is a Monte Carlo-based ensemble trajectory model, and a method of realistic traceability analysis was proposed in this study by using virtual spatiotemporal drift trajectory prediction. Here,measured data from a drifting buoy observation experiment in the northern South China Sea in April 2019,combined with surface current data obtained from the finite volu... 相似文献
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Yong CHEN Junling AN Yele SUN Xiquan WANG Yu QU Jingwei ZHANG Zifa WANG Jing DUAN 《大气科学进展》2018,35(12):1455-1468
Three-month wind profiles, 260 m PM1 concentrations [i.e., particulate matter (PM) with an aerodynamic diameter ≤ 1 μm], and carrier-to-noise ratio data at two Beijing sites 55 km apart (urban and suburban) were collected to analyze the characteristics of low-level nocturnal wind and PM in autumn and winter. Three mountain-plain wind events with wind shear were selected for analysis. The measurements indicated that the maximum wind speeds of the northerly weak low-level jet (LLJ) below 320 m at the suburban site were weaker than those at the urban site, and the LLJ heights and depths at the suburban site were lower than those at the urban site. The nocturnal 140 m mean vertical velocities and the variations in vertical velocity at the urban site were larger than those at the suburban site. A nocturnal breeze with a weak LLJ of ～3 m s-1 noticeably offset nocturnal PM transport due to southerly flow and convergence within the northern urban area of Beijing. Characteristics of the nocturnal LLJ, such as start-up time, structure, intensity, and duration, were important factors in determining the decrease in the nocturnal horizontal range and site-based low-level variations in PM. 相似文献
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Growth of fine aerosol particles is investigated during the Aerosol–CCN–Cloud Closure Experiment campaign in June2013 at an urban site near Beijing. Analyses show a high frequency(~ 50%) of fine aerosol particle growth events, and show that the growth rates range from 2.1 to 6.5 nm h~(-1) with a mean value of ~ 5.1 nm h~(-1). A review of previous studies indicates that at least four mechanisms can affect the growth of fine aerosol particles: vapor condensation, intramodal coagulation,extramodal coagulation, and multi-phase chemical reaction. At the initial stage of fine aerosol particle growth, condensational growth usually plays a major role and coagulation efficiency generally increases with particle sizes. An overview of previous studies shows higher growth rates over megacity, urban and boreal forest regions than over rural and oceanic regions. This is most likely due to the higher condensational vapor, which can cause strong condensational growth of fine aerosol particles.Associated with these multiple factors of influence, there are large uncertainties for the aerosol particle growth rates, even at the same location. 相似文献
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Observation of wind shear during evening transition and an estimation of submicron aerosol concentrations in Beijing using a Doppler wind lidar 
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下载免费PDF全文 Yong Chen Junling An Xiquan Wang Yele Sun Zifa Wang Jing Duan 《Acta Meteorologica Sinica》2017,31(2):350-362
The wind speed and direction measured over six months by a Doppler wind lidar (Windcube-8) were compared with wind cup anemometers mounted on the 325-m Beijing meteorological tower (BMT). Five mountain–plain wind cases characterized by wind direction shear were selected based on the high-frequency (1.1 s) wind profile of the Windcube-8 and analyzed with 1-h mesoscale surface weather charts. Also analyzed was the relationship between in-situ PM1 (aerodynamic diameter ≤ 1 μm) concentrations measured at 260 m on BMT and the carrier-to-noise ratio (CNR) of the co-located Windcube-8. The results showed that the 10-min averaged wind speed and direction were highly correlated (R = 0.96–0.99) at three matched levels (80, 140, and 200 m). The evening transition duration was 1–3 h, with an average wind speed of 1 m s–1 at 80 m above the ground. In addition, there was a zero horizontal-wind-speed zone along the wind direction shear line, and in one case, the wind speed was characterized by a Kelvin–Helmholtz gravity wave. The variability of the PM1 concentrations was captured by the CNR of the Windcube-8 in a fair weather period without the long-range transport of dust. 相似文献
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Yuting ZHANG Xiaole PAN Yu TIAN Hang LIU Xueshun CHEN Baozhu GE Zhe WANG Xiao TANG Shandong LEI Weijie YAO Yuanzhe REN Yongli TIAN Jie LI Pingqing FU Jinyuan XIN Yele SUN Junji CAO Zifa WANG 《大气科学进展》2022,39(10):1608-1622
The attainment of suitable ambient air quality standards is a matter of great concern for successfully hosting the XXIV Olympic Winter Games (OWG). Transport patterns and potential sources of pollutants in Zhangjiakou (ZJK) were investigated using pollutant monitoring datasets and a dispersion model. The PM2.5 concentration during February in ZJK has increased slightly (28%) from 2018 to 2021, mostly owing to the shift of main potential source regions of west-central Inner Mongolia and Mongolian areas (2015–18) to the North China Plain and northern Shanxi Province (NCPS) after 2018. Using CO as an indicator, the relative contributions of the different regions to the receptor site (ZJK) were evaluated based on the source-receptor-relationship method (SRR) and an emission inventory. We found that the relative contribution of pollutants from NCPS increased from 33% to 68% during 2019–21. Central Inner Mongolia (CIM) also has an important impact on ZJK under unfavorable weather conditions. This study demonstrated that the effect of pollution control measures in the NCPS and CIM should be strengthened to ensure that the air quality meets the standard during the XXIV OWG. 相似文献
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基于GIS的呼和浩特市近百年街道时空演变及其特征分析 总被引：1，自引：1，他引：0
以历史文化名城——呼和浩特市城区为研究区,以GIS为技术平台,运用现代地图、古地图、遥感影像数据以及史料和现代文献,制作了6个典型时期历史街道GIS数据,定量与定性相结合分析了研究区近百余年的街道时空演变过程及其特征。结果显示：研究区近百年的街道时空演变具有“摊饼式”空间扩展特征、先集聚后分散的空间演变特征;解放初期至改革开放时期的街道演变具有向内填充式发展与向北缓慢扩展相结合演变的特点,而快速城市化时期研究区新增街道以原归化、绥远城为中心向四周延伸,呈现出向外扩展的空间演变特征;百余年后的今天,原归化城内的街巷基本消失,而绥远城内的街道基本上保持了清代的棋盘式格局;人口增加、城市规划与建设、集聚与分散以及地质地貌条件等是研究区街道时空演变的主要驱动因素。 相似文献
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