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排序方式: 共有379条查询结果,搜索用时 125 毫秒
1.
Naoki Shirai Yuzuru Karouji Kazuya Kumagai Masayuki Uesugi Kaori Hirahara Motoo Ito Naotaka Tomioka Kentaro Uesugi Akira Yamaguchi Naoya Imae Takuji Ohigashi Toru Yada Masanao Abe 《Meteoritics & planetary science》2020,55(7):1665-1680
Chemical compositions of materials used for new sample holders (vertically aligned carbon nanotubes [VACNTs] and polyimide film), which were developed for the analysis of Hayabusa2‐return samples, were determined by instrumental neutron activation analysis and/or instrumental photon activation analysis, to estimate contamination effects from the sample holders. The synthetic quartz plate used for the sample holders was also analyzed. Ten elements (Na, Al, Cr, Mn, Fe, Ni, Eu, W, Au, and Th) and 14 elements (Na, Al, K, Sc, Ti, Cr, Zn, Ga, Br, Sb, La, Eu, Ir, and Au) could be detected in the VACNTs and polyimide film, respectively. The VACNT data show that contamination by this material with respect to the Murchison meteorite is negligible in terms of the elemental ratios (e.g., Fe/Mn, Na/Al, and Mn/Cr) used for the classification of meteorites due to the extremely low density of VACNTs. However, for the Au/Cr ratio, even small degrees (1.7 wt%) of contamination by VACNTs will change the Au/Cr ratio. Elemental ratios used for the classification of meteorites are only influenced by large amounts of contamination (>60 wt%) of polyimide film, which is unlikely to occur. In contrast, detectable effects on Ti isotopic compositions are caused by >0.1 and >0.3 wt% contamination by VACNTs and polyimide film, respectively, and Hf isotopic changes are caused by >0.1 wt% contamination by VACNTs. The new sample holders (VACNTs and polyimide film) are suitable for chemical classification of Hayabusa2‐return samples, because of their ease of use, applicability to multiple analytical instruments, and low contamination levels for most elements. 相似文献
2.
Solution Chemistry and the 36~(th) International Conference on Solution Chemistry (36 ICSC) in Xining,China 下载免费PDF全文
Toshio YAMAGUCHI 《盐湖研究》2019,(2)
<正>Solution chemistry covers a broad and interdisciplinary area in chemistry,physics,biology,pharmaceutical,and medical sciences,as well as various application fields. With the advent of new theories,analytical methods,computers,and technology,the research area of solution chemistry has now been widely and deeply 相似文献
3.
Ratan K. Majumder M. A. Halim B. B. Saha Reo Ikawa Toshio Nakamura Makoto Kagabu Jun Shimada 《Environmental Earth Sciences》2011,64(5):1343-1352
A total number of 328 groundwater samples are analysed to evaluate the groundwater flow systems in Bengal Delta aquifers,
Bangladesh using environmental isotope (2H, 18O, 13C, 3H, and 14C) techniques. A well-defined Local Meteoric Water Line (LMWL) δ2H = 7.7 δ18O + 10.7 ‰ is constructed applying linear correlation analyses to the monthly weighted rainfall isotopic compositions (δ18O and δ2H). The δ18O and δ2H concentrations of all groundwater samples in the study area are plotted more or less over the LMWL, which provides compelling
evidence that all groundwaters are derived from rainfall and floodwater with a minor localized evaporation effects for the
shallow groundwaters. Tritium concentration is observed in 40 samples out of 41 with values varying between 0.3 and 5.0 TU,
which represents an evidence of young water recharge to the shallow and intermediate aquifers. A decreasing trend of 14C activity is associated with the heavier δ13C values, which indicates the presence of geochemical reactions affecting the 14C concentration along the groundwater flow system. Both vertical and lateral decrease of 14C activity toward down gradient show the presence of regional groundwater flow commencing from the unconfined aquifers, which
discharges along the coastal regions. Finally, shallow, intermediate, and deep groundwater flow dynamics has revealed in the
Bengal Delta aquifers, Bangladesh. 相似文献
4.
Nickel plays a central role as an enzyme co-factor in the metabolism of methanogenic Archaea. Methanogens can fractionate Ni isotopes during assimilation, opening the possibility of using the stable isotopic composition of Ni as a biomarker. However, other sources of Ni isotopic variations need to be evaluated before one can establish Ni isotopes as an unambiguous tracer of methanogenesis in the rock record. Equilibrium exchange of Ni between the different species present in the ocean is a potential source of isotopic fractionation. Through controlled laboratory experiments and theoretical calculations, we quantify equilibrium Ni isotope fractionation between different species relevant to the modern and ancient ocean: Ni(H2O)62+, Ni(H2O)182+, NiOH(H2O)5+, Ni(OH)2(H2O)4, NiCl(H2O)5+, cis-NiCl2(H2O)4, trans-NiCl2(H2O)4, NiHS(H2O)5+, Ni(HS)2(H2O)4, NiSO4(H2O)4, NiHCO3(H2O)4+, NiCO3(H2O)4, and organic ligands (crown ether and oxalic acid). The magnitude of ligand-controlled Ni isotopic fractionation, approximately 1.25‰/amu (2.5‰ for the 60Ni/58Ni ratio), is similar to that previously measured in cultures of methanogenic Archaea. 相似文献
5.
