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1.
Rhizofiltration is a subset technique of phytoremediation which refers to the approach of using plant biomass for removing contaminants, primarily toxic metals, from polluted water. The effective implementation of this in situ remediation technology requires experimental as well as conceptual insight of plant–water interactions that control the extraction of targeted metal from polluted water resources. Therefore, pot and simulation experiments are used in this study to investigate the rhizofiltration of a lead containing wastewater using plants of Carex pendula, a common wetland plant found in Europe. The metal contaminant extraction along with plant growth and water uptake rates from a wastewater having varying Pb concentration is studied experimentally for 2 wk. The temporal distribution of the metal concentration in the wastewater and the accumulated metal in different compartments of C. pendula at the end are analyzed using atomic absorption spectrometry. Parameters of the metal uptake kinetics are deduced experimentally for predicting the metal removal by root biomass. Further, mass balance equations coupled with the characterized metal uptake kinetics are used for simulating the metal partitioning from the wastewater to its accumulation in the plant biomass. The simulated metal content in wastewater and plant biomass is compared with the observed data showing a good agreement with the later. Results show that C. pendula accumulates considerable amounts of lead, particularly in root biomass, and can be considered for the cleanup of lead contaminated wastewaters in combination with proper biomass disposal alternatives. Also, the findings can be used for performing further non‐hydroponics experiment to mimic the real wetland conditions more closely.  相似文献   
2.
Correct interpretation of zircon ages from high-grade metamorphic terrains poses a major challenge because of the differential response of the U–Pb system to metamorphism, and many aspects like pressure–temperature conditions, metamorphic mineral transformations and textural properties of the zircon crystals have to be explored. A large (c. 450?km2) coherent migmatite complex was recently discovered in the Bohemian Massif, Central European Variscides. Rocks from this complex are characterized by granulite- and amphibolite-facies mineral assemblages and, based on compositional and isotopic trends, are identified as the remnants of a magma body derived from mixing between tonalite and supracrustal rocks. Zircon crystals from the migmatites are exclusively large (200–400?μm) and yield 207Pb/206Pb evaporation ages between 342–328?Ma and single-grain zircon fractions analysed by U–Pb ID-TIMS method plot along the concordia curve between 342 and 325?Ma. High-resolution U–Pb SHRIMP analyses substantiate the existence of a resolvable age variability and yield older 206Pb/238U ages (342–330?Ma, weighted mean age?=?333.6?±?3.1?Ma) for inner zone domains without relict cores and younger 206Pb/238U ages (333–320?Ma, weighted mean age?=?326.0?±?2.8?Ma) for rim domains. Pre-metamorphic cores were identified only in one sample (206Pb/238U ages at 375.0?±?3.9, 420.3?±?4.4 and 426.2?±?4.4?Ma). Most zircon ages bracket the time span between granulite-facies metamorphism in the Bohemian Massif (~345?Ma) and the late-Variscan anatectic overprint (Bavarian phase, ~325?Ma). It is argued that pre-existing zircon was variously affected by these metamorphic events and that primary magmatic growth zones were replaced by secondary textures as a result of diffusion reaction processes and replacement of zircon by dissolution and recrystallization followed by new zircon rim growth. Collectively, the results show that the zircons equilibrated during high-grade metamorphism and record partial loss of radiogenic Pb during post-peak granulite events and new growth under subsequent anatectic conditions.  相似文献   
3.
