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The second-harmonic generation (SHG) circular dichroism in the light of reflection from chiral films of tripod-like chiral molecules is investigated. The expressions of the second-harmonic generation circular dichroism are derived from our presented three-coupled-oscillator model for the tripod-like chiral molecules. Spectral dependence of the circular dichroism of SHG from film surface composed of tripod-like chiral molecules is simulated numerically and analysed. Influence of chiral parameters on the second-harmonic generation circular dichroism spectrum in chiral films is studied. The result shows that the second-harmonic generation circular dichroism is a sensitive method of detecting chirality compared with the ordinary circular dichroism in linear optics. All of our work indicates that the classical molecular models are very effective to explain the second-harmonic generation circular dichroism of chiral molecular system. The classical molecular model theory can give us a clear physical picture and brings us very instructive information about the link between the molecular configuration and the nonlinear processes. 相似文献
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柏杖子金矿系辽西凌源地区重要的岩浆热液型金矿.矿区出露的地层主要为中元古代长城系大红峪组,其次为太古宙建平群变质岩系.长城系大红峪组为金矿的主要容矿围岩,太古宙建平群变质岩系为金矿的矿源层.柏杖子岩体为区域上大柱子岩体的分支岩体,柏杖子岩体由地壳深部上侵的过程中萃取了建平群变质岩系中的成矿物质,沿北北东-北东方向上侵并在长城系大红峪组地层中形成金矿体.通过总结、分析成矿的主要过程,建立了柏杖子金矿的成矿模式. 相似文献
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