60Fe–60Ni systematics in the eucrite parent body: A case study of Bouvante and Juvinas     

Ghylaine Quitté  Christopher Latkoczy  Maria Schönbächler  Alex N. Halliday  Detlef Günther 《Geochimica et cosmochimica acta》2011,75(23):7698-7706

Eucrites are basaltic meteorites that cooled rapidly but are in many instances thermally metamorphosed and impact brecciated. The exact timing of these events remains unclear. In this study, Ni isotopic compositions and Fe/Ni elemental ratios are presented for two non-cumulate eucrites, Bouvante and Juvinas, including mineral separates from the latter. The samples are characterized by variable, well-resolved ⁶⁰Ni-excesses consistent with the former presence of live ⁶⁰Fe (t_1/2 = 2.62 Ma) at the time of eucrite crystallization. A significant fraction of Ni with a terrestrial-like composition appears to be surface correlated. This Ni may be the product of terrestrial contamination or was introduced by a chondritic impactor during brecciation. Altogether, the data provide evidence for a complex and probably multi-stage history of Fe and/or Ni redistribution, which impedes the interpretation of the chronological data.  相似文献   

Evolution of anthropogenic and biomass burning emissions of air pollutants at global and regional scales during the 1980�C2010 period     

Claire Granier  Bertrand Bessagnet  Tami Bond  Ariela D��Angiola  Hugo Denier van der Gon  Gregory J. Frost  Angelika Heil  Johannes W. Kaiser  Stefan Kinne  Zbigniew Klimont  Silvia Kloster  Jean-Fran?ois Lamarque  Catherine Liousse  Toshihiko Masui  Frederik Meleux  Aude Mieville  Toshimasa Ohara  Jean-Christophe Raut  Keywan Riahi  Martin G. Schultz  Steven J. Smith  Allison Thompson  John van Aardenne  Guido R. van der Werf  Detlef P. van Vuuren 《Climatic change》2011,109(1-2):163-190

Several different inventories of global and regional anthropogenic and biomass burning emissions are assessed for the 1980?C2010 period. The species considered in this study are carbon monoxide, nitrogen oxides, sulfur dioxide and black carbon. The inventories considered include the ACCMIP historical emissions developed in support of the simulations for the IPCC AR5 assessment. Emissions for 2005 and 2010 from the Representative Concentration Pathways (RCPs) are also included. Large discrepancies between the global and regional emissions are identified, which shows that there is still no consensus on the best estimates for surface emissions of atmospheric compounds. At the global scale, anthropogenic emissions of CO, NO_x and SO₂ show the best agreement for most years, although agreement does not necessarily mean that uncertainty is low. The agreement is low for BC emissions, particularly in the period prior to 2000. The best consensus is for NO_x emissions for all periods and all regions, except for China, where emissions in 1980 and 1990 need to be better defined. Emissions of CO need better quantification in the USA and India for all periods; in Central Europe, the evolution of emissions during the past two decades needs to be better determined. The agreement between the different SO₂ emissions datasets is rather good for the USA, but better quantification is needed elsewhere, particularly for Central Europe, India and China. The comparisons performed in this study show that the use of RCP8.5 for the extension of the ACCMIP inventory beyond 2000 is reasonable, until more global or regional estimates become available. Concerning biomass burning emissions, most inventories agree within 50?C80%, depending on the year and season. The large differences between biomass burning inventories are due to differences in the estimates of burned areas from the different available products, as well as in the amount of biomass burned.  相似文献   

How well do integrated assessment models simulate climate change?     

