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Mangrove-derived dissolved organic matter(DOM) has an important effect on estuarine and coastal area on a large scale.In order to improve the understanding of origin,composition,and fate of DOM in mangrove-fringed estuarine and coastal areas,dissolved humic substances(DHS) were isolated from one mangrove pore-water sample and one near-shore seawater sample downstream the mangrove pore-water site in the eastern coast of Hainan Island,South China.Fulvic acids,humic acids and XAD-4 fractions were obtained from the two water samples by using a two-column array of XAD-8 and XAD-4 resins.Chemical and spectroscopic methods were used to analyze the features of these DHS.Compared to the mangrove pore-water DHS,the near-shore seawater DHS were found rich in 13 C with lower C/N ratios and more aliphatic compounds and carbohydrates,but less aromatic structures and carboxyl groups.As for the three fractions of the two DHS,XAD-4 fractions contain more aliphatics,carbohydrates,carboxyl groups,and enrich in 13 C with respect to both fulvic and humic acids.Photo-oxidation transformation and contribution from marine-derived DOM were considered as the main reasons resulted in the difference in compositional features for these DHS in this study. 相似文献
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The Lake Tian E Zhou(TEZ,an oxbow lake)was formed during the rerouting of the Changjiang River in 1972,with strong influences from the main river channel and flood events.Herein,a sediment core was collected from the Lake TEZ for the measurements of carbon isotopes and biomarkers,including stable carbon isotopes(δ13C),radiocarbon composition(?14C),and lignin phenols,as well as lead-210 to reconstruct recent heavy flood events over the past 70 years.At the 24–26 cm interval,the sediment contained the highest OC%,TN%,and lignin phenols content,as well as significantly depleted 13C but enriched 14C,corresponding to the extreme flood event in 1998.In addition,statistics from t-test showed that lignin phenols normalized to OC(Λ8),the concentration of 3,5-dihydroxy benzoic acid(3,5-BD),and the ratio of p-hydroxy benzophenone to total hydroxyl phenols(PHB/HP)were all significantly different between the layers containing flood deposits and the layers deposited under normal non-flood conditions(p<0.05).These results indicate that the later three parameters are highly related to flood events and can be used as compelling proxies,along with sediment chronology,for hydrological changes and storm/flood events in the river basin and coastal marine environments. 相似文献
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Chemical characterization of fractions of dissolved humic substances from a marginal sea—a case from the Southern Yellow Sea 总被引：1，自引：0，他引：1
Marine dissolved organic matter(DOM) is one of the largest dynamic pools of organic carbon in the global carbon cycle, yet DOM is still chemically poorly characterized. To better understand the origin, composition, and cycling of DOM in the China marginal sea, dissolved humic substances(DHS) were isolated from seawaters in two locations in the Southern Yellow Sea. The DHS were subdivided into fulvic acids(FAs), humic acids(HAs) and the XAD-4 fractions. Complementary analytical approaches were used to characterize the isolated DHS samples including stable carbon isotopic composition, Fourier transform infrared spectroscopy(FTIR), ~(13) C cross polarization