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William A. Bonner Neal E. Blair Richard M. Lemmon Jose J. Flores Glenn E. Pollock 《Geochimica et cosmochimica acta》1979,43(11):1841-1846
The optically pure d- and l-enantiomers of isovaline (I), which cannot be racemized by ordinary chemical mechanisms involving α-hydrogen removal, and which has been isolated in apparently racemic form from the Murchison meteorite, have been subjected to partial radiolysis by the ionizing radiation from a 3000 Ci 60Co γ-ray source. Both in the anhydrous and hydrated solid states and as solid sodium or hydrochloride salts each enantiomer suffered significant radioracemization of the undestroyed residue during its partial radiolysis. The sodium salt of isovaline in 0.1 M aqueous solution suffered extensive radiolysis with relatively small radiation doses, but showed no detectable radioracemization. The significance of these observations with respect to the primordial enantiomeric composition of the isovaline (and other amino acids) indigenous to meteroties is discussed. 相似文献
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P. Descamps F. Marchis T. Michalowski J. Pollock M. Birlan F. Vachier M. Fauvaud F. Pilcher 《Icarus》2009,203(1):102-111
Mutual event observations between the two components of 90 Antiope were carried out in 2007-2008. The pole position was refined to λ0 = 199.5 ± 0.5° and β0 = 39.8 ± 5° in J2000 ecliptic coordinates, leaving intact the physical solution for the components, assimilated to two perfect Roche ellipsoids, and derived after the 2005 mutual event season (Descamps, P., Marchis, F., Michalowski, T., Vachier, F., Colas, F., Berthier, J., Assafin, M., Dunckel, P.B., Polinska, M., Pych, W., Hestroffer, D., Miller, K., Vieira-Martins, R., Birlan, M., Teng-Chuen-Yu, J.-P., Peyrot, A., Payet, B., Dorseuil, J., Léonie, Y., Dijoux, T., 2007. Figure of the double Asteroid 90 Antiope from AO and lightcurves observations. Icarus 187, 482-499). Furthermore, a large-scale geological depression, located on one of the components, was introduced to better match the observed lightcurves. This vast geological feature of about 68 km in diameter, which could be postulated as a bowl-shaped impact crater, is indeed responsible of the photometric asymmetries seen on the “shoulders” of the lightcurves. The bulk density was then recomputed to 1.28 ± 0.04 g cm−3 to take into account this large-scale non-convexity. This giant crater could be the aftermath of a tremendous collision of a 100-km sized proto-Antiope with another Themis family member. This statement is supported by the fact that Antiope is sufficiently porous (∼50%) to survive such an impact without being wholly destroyed. This violent shock would have then imparted enough angular momentum for fissioning of proto-Antiope into two equisized bodies. We calculated that the impactor must have a diameter greater than ∼17 km, for an impact velocity ranging between 1 and 4 km/s. With such a projectile, this event has a substantial 50% probability to have occurred over the age of the Themis family. 相似文献
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We evaluated controls on locations of channel incision, variation in channel evolution pathways and the time required to reconnect incised channels to their historical floodplains in the Walla Walla and Tucannon River basins, northwestern USA. Controls on incision locations are hierarchically nested. A first‐order geological control defines locations of channels prone to incision, and a second‐order control determines which of these channels are incised. Channels prone to incision are reaches with silt‐dominated valley fills, which have sediment source areas dominated by loess deposits and channel slopes less than 0·1(area)?0·45. Among channels prone to incision, channels below a second slope–area threshold (slope = 0·15(area)?0·8) did not incise. Once incised, channels follow two different evolution models. Small, deeply incised channels follow Model I, which is characterized by the absence of a significant widening phase following incision. Widening is limited by accumulation of bank failure deposits at the base of banks, which reduces lateral channel migration. Larger channels follow Model II, in which widening is followed by development of an inset floodplain and aggradation. In contrast to patterns observed elsewhere, we found the widest incised channels upstream of narrower reaches, which reflects a downstream decrease in bed load supply. Based on literature values of floodplain aggradation rates, we estimate recovery times for incised channels (the time required to reconnect to the historical floodplain) between 60 and 275 years. Restoration actions such as allowing modest beaver recolonization can decrease recovery time by 17–33 per cent. Published in 2007 by John Wiley & Sons, Ltd. 相似文献
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A Controlled Experiment in Ground Water Flow Model Calibration 总被引：3，自引：0，他引：3
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Semianalytical Computation of Path Lines for Finite-Difference Models 总被引：13，自引：0，他引：13
David W. Pollock 《Ground water》1988,26(6):743-750
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P. J. Crutzen A. C. Delany J. Greenberg P. Haagenson L. Heidt R. Lueb W. Pollock W. Seiler A. Wartburg P. Zimmerman 《Journal of Atmospheric Chemistry》1985,2(3):233-256
Field measurement programs in Brazil during the dry seasons in August and September 1979 and 1980 have demonstrated the large importance of the continental tropics in global air chemistry. Many important trace gases are produced in large amounts over the continents. During the dry season, much biomass burning takes place, especially in the cerrado regions, leading to a substantial emission of air pollutants, such as CO, NO
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, N2O, CH4 and other hydrocarbons. Ozone concentrations are enhanced due to photochemical reactions. The large biogenic organic emissions from tropical forests play an important role in the photochemistry of the atmosphere and explain why CO is present in such high concentrations in the boundary layer of the tropical forest. Carbon monoxide production may represent more than 3% of the net primary productivity of the tropical forests. Ozone concentrations in the boundary layer of the tropical forests indicate strong removal processes. Due to atmospheric supply of NO
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by lightning, there is probably a large production of O3 in the free troposphere over the Amazon tropical forests. This is transported to the marine-free troposphere and to the forest boundary layer. 相似文献