The Qinling Group was previously interpreted as the oldest Precambrian basement unit of the North Qinling Terrain, recording its formation and early crustal evolution. The Qinling Group consists predominantly of gneisses, amphibolites, and marbles, which underwent multi-phase deformation and metamorphism. In order to better constrain the provenance and tectonic setting of this group and the evolution of the North Qinling orogenic belt, in situ U–Pb dating and oxygen isotopic analysis of zircons in combination with whole-rock geochemistry and Sr–Nd isotope analysis was performed on the two dominant rock types, amphibolite and felsic gneiss. Felsic gneisses exhibit enrichment of LREEs and LILEs (Rb, Ba, Th, K, Pb), negative Eu anomalies and depletion of HFSEs (Nb, Ta, P, Ti). The rocks have slightly elevated δ18O values (6.5–9.3 ‰) and initial ε Nd values of ?4.6 corresponding to two-stage Nd model age of 1.99 Ga. Amphibolites are also enriched in LILEs and LREEs and depleted in Nb and Ta and have homogeneous δ18O values (5.0–6.0 ‰), but higher initial ε Nd values (2.8–3.3) and younger two-stage Nd model ages (1.29–1.24 Ga) compared to the gneisses. The zircon age record indicates that the gneisses and amphibolites were formed in a ~960 Ma volcanic arc environment rather than in a rift setting as previously suggested. A major metamorphic event took place during the Early Paleozoic. Based on the age spectrum of detrital zircons, the Qinling Group is interpreted as an autonomous geological unit, which was mainly derived mostly from 1,000 to 900 Ma old granitoid rocks. The North Qinling Terrain can be regarded as a remnant of the Grenville orogenic belt with an early Neoproterozoic evolution different from that of the North and South China blocks.  相似文献   
4.
The petrogenetic potential of in situ laser ablation Hf isotope data from melt precipitated zircons was explored through the analyses of about 700 individual crystals derived from about 20 different granitic intrusions covering the Variscan basement segment of eastern Bavaria, SE Germany. In combination with geochemical features, four major suites of granitic rocks can be distinguished: (1) NE Bavarian redwitzites (52–57 wt% SiO2, intrusion ages around 323 Ma) have chondritic εHf(t) values (+0.8 to –0.4). The redwitzites are hybrid rocks and the Hf data are permissive of mixing of a mantle progenitor and crustal melts. (2) Various intermediate rock types (dioritic dyke, granodiorite, palite, 59–63 wt% SiO2, 334–320 Ma) from the Bavarian Forest yield negative εHf(t) values between –3.4 and –5.1. These values which apparently contradict a mantle contribution fingerprint an enriched (metasomatized) mantle component that was mixed with crustal material. (3) Voluminous, major crust forming granites sensu stricto (67–75 wt% SiO2, 328–298 Ma) are characterized by a range in εHf(t) values from –0.5 to –5.6. Different crustal sources and/or modification of crustal melts by various input of juvenile material can explain this variation. (4) Post-plutonic (c. 299 Ma) porphyritic dykes of dacitic composition (64–67 wt% SiO2) from the southern Bavarian Forest have chondritic εHf(t) values (+0.6 to –1.1) and display large intergrain Hf isotope variation. The dykes form a separate petrogenetic group and the Hf data suggest that the zircons crystallized when a pristine mantle-derived parental melt was modified by infiltration of crustal material. The zircon Hf data form a largely coherent positive array with the whole-rock Nd data and both systems yield similar two-stage depleted mantle model ages (1.1–1.7 Ga).  相似文献   
5.
On the eastern extremity of the Jiaodong peninsula, China, shoshonitic magmas have been injected into the supracrustal rocks of the Sulu ultra-high pressure (UHP) terrane during the crustal exhumation phase. These granitoids (collectively termed the Shidao igneous complex or Jiazishan alkaline complex) show geochemical and isotopic signatures of an enriched subcontinental lithospheric mantle and intruded soon after the subducted Yangtze crust had reached peak metamorphic pressure conditions (240–220 Ma). We have applied various geochronometers to an alkali-gabbro sample from the Jiazishan pluton and the results allow reconstruction of the Triassic-to-present thermal history. Initial rapid cooling of the gabbro at crustal depths is indicated by the close agreement between the Sm-Nd mineral isochron age (228?±?36 Ma) and the Rb-Sr biotite age (207?±?1) Ma. This interpretation is confirmed by previously published U-Pb zircon ages (225–209 Ma), and 40Ar/39Ar amphibole and K-feldspar ages (~214 Ma) from the Jiazishan syenites. A titanite fission-track age of 166?±?8 Ma (closure temperature range 285–240°C) records widespread Jurassic magmatism in the Jiaodong peninsula, indicating that the gabbro reached upper crustal levels before it was reheated by nearby Jurassic plutons. A subsequent cooling and reheating event is indicated by an apatite fission-track age of 106?±?6 Ma which coincides with the emplacement of the adjacent Weideshan pluton (108?±?2 Ma) and postdates a period of regional lithospheric thinning beneath eastern China. A period of slow cooling (or thermal stability) from late Cretaceous to early Tertiary, documented by an apatite (U-Th)/He age of 39?±?5 Ma, was followed by a final stage of more enhanced cooling since the late Eocene. Results of this work imply that the eastern Sulu terrane has experienced a complex cooling and reheating history. Our data are consistent with a model of initial rapid cooling (sudden exhumation) of the UHP terrane, driven by the release of buoyancy forces, followed by two progressively slower cooling intervals (both after renewed crustal reheating) during the Jurassic and Cretaceous.  相似文献   
6.