magic angle spinning(CP/MAS) nuclear magnetic resonance(NMR), and pyrolysis gas chromatography-mass spectrometry(Py-GC/MS). The results demonstrated that both DHS samples encountered the influences from marine source, indicating that algal and microbial-derived materials are the predominant precursors for the studied samples. The three fractions of DHS showed diff erent properties. FAs presented more aromatic features, whereas HAs contained more aliphatic lipids and proteinaceous materials. The XAD-4 fractions were enriched in ~(13) C and contained more carbohydrates but less aromatic compounds. The lower molecular weight and higher heteroatom content and number of carboxyl groups for the XAD-4 fractions may give them considerable geochemical significance for aspects of trace metal species, bioavailability of pollutants, mineral weathering and water acidification in marine environments. 相似文献
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海底地下水排放对典型红树林蓝碳收支的影响 总被引：1，自引：0，他引：1
海底地下水排放(Submarine Groundwater Discharge，SGD)是陆海相互作用的重要表现形式之一，其携带的物质对近岸海域生源要素的收支有重要影响。本文利用222Rn示踪技术估算了我国典型红树林海湾—广西珍珠湾在2019年枯季(1月)SGD携带的碳通量。调查发现，地下水中222Rn活度、溶解无机碳(DIC)和溶解有机碳(DOC)的平均浓度均高于河水和湾内表层海水。利用222Rn质量平衡模型估算得到珍珠湾SGD速率为(0.36±0.36) m/d，SGD输入到珍珠湾的DIC和DOC通量分别为(2.41±2.63)×107 mol/d和(1.96±2.20)×106 mol/d。珍珠湾溶解碳的源汇收支表明，SGD携带的DIC和DOC分别占珍珠湾总DIC和总DOC来源的91%和89%。因此，SGD携带的DIC和DOC是珍珠湾DIC和DOC的主要来源，是海岸带蓝碳收支和生物地球化学循环过程中的重要组成。 相似文献
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The 226 Ra and 228 Ra activities of Qinghai Lake surface water,groundwater,river water,suspended particles,and bottom sediments were measured in a gamma-ray spectrometer.The sources of 226 Ra and 228 Ra were discussed according to their distribution characteristics.226 Ra and 228 Ra activities(dpm/(100 L)) ranged from 14.13±0.22 to 19.22±0.42 and 17.72±0.66 to 30.96±1.47 in the surface water of the North Bay,respectively,and from 7.88±0.24 to 33.80±0.47 and 15.73±0.74 to 57.31±1.44,respectively,in the South Bay.The surface water near the estuary had a lower salinity and had a higher concentration of radium isotopes than the samples collected further away.The farther offshore the sample,the higher the salinity was,and the lower the radium isotope activity.The distribution of radium activities in the western part of Qinghai Lake is controlled by several factors,including Buha River runoff,desorption from suspended particles derived from the river,groundwater discharge,and a small amount of diffusion from the sediment. 相似文献
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长江口崇明东滩不同植被带沉积速率研究 总被引：1，自引：0，他引：1
利用2007年丰水期、枯水期在崇明东滩芦苇带、藨草带和光滩采集的6根沉积物柱状样,研究了沉积物的粒度特征和过剩的210Pb和228Th及7Be活度的垂向分布特征,探讨了由陆地向海洋不同植被间的沉积物粒度变化规律。依据恒定比活度沉积速率模型,估算了不同时间尺度的崇明东滩芦苇带、藨草带和光滩的表观沉积速率。结果表明:3种核素示踪的崇明东滩的表观沉积速率都随潮滩植被的不同从陆到海方向逐渐降低,同时依过剩的210Pb和228Th,7Be的次序而增大。由过剩的210Pb和228Th计算的夏季沉积速率比冬季的稍高,而由7Be计算的夏季表观沉积速率则明显高于冬季的。结合沉积物粒度的时空分布和这些核素的大气通量,对利用这些核素测定潮滩沉积速率的影响因素进行了探讨。 相似文献
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基于2011-04,2011-08,2011-10和2012-01对桑沟湾海域大面调查的资料,利用改进的荧光镓(LMG)分子荧光光谱分析法测定溶解态铝的含量,研究了桑沟湾溶解态铝的分布和季节变化特征。结果表明,4个航次桑沟湾溶解态铝的平均浓度分别是(47.3±14.4),(56.0±14.6),(64.5±11.3)和(32.1±6.0)nmol/L,呈现出明显的季节变化,即秋季最高,夏季、春季次之,冬季最低。除几个异常站位外,溶解态铝的分布大致呈现随离岸距离的增加其浓度逐渐降低的趋势。夏季表层溶解态铝的浓度在近岸出现低值,夏、秋季湾口北部均出现高值。影响桑沟湾溶解态铝分布的主要因素包括与黄海的水交换、河流及地下水、浮游植物和养殖生物、悬浮颗粒物。根据简单箱式模型对桑沟湾溶解态铝的通量进行了估算,结果显示,除了河流和大气沉降外,桑沟湾溶解态铝还存在其他的源。与相邻的爱莲湾和俚岛湾相比,桑沟湾溶解态铝的浓度在春季较高,在夏季较低。与世界大洋相比,桑沟湾溶解态铝的浓度全年均较高。 相似文献
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