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This review is devoted to problems in the photochemical modeling of atmospheric processes. The physicochemical and mathematical foundations underlying the construction of photochemical models are described, a classification of the atmospheric reactions is presented, and the features of photochemical modeling are considered under various irradiance conditions for various atmospheric layers and geographical regions. Atmospheric processes that are important to photochemical models are discussed. Applications involving photochemical models are outlined. Some results are presented to illustrate the capabilities of photochemical models. Special attention is given to relatively recent directions in photochemical modeling, such as data assimilation and inverse problems. The review can be used by experts in areas related to atmospheric chemistry as a basic source of knowledge on the subject and for the development of photochemical modules for atmospheric models. 相似文献
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V. A. Frol’kis I. L. Karol’ A. A. Kiselev Yu. E. Ozolin V. A. Zubov 《Izvestiya Atmospheric and Oceanic Physics》2007,43(4):413-422
This is a study of the sensitivity of model results (atmospheric content of main gas constituents and radiative characteristics of the atmosphere) to errors in emissions of a number of atmospheric gaseous pollutants. Groups of the model variables most dependent on these errors are selected. Two variants of emissions are considered: one without their evolution and the other with their variation according to the IPCC scenario. The estimates are made on the basis of standard statistical methods for the results obtained with the detailed onedimensional radiative—photochemical model of the Main Geophysical Observatory (MGO). Some approaches to such estimations with models of higher complexity and to the solution of the inverse problem (i.e., the estimation of the necessary accuracy of external model parameters for obtaining the given accuracy of model results) are outlined. 相似文献
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Karolina Kośmińska Frank S. Spear Jarosław Majka Karol Faehnrich Maciej Manecki Karsten Piepjohn Winfried K. Dallmann 《Journal of Metamorphic Geology》2020,38(5):471-493
Quartz-in-garnet inclusion barometry integrated with trace element thermometry and calculated phase relations is applied to mylonitized schists of the Pinkie unit cropping out on the island of Prins Karls Forland, western part of the Svalbard Archipelago. This approach combines conventional and novel techniques and allows deciphering of the pressure–temperature (P–T) evolution of mylonitic rocks, for which the P–T conditions could not have been easily deciphered using traditional methods. The results obtained suggest that rocks of the Pinkie unit were metamorphosed under amphibolite facies conditions at 8–10 kbar and 560–630°C and mylonitized at ~500 to 550°C and 9–11 kbar. The P–T results are coupled with in-situ Th–U-total Pb monazite dating, which records amphibolite facies metamorphism at c. 359–355 Ma. This is the very first evidence of late Devonian–early Carboniferous metamorphism in Svalbard and it implies that the Ellesmerian Orogeny on Svalbard was associated with metamorphism up to amphibolite facies conditions. Thus, it can be concluded that the Ellesmerian collision between the Franklinian margin of Laurentia and Pearya and Svalbard caused not only commonly accepted brittle deformation and weak greenschist facies metamorphism, but also a burial and deformation of rock complexes at much greater depths at elevated temperatures. 相似文献
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The determination of the bottom of a subfossil meandering palaeochannel is important for investigations of the palaeohydrology of valley bottoms, and crucial for the quantitative estimation of past river discharges. The authors present a procedure on the basis of which the bottom of a palaeochannel can be precisely determined. It is based on an analysis of the stratigraphic variability of such features of deposits as: mean diameter, standard deviation of the grain-size composition, the percentage of sand, and ignition loss. 相似文献
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Linear trend analysis of geophysical time series is considered in connection with the problem of determining long-period variations (possibly of man-made origin) in the presence of short period noise of larger amplitude. Criteria for testing hypotheses about linear trends are presented for the cases of independent observations and of the observations whose correlation function is known. The possibility of increasing the precision of the results using area-averaged values is investigated. Examples are given of the long time series analysis of air temperature, carbon dioxide and water vapor content. Time series of total atmospheric ozone content at some stations are also considered, and conditions for correct statistical analysis of such data are given. 相似文献
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The paper presents a numerical solution of the oblique derivative boundary value problem on and above the Earth’s topography using the finite volume method (FVM). It introduces a novel method for constructing non-uniform hexahedron 3D grids above the Earth’s surface. It is based on an evolution of a surface, which approximates the Earth’s topography, by mean curvature. To obtain optimal shapes of non-uniform 3D grid, the proposed evolution is accompanied by a tangential redistribution of grid nodes. Afterwards, the Laplace equation is discretized using FVM developed for such a non-uniform grid. The oblique derivative boundary condition is treated as a stationary advection equation, and we derive a new upwind type discretization suitable for non-uniform 3D grids. The discretization of the Laplace equation together with the discretization of the oblique derivative boundary condition leads to a linear system of equations. The solution of this system gives the disturbing potential in the whole computational domain including the Earth’s surface. Numerical experiments aim to show properties and demonstrate efficiency of the developed FVM approach. The first experiments study an experimental order of convergence of the method. Then, a reconstruction of the harmonic function on the Earth’s topography, which is generated from the EGM2008 or EIGEN-6C4 global geopotential model, is presented. The obtained FVM solutions show that refining of the computational grid leads to more precise results. The last experiment deals with local gravity field modelling in Slovakia using terrestrial gravity data. The GNSS-levelling test shows accuracy of the obtained local quasigeoid model. 相似文献
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During a cruise of r/v ‘Oceania’ in May 2006, seven vertical dissolved organic carbon (DOC) concentration profiles were produced against a background of CTD, chlorophyll a (chl a) and phaeopigment concentration profiles. The results indicate distinct vertical and spatial DOC fluctuations, ranging from 248 ± 7 μmol C dm−3 at 70 m depth at the westernmost station G/06 to 398 ± 5 μmol C dm−3 at 5 m depth at station A/06 in the western Gulf of Gdańsk. DOC concentrations were the highest at 10 m depth, where phytoplankton activity was relatively intensive, as reflected by the active chl a concentration distribution. DOC concentrations decreased towards the sea bottom. 相似文献
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A. I. Reshetnikov A. V. Zinchenko S. V. Yagovkina I. L. Karol V. E. Lagun N. N. Paramonova 《Russian Meteorology and Hydrology》2009,34(3):171-179
Methane emitted into the atmosphere from sources located in the Urengoi natural gas field is estimated from direct methane concentration measurements in the atmospheric boundary layer and modeling. The results of direct profile measurements in the summer-fall season of 2003 are generalized versus the data from the previous field studies and background monitoring of greenhouse gases in the northern polar region. The use of models for calculating the intensity of emission from sources located in the field area together with a set of methane concentration measurements at three altitudes allowed the authors to develop a method of verification of emission from a specific source, a deposit. The method estimates the emission both from part of the field area and from the whole field with an irregular distribution of the intensity of sources across the deposit area. 相似文献