We determined U–Pb ages on zircons from Ladakh granitoid samples of three previously undated plutons and deduced four distinct age groups between c. 67 and c. 45 Ma (66.6 ± 2.1, 57.6 ± 1.4, 53.4 ± 1.8, 52.50 ± 0.53 and 45.27 ± 0.56 Ma). This suggests that the Ladakh batholith grew by addition of at least four distinct subduction‐related magma pulses at c. 67, 58, 53 and 45 Ma, thus indicating that the belt was continuously active throughout the Palaeocene and the Middle Eocene (Lutetian). The 45.27 ± 0.56 Ma pluton at Daah‐Hanu is the last major calcalkaline arc magmatic pulse in the Ladakh batholith. Thereafter, the subduction‐related major plutonism gradually waned. The earlier estimate for the youngest pluton within the Ladakh batholith is 49.8 ± 0.8 Ma for the Leh pluton ( J. Geol., 2000, 108 , 303 ).  相似文献   
7.
The Rozvadov Pluton is a complex of mainly Variscan granitoid rocks situated near the Bohemian-Bavarian border between Bärnau, Tachov, Rozvadov and Waidhaus, 25 km ESE of the KTB site. Five mappable units can be distinguished, which intruded as folows: (1) slightly deformed leucocratic meta-aplite/metapegmatite dykes with garnet and tourmaline; (2) a complex of cordierite-bearing granitoids, which have been divided into three facies (a) biotite granite with cordierite (at the margin of the complex), (b) biotite-cordierite granite and (c) cordierite tonalite (in the centre of the complex; (3) fine-grained biotite granite of the Rozvadov type with associated pegmatite bodies; (4) two-mica Bärnau granite; and (5) geochemically specialized albite-zinnwaldite-topaz granite (Kríový kámen/Kreuzstein granite) with indications of Sn-Nb-Ta mineralization and associated phosphorus-rich pegmatite cupolas. Rare earth element data suggest that meta-aplite/pegmatite dykes are the result of a batch partial melting process, whereas the compositional variation of the other rock types was mainly controlled by fractional crystallization. The genesis of the cordierite granitoid suite is best explained in terms of a batch melting of metapelitic source followed by crystallization of a cordierite-rich cumulate and K-feldspar enriched melt. The leucocratic pluton constituents — the meta-aplites and the Bärnau and Kíový kámen granites are rich in phosphorus (0.5–0.8%). The main carriers of phosphorus are alkali feldspars, especially K-feldspar (up to 0.8% P2O5). The presence of P-rich leucocratic granites is one of the features distinguishing the Variscan granitoids within the Moldanubian zone from the nearly contemporaneous granitoids in the Saxothuringian zone.  相似文献   
8.