Detlef P. van Vuuren  Jason Lowe  Elke Stehfest  Laila Gohar  Andries F. Hof  Chris Hope  Rachel Warren  Malte Meinshausen  Gian-Kasper Plattner 《Climatic change》2011,104(2):255-285

Integrated assessment models (IAMs) are regularly used to evaluate different policies of future emissions reductions. Since the global costs associated with these policies are immense, it is vital that the uncertainties in IAMs are quantified and understood. We first demonstrate the significant spread in the climate system and carbon cycle components of several contemporary IAMs. We then examine these components in more detail to understand the causes of differences, comparing the results with more complex climate models and earth system models (ESMs), where available. Our results show that in most cases the outcomes of IAMs are within the range of the outcomes of complex models, but differences are large enough to matter for policy advice. There are areas where IAMs would benefit from improvements (e.g. climate sensitivity, inertia in climate response, carbon cycle feedbacks). In some cases, additional climate model experiments are needed to be able to tune some of these improvements. This will require better communication between the IAM and ESM development communities.  相似文献   

An ESA NEOCC Effort to Eliminate High Palermo Scale Virtual Impactors     

Marco Micheli  Detlef Koschny  Gerhard Drolshagen  Olivier Hainaut  Fabrizio Bernardi 《Earth, Moon, and Planets》2014,113(1-4):1-13

In this work we summarize the initial results of a targeted effort of the ESA NEO Coordination Centre to obtain additional observational data in order to eliminate or reduce the impact probability estimate of a subset of the known near-Earth objects representing the highest fraction of the total known impact risk, as measured by the Palermo Scale.  相似文献   

Consistent realization of Celestial and Terrestrial Reference Frames     

Younghee Kwak  Mathis Bloßfeld  Ralf Schmid  Detlef Angermann  Michael Gerstl  Manuela Seitz 《Journal of Geodesy》2018,92(9):1047-1061

The Celestial Reference System (CRS) is currently realized only by Very Long Baseline Interferometry (VLBI) because it is the space geodetic technique that enables observations in that frame. In contrast, the Terrestrial Reference System (TRS) is realized by means of the combination of four space geodetic techniques: Global Navigation Satellite System (GNSS), VLBI, Satellite Laser Ranging (SLR), and Doppler Orbitography and Radiopositioning Integrated by Satellite. The Earth orientation parameters (EOP) are the link between the two types of systems, CRS and TRS. The EOP series of the International Earth Rotation and Reference Systems Service were combined of specifically selected series from various analysis centers. Other EOP series were generated by a simultaneous estimation together with the TRF while the CRF was fixed. Those computation approaches entail inherent inconsistencies between TRF, EOP, and CRF, also because the input data sets are different. A combined normal equation (NEQ) system, which consists of all the parameters, i.e., TRF, EOP, and CRF, would overcome such an inconsistency. In this paper, we simultaneously estimate TRF, EOP, and CRF from an inter-technique combined NEQ using the latest GNSS, VLBI, and SLR data (2005–2015). The results show that the selection of local ties is most critical to the TRF. The combination of pole coordinates is beneficial for the CRF, whereas the combination of \(\varDelta \hbox {UT1}\) results in clear rotations of the estimated CRF. However, the standard deviations of the EOP and the CRF improve by the inter-technique combination which indicates the benefits of a common estimation of all parameters. It became evident that the common determination of TRF, EOP, and CRF systematically influences future ICRF computations at the level of several \(\upmu \)as. Moreover, the CRF is influenced by up to \(50~\upmu \)as if the station coordinates and EOP are dominated by the satellite techniques.  相似文献   

Ablation Characteristic of Ilmenite using UV Nanosecond and Femtosecond Lasers: Implications for Non‐Matrix‐Matched Quantification          下载免费PDF全文

Zhen Li  Zhaochu Hu  Detlef Günther  Keqing Zong  Yongsheng Liu  Tao Luo  Wen Zhang  Shan Gao  Shenghong Hu 《Geostandards and Geoanalytical Research》2016,40(4):477-491