The microstructural state and evolution of fault gouge has important implications for the mechanical behaviour, and hence
the seismic slip potential of faults. We use 3D discrete element (DEM) simulations to investigate the fragmentation processes
operating in fault gouge during shear. Our granular fault gouge models consist of aggregate grains, each composed of several
thousand spherical particles stuck together with breakable elastic bonds. The aggregate grains are confined between two blocks
of solid material and sheared under a given normal stress. During shear, the grains can fragment in a somewhat realistic way
leading to an evolution of grain size, grain shape and overall texture. The ‘breaking up’ of the fault gouge is driven by
two distinct comminution mechanisms: grain abrasion and grain splitting. The relative importance of the two mechanisms depends
on applied normal stress, boundary wall roughness and accumulated shear strain. If normal stress is sufficiently high, grain
splitting contributes significantly to comminution, particularly in the initial stages of the simulations. In contrast, grain
abrasion is the dominant mechanism operating in simulations carried out at lower normal stress and is also the main fragmentation
mechanism during the later stages of all simulations. Rough boundaries promote relatively more grain splitting whereas smooth
boundaries favor grain abrasion. Grain splitting (plus accompanying abrasion) appears to be an efficient mechanism for reducing
the mean grain size of the gouge debris and leads rapidly to a power law size distribution with an exponent that increases
with strain. Grain abrasion (acting alone) is an effective way to generate excess fine grains and leads to a bimodal distribution
of grain sizes. We suggest that these two distinct mechanisms would operate at different stages of a fault’s history. The
resulting distributions in grain size and grain shape may significantly affect frictional strength and stability. Our results
therefore have implications for the earthquake potential of seismically active faults with accumulations of gouge. They may
also be relevant to the susceptibility of rockslides since non-cohesive basal shear zones will evolve in a similar way and
potentially control the dynamics of the slide. 相似文献
6.
7.
Maki Morimoto Kyoko Kawanobe Osamu Abe Takayoshi Kawai Toshiyuki Kawamura Kunio Shirasawa 《水文研究》2010,24(7):904-916
In winter, lakes and lagoons at high altitudes or high latitudes have interesting hydrological cycles that differ from those in other seasons or in other regions, because water surfaces are covered with ice. Hydrological balances of lakes and lagoons are complex dynamic systems, and to elucidate them, isotopic tracers of water have been used as effective tools along with observations of precipitation, evaporation, inflows, and outflows. Here, to understand hydrological processes during freezing periods in the brackish Saroma‐ko Lagoon, Hokkaido, northern Japan, we examined horizontal and vertical distributions of salinity and isotope compositions of lagoon water and ice in 2005 and 2006. Horizontal and vertical gradients of salinity and isotope compositions were observed from the river mouth to the sea channel, and factors determining these distributions were considered. The mixing of freshwater and seawater and a freezing effect were presumed to be factors in relationships between salinity and isotopes and in relationships between surface waters and ice just above the water. A simple box model for water balance was constructed based on these putative factors to reproduce the distributions of salinity and isotope compositions of surface waters and ice. An evaluation of the model revealed that this hydrological system is controlled primarily by horizontal advection of the epilimnion, freshwater influx, and the ice growth rate. Copyright © 2009 John Wiley & Sons, Ltd. 相似文献
8.
Kazuo Abe 《Journal of Oceanography》2002,58(4):577-588
The relationship between dissolved cadmium (Cd) and phosphate (PO4) was examined at three stations in the subtropical area near the Ryukyu Islands in May 1999. Preformed PO4 was obtained using the Redfield ratio in order to separate the surface water and the other layers in this study area. Almost
0 μM (−0.043 μM to 0.094 μM) was estimated in the layers above 300 m and 250 m at Sts. 1 and 3 and at St. 2, respectively.
Up to these depths, water was considered to be uniform, and these layers were defined as the surface water in this study area.
In the surface water, the slopes of the regression lines of the Cd-PO4 plot were 0.162, 0.156, and 0.226 (nM/μM) at Sts. 1, 2, and 3, respectively, and these values were much closer to the estimated
regenerated ratio of Cd to PO4 from the Apparent Oxygen Utilization (AOU)-Cd/PO4 plots, which was 0.197 (nM/μM) in this study area. Below surface layers, the slopes of the Cd-PO4 plot changed to 0.371, 0.352, and 0.362 (nM//μM) at Sts. 1, 2, and 3, respectively. In the relationships between Cd and PO4, clear deviations or kinks were observed at three stations at a PO4 concentration of approximately 0.2 μM in the plot, which was attributable to the discontinuity of surface water and the other
layers across the North Pacific subtropical mode water. In studies of the interaction between surface water and biogenic particles
concerning the Cd/PO4 ratio, separate analyses of seawater (surface water and the other layers) should be carried out to obtain the individual
surface water ratio because the Cd/PO4 ratio in the surface water is expected to differ from that of the underlying water. Furthermore, the biological fractionation
of these constituents is based on the surface water ratio.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
9.
Humitake Seki Hideshi Abe Yukuya Yamaguchi Shun-ei Ichimura 《Journal of Oceanography》1974,30(3):151-156
About 106 of total bacteria (direct microscopic count) or heterotrophic bacteria (colony count with Medium 2216E) and about 104 of petroleumlytic bacteria (oil-oxidizing bacteria) were enumerated per square centimeter of the surface of petroleum globules suspended in the topmost 10 meters of water from a station (22°00.2N, 125°51.9E) in the western North Pacific central water, where about 107 of total bacteria, about 103 of heterotrophic bacteria and about 10 of petroleumlytic bacteria were enumerated per liter of seawater. 相似文献
10.
In inviscid shallow water models currents generated by spatially uniform winds are transient and are eliminated by Rossby and equatorial Kelvin waves excited at the eastern and western coasts, respectively. The inclusion of mixing processes can lead to an entirely different steady state in which currents are present. It is shown that the mixing of heat affects the steady state more than does the mixing of momentum because the waves that are important in the oceanic adjustment are divergent. 相似文献