The Baoshan block of the Tethyan Yunnan, southwestern China, is considered as northern part of the Sibumasu microcontinent. Basement of this block that comprises presumably greenschist-facies Neoproterozoic metamorphic rocks is covered by Paleozoic to Mesozoic low-grade metamorphic sedimentary rocks. This study presents zircon ages and Nd–Hf isotopic composition of granites generated from crustal reworking to reveal geochemical feature of the underlying basement. Dating results obtained using the single zircon U–Pb isotopic dilution method show that granites exposed in the study area formed in early Paleozoic (about 470 Ma; Pingdajie granite) and in late Yanshanian (about 78–61 Ma, Late Cretaceous to Early Tertiary; Huataolin granite). The early Paleozoic granite contains Archean to Mesoproterozoic inherited zircons and the late Yanshanian granite contains late Proterozoic to early Paleozoic zircon cores. Both granites have similar geochemical and Nd–Hf isotopic charateristics, indicating similar magma sources. They have whole-rock T DM(Nd) values of around 2,000 Ma and zircon T DM(Hf) values clustering around 1,900–1,800 and 1,600–1,400 Ma. The Nd–Hf isotopic data imply Paleoproterozoic to Mesoproterozoic crustal material as the major components of the underlying basement, being consistent with a derivation from Archean and Paleoproterozoic terrains of India or NW Australia. Both granites formed in two different tectonic events similarly originated from intra-crustal reworking. Temporally, the late Yanshanian magmatism is probably related to the closure of the Neotethys ocean. The early Paleozoic magmatism traced in the Baoshan block indicates a comparable history of the basements during early Paleozoic between the SE Asia and the western Tethyan belt, such as the basement outcrops in the Alpine belt and probably in the European Variscides that are considered as continental blocks drifting from Gondwana prior to or simultaneously with those of the SE Asia.  相似文献   
9.
We present a geochemical and isotopic study that, consistent with observed field relations, suggest Sangmelima late Archaean high-K granite was derived by partial melting of older Archaean TTG. The TTG formations are sodic-trondhjemitic, showing calcic and calc-alkalic trends and are metaluminous to peraluminous. High-K granites in contrast show a potassic calc-alkaline affinity that spans the calcic, calc-alkalic, alkali-calcic and alkalic compositions. The two rock groups (TTG and high-K granites) on the other hand are both ferroan and magnesian. They have a similar degree of fractionation for LREE but a different one for HREE. Nd model ages and Sr/Y ratios define Mesoarchaean and slab-mantle derived magma compositions respectively, with Nb and Ti anomalies indicating a subduction setting for the TTG. Major and trace element in addition to Sr and Nd isotopic compositions support field observations that indicate the derivation of the high-K granitic group from the partial melting of the older TTG equivalent at depth. Geochemical characteristics of the high-K granitic group are therefore inherited features from the TTG protolith and cannot be used for determining their tectonic setting. The heat budget required for TTG partial melting is ascribed to the upwelling of the mantle marked by a doleritic event of identical age as the generated high-K granite melts. The cause of this upwelling is related to linear delamination along mega-shear zones in an intracontinental setting.  相似文献   
10.
Summary Late-Variscan granitoid plutons in western Bohemia (Bor, Waidhaus-Rozvadov) have distinct petrographic, geochemical and isotopic features that suggest different magmatic evolutions. The Bor pluton comprises a suite of metaluminous tonalites and quartz diorites (Bor I), weakly peraluminous (monzo-)granites and granodiorites (Bor II) and medium-aluminous, late vein-forming leucomonzogranites (Bor III). The Waidhaus-Rozvadov pluton is strongly peraluminous, comprising a cordierite-biotite granitoid (CBG), the Rozvadov granite (ROG), the Bärnau granite (BÄG) and the subordinate, highly evolved Kreuzstein (Kíový kámen) granite (KG). Geochemical parameters and initial87Sr/86Sr ratios straddle the boundary between I- and S-type granites in the Bor pluton and are characteristic of purely S-type granites in the Waidhaus-Rozvadov pluton.The Bor II granitoids have been dated by the Rb-Sr whole-rock method at 341±17 Ma (ISr = 0.70724±0.00060). K-Ar biotite and muscovite ages of all units of the Bor pluton are mainly in the range 321-315 Ma. The K-Ar mineral ages are in good agreement with recently published U-Pb zircon data of these rocks. The different units of the Waidhaus-Rozvadov pluton have yielded less well-constrained Rb-Sr whole-rock ages, ranging from 313 to 300 Ma. However, the intrusion sequence is constrained by K-Ar muscovite ages (312-302 Ma), which define a systematic decrease towards the chemically more evolved granite types. Taken as a whole, it seems likely that the new radiometric ages characterize two temporally distinct periods of late-Variscan granitoid intrusion. The regional significance of these periods is emphasized by contemporaneous ages previously found in the adjacent northeastern Bavarian granitoids.The initial Sr and Nd isotope systematics indicate that the Bor and the WaidhausRozvadov plutons were derived from different source rocks. The Bor granitoids reflect the influence of less evolved crustal material which may have been similar to paragneisses of the Teplá-Barrandian region, including the Zone of ErbendorfVohenstrauß (ZEV). The Waidhaus-Rozvadov granitoids probably resulted from anatexis of rocks resembling surrounding Moldanubian paragneisses or metapelites. In addition, the two plutons exhibit poorly defined, opposite trends of Nd(T) variation which are ascribed to assimilation processes.