Ilmenite (FeTiO₃) is a common accessory mineral and has been used as a powerful petrogenetic indicator in many geological settings. Elemental fractionation and matrix effects in ilmenite (CRN63E‐K) and silicate glass (NIST SRM 610) were investigated using 193 nm ArF excimer nanosecond (ns) laser and 257 nm femtosecond (fs) laser ablation systems coupled to an inductively coupled plasma‐mass spectrometer. The concentration‐normalised ⁵⁷Fe and ⁴⁹Ti responses in ilmenite were higher than those in NIST SRM 610 by a factor of 1.8 using fs‐LA. Compared with the 193 nm excimer laser, smaller elemental fractionation was observed using the 257 nm fs laser. When using 193 nm excimer laser ablation, the selected range of the laser energy density had a significant effect on the elemental fractionation in ilmenite. Scanning electron microscopy images of ablation craters and the morphologies of the deposited aerosol materials showed more melting effects and an enlarged particle deposition area around the ablation site of the ns‐LA‐generated crater when compared with those using fs‐LA. The ejected material around the ns crater predominantly consisted of large droplets of resolidified molten material; however, the ejected material around the fs crater consisted of agglomerates of fine particles with ‘rough' shapes. These observations are a result of the different ablation mechanisms for ns‐ and fs‐LAs. Non‐matrix‐matched calibration was applied for the analysis of ilmenite samples using NIST SRM 610 as a reference material for both 193 nm excimer LA‐ICP‐MS and fs‐LA‐ICP‐MS. Similar analytical results for most elements in ilmenite samples were obtained using both 193 nm excimer LA‐ICP‐MS at a high laser energy density of 12.7 J cm^?2 and fs‐LA‐ICP‐MS.  相似文献   

Erratum to: Linking the thermal evolution and emplacement history of an upper-crustal pluton to its lower-crustal roots using zircon geochronology and geochemistry (Southern Adamello Batholith,N. Italy)     

Cindy Broderick  Jörn F. Wotzlaw  Daniel A. Frick  Axel Gerdes  Alex Ulianov  Detlef Günther  Urs Schaltegger 《Contributions to Mineralogy and Petrology》2016,171(3):27

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On Boussinesq's problem for Maxwell continua subject to an external gravity field     

Detlef Wolf 《Geophysical Journal International》1985,80(1):275-279

Summary. Boussinesq's problem is solved for a uniform and incompressible Maxwell half-space subject to an external gravity field. The solution is based on momentum equations which account for stress advection in the hydrostatically pre-stressed continuum during its deformation. The analysis shows that disregarding the pre-stress term renders the theoretical stress distribution incorrect and the deformation singular in the inviscid limit of the Maxwell continuum. Our solution is contrasted with a recently published alternative solution of the same problem, where regularity in the inviscid limit was forced by modified boundary conditions.  相似文献   

Viscoelastodynamics of A Stratified, Compressible Planet: Incremental Field Equations and Short- and Long-Time Asymptotes     

Detlef Wolf 《Geophysical Journal International》1991,104(2):401-417

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The effect of iron availability on the regulation of inorganic carbon acquisition in the coccolithophore Emiliania huxleyi and the significance of cellular compartmentation for stable carbon isotope fractionation     

K.G. Schulz  B. Rost  U. Riebesell  D.A. Wolf-Gladrow 《Geochimica et cosmochimica acta》2007,71(22):5301-5312

Iron is limiting phytoplankton productivity in large parts of today’s oceans, the so-called HNLC (high nutrient low chlorophyll) areas. It is a key component in photosynthesis during which inorganic carbon fixation in most phytoplankton species is sustained by so-called carbon concentrating mechanisms (CCMs). Here we investigate CCM regulation in the coccolithophore Emiliania huxleyi in response to varying degrees of iron limitation by means of membrane-inlet mass spectrometry. Compared to iron replete conditions rates of both active CO₂ and uptake were markedly reduced under iron limitation leading to significantly diminished growth rates. Moreover, there was a concomitant decrease in CCM efficiency, reflected in an increased CO₂ loss from the cell in relation to carbon fixation. Under such conditions higher values for carbon isotope fractionation (?_p) would be expected. However, direct measurements of ?_p showed that carbon isotope fractionation was insensitive to changes in growth rates and CCM activity. This can be explained by concomitant changes in internal DIC fluxes in and out of the chloroplast as demonstrated with a simple cell model comprising two compartments. Thus, carbon isotope fractionation reflects the ability of phytoplankton to actively control their inorganic carbon acquisition depending on environmental conditions. The insensitivity of carbon isotope fractionation to changes in the availability of iron could be of interest for paleoreconstructions in the HNLC areas of today’s oceans.  相似文献