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O'Neill BC Gaffin SR Tubiello FN Oppenheimer M 《Tellus. Series B, Chemical and physical meteorology》1994,46(5):378-389
Non-steady state timescales are complicated and their application to specific geophysical systems requires a common theoretical foundation. We first extend reservoir theory by quantifying the difference between turnover time and transit time (or residence time) for time-dependent systems under any mixing conditions. We explicitly demonstrate the errors which result from assuming these timescales are equal, which is only true at steady state. We also derive a new response function which allows the calculation of age distributions and timescales for well-mixed reservoirs away from steady state, and differentiate between timescales based on gross and net fluxes. These theoretical results are particularly important to tracer-calibrated "box models" currently used to study the carbon cycle, which usually approximate reservoirs as well-mixed. We then apply the results to the important case of anthropogenic CO2 in the atmosphere, since timescales describing its behavior are commonly used but ambiguously defined. All relevant timescales, including lifetime, transit time, and adjustment time, are precisely defined and calculated from data and models. Apparent discrepancies between the current, empirically determined turnover time of 30-60 years and longer model-derived estimates of expected lifetime and adjustment time are explained within this theoretical framework. We also discuss the results in light of policy issues related to global warming, in particular since any comparisons of the "lifetimes" of different greenhouse gases (CO2, CH4, N2O, CFC's etc.) must use a consistent definition to be meaningful. 相似文献
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The concentrations of Ni, Cu, Zn, Ga, Ge, and Se in five, fine-grained chondrule rims in the highly unequilibrated CO3 chondrite ALH A77307 (3.0) have been determined for the first time by synchrotron X-ray fluorescence (SXRF) microprobe at Brookhaven National Laboratory. These elements are especially useful for tracing the role of condensation and evaporation processes which occurred at moderate temperatures in the solar nebula. Understanding the distribution of moderately volatile elements between matrix and chondrules is extremely important for evaluating the different models for the volatile depletions in chondritic meteorites. The data show that the trace element chemistry of rims on different chondrules is remarkably similar, consistent with data obtained for the major and minor elements by electron microprobe. These results support the idea that rims are not genetically related to individual chondrules, but all sampled the same reservoir of homogeneously mixed dust. Of the trace elements analyzed, Zn and Ga show depletions relative to CI chondrite values, but in comparison with bulk CO chondrites all the elements are enriched by approximately 1.5 to 3.5 x CO. The abundance patterns for moderately volatile elements in ALH A77307 chondrule rims closely mimic those observed in the bulk chondrite, indicating that matrix is the major reservoir for these elements. The close matching of the patterns for the volatile depleted bulk chondrite and enriched matrix is especially striking for Na, which is anomalously depleted in ALH A77307 in comparison with average CO chondrite abundances. The depletion in Na is probably attributable to the effects of leaching in Antarctica. With the exception of Na, the volatile elements show a relatively smooth decrease in abundance as a function of condensation temperature, indicating that their behavior is largely controlled by their volatility. 相似文献
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武夷山高溪和富城花岗岩体地球化学及其与铀成矿的关系 总被引：6，自引：2，他引：6
从成矿地质条件分析，武夷火山铀成矿带中的主要铀矿床的共同点是都具有花岗岩基底岩石。选择富城和高溪两花岗岩体进行地球化学研究。这两个岩体均为复式岩基，其主体岩石都形成于印支晚期（高溪：２１４．６Ｍａ；富城：２０３～２２６Ｍａ）。岩体中的长石为微斜长石；黑云母为铁云母和铁叶云母。岩石化学表现为富硅、偏碱和铝过饱和的特征。微量元素Ｃｏ、Ｎｉ、Ｃｒ、Ｓｒ、Ｂａ含量和Ｓｒ／Ｂａ比值较低，Ｒｂ、Ｎｂ、Ｐｂ、Ｚｎ的含量和Ｒｂ／Ｓｒ比值高。稀土总量较高，轻稀土富集，轻、重稀土的比值高，并有强烈的铕亏损。高溪和富城两岩体的初始锶同位素组成高（分别为０．７１２３９和０．７１９８），钕同位素组成低（－６．６２～－１２．８４），这些表明高溪岩体属改造型花岗岩。两岩体中活性铀的比例高，特别是在蚀变作用中活性铀的比例增加。铅同位素追踪研究表明，在蚀变过程中岩体中的铀发生了大量的丢失。矿石铅同位素和岩体铅同位素都位于造山带的演化线附近，且矿石铅、火山岩铅、花岗岩铅及基底变质岩铅同位素组成呈线性关系，据此认为高溪和富城花岗岩体分别是形成５７０和６７２２矿床主要铀源体之一 相似文献
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毛洋头铀（银,钼）矿床同位素地球化学研究 总被引：1，自引：0，他引：1
毛洋头铀矿床的（Ｈ、Ｏ）同位素特征表明：早期矿化热液主要为岩浆水，而晚期矿化热液则主要为大气降水。铅同位素组成反映该矿床中铅为不同来源的混合铅。Ｃ、Ｓ同位素组成变化范围小，且与火成岩的Ｃ、Ｓ同位素组成相当，说明矿床中的碳和硫主要淋取于火成围岩或源于地壳深部。 相似文献
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以前有关深成岩体的侵位研究都试图解释岩体侵位空间如何形成。事实上，幔源岩浆侵位期间在地壳中“制造空间”的途径不外乎；（１）莫霍面降低；（２）地球表面外移。其它的“岩体侵位机制”均是不增加地壳体积的物质迁移作用（ＭＴＰｓ）。得到广泛引用的“同心带状气球膨胀岩体”侵位时的ＭＴＰｓ是岩体附近围岩的韧性流动。这类深成岩体附近可能形成的构造和总应变与岩体的三维形态、接触变质带的宽度以及岩体是否为刺穿底辟有关 相似文献
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