Petrogenese kontrastierender Granitplutone in Westböhmen (Tschechien)
Zusammenfassung Spätvariscische Granitplutone in Westböhmen (Bor, Waidhaus-Rozvadov) weisen petrographische, geochemische und isotopische Kontraste auf, die unterschiedliche magmatische Entwicklungen nahelegen. Der Bor Pluton umfaßt metalumine Tonalite und Quarzdiorite (Bor I), schwach peralumine (Monzo-)granite und Granodiorite (Bor II) und mäßig alumine, gangbildende Leukomonzogranite (Bor III). Der WaidhausRozvadov Pluton besitzt stark peralumine Zusammensetzung und läßt sich in einen Cordierit-Biotit Granitoid (CBG), den Rozvadov Granit (ROG), den Bärnau Granit (BÄG) und den stofflich hochentwickelten Kreuzstein (Kíový kámen) Granit (KG) untergliedern. Geochemische Parameter und initiale87Sr/86Sr-Verhältnisse liegen im Falle des Bor Plutons im Übergangsbereich zwischen I- und S-Typ Graniten und im Falle des Waidhaus-Rozvadov Plutons im Bereich reiner S-Typ Granite.Die Bor II Granitoide wurden nach der Rb-Sr Gesamtgesteinsmethode auf 341±17 Ma (ISr = 0.70724±0.00060) datiert. K-Ar Biotit- und Muskovitalter der Bor Granitoide liegen zwischen 321 and 315 Ma. Die K-Ar Mineralalter stehen im Einklang mit den kürzlich publizierten U-Pb Zirkondaten dieser Gesteine. Die verschiedenen Teilintrusionen des Waidhaus-Rozvadov Plutons liefern weniger gut definierte Rb-Sr Gesamtgesteinsalter zwischen 313 and 300 Ma. Die Intrusionsabfolge läßt sich dennoch durch K-Ar Muskovitalter festlegen (312-302 Ma), die eine systematische Abnahme von den weniger zu den starker entwickelten Granittypen aufweisen. Als Ganzes betrachtet dokumentieren die neuen radiometrischen Daten zwei zeitlich voneinander getrennte spdtvariscische Intrusionsereignisse. Die regionale Signifikanz dieser Ereignisse wird durch eine analoge Altersverteilung in den benachbarten nordostbayerischen Granitoiden untermauert.Anhand der initialen Sr und Nd Isotopensystematik können für die Bor und Waidhaus-Rozvadov Plutone unterschiedliche Quellen abgeleitet werden. Die Bor Granitoide spiegeln den Einfluß von gering entwickelten krustalen Material wider, das ähnliche stoffliche Eigenschaften besaß, wie Paragneise des Teplá-Barrandiums und der Zone von Erbendorf-Vohenstrauss (ZEV). Die Waidhaus-Rozvadov Granitoide lassen sich als Derivate moldanubischer Paragneise and Metapelite oder vergleichbarer Gesteine auffassen. Die zwei Plutone weisen schwach ausgeprägte gegensätzliche Nd(T)-Variationen auf, was auf unterschiedliche Assimilationsprozesse zurückgeführt wird.


With 10 Figures  相似文献   
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