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Organotins, especially tributyltins (TBT) are highly toxic to many marine organisms. These compounds are introduced in marine waters by ship trafficking, ship scrapping activities, as antifouling compounds and sewage disposal. Marine fishes, crustaceans and molluscans are easily prone to organotins contamination. In view of this, a baseline monitoring study was conducted in order to establish the levels of organotins in edible marine fishes, bivalves, shrimps, squids and crabs collected from Mumbai, Goa and Karwar on the west coast of India. At these locations average organotin concentration found in fishes, clams, shrimps, squids and crabs was 108, 852, 179, 70 and 89 ng Sn g−1 dw, respectively. In all the samples butyltins dominated over phenyltins. The levels of organotins suggest that all the organisms were contaminated with organotins and their consumption may pose health problems to humans. 相似文献
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Nicolas Briant Chrystelle Bancon-Montigny Françoise Elbaz-Poulichet Rémi Freydier Sophie Delpoux Daniel Cossa 《Marine pollution bulletin》2013
The study of trace elements (Cu, Zn, Pb, As, Hg) and butyltin concentrations in the sediments of Port Camargue enabled assessment of the levels and history of the contamination of the largest European marina linked with the use of antifouling paints. Surface sediments near the boat maintenance area were heavily contaminated with up to 1497 μg g−1 of Cu, 475 μg g−1 of Zn, 0.82 μg g−1 of Hg, 94 μg g−1 of Pb and over 10,000 ngSn g−1 of tributyltin (TBT). High concentrations of Hg and TBT indicate ongoing sources of these elements despite the ban on their use as biocides in paints. Sediment cores provided records of contamination since 1969. The peak concentrations of As, Hg, Pb and TBT in the sediment profile reflect their presence on boat hulls when the marina was built at the end of the 1960s. Degradation of TBT in the sediments near the boat maintenance area is slow compared to other less contaminated area of the marina. 相似文献
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The concentrations of butyltins along the Japanese coastline were investigated from 1997 to 1999, 7 to 9 years after implementation of legislation limiting the use of tributyltin (TBT) in Japan. Seawater was sampled at 0.5 m depth, and Caprella spp. were collected from Sargassum spp. and aquaculture facilities from 18 areas within four broad areas along the coastline of Japan, i.e., the Pacific coast of northern Japan, the coast along the Sea of Japan, Tokyo Bay and adjacent areas, and western Japan. Butyltins (MBT, DBT and TBT) were detected in 32 of the 63 seawater samples with average concentrations of 4.6 ng MBT/l, 4.5 ng DBT/l and 6.8 ng TBT/l, respectively. Butyltin concentrations in seawater from western Japan indicate "hot spots" even in unpopulated areas. Butyltins (MBT, DBT and TBT) were detected in all samples of Caprella spp., varying from 2.3 ng BTs /g wet wt in C. penantis R-type from Tobishima Island in the Sea of Japan to 464 ng BTs /g wet wt in C. decipiens Mayer from Amakusa, western Kyushu. The BT concentrations in Caprella spp. form western Japan were significantly higher than those from other areas, including Tokyo Bay and adjacent areas, where large scale industry and international ports are located. These results indicate that butyltin contamination still remains even in unpopulated areas after the regulation on TBT usage, and that the regulation governing TBT usage since 1990 has not been effective enough to concede recovery of shallow water ecosystems around Japan. 相似文献
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The time series of analyzed values indicated that concentration of butyltin (BT) compounds in ballast water varied widely depending on the tanks, depths, and dates of sampling, ranging 4–93 ng l−1 during 7-day voyage. Variations in concentrations of BT in the two ballast tanks corresponded well with the level of BT contamination in different pumping sites of ballast waters. Concentrations of BT species detected in ballast water were rather consistent with those found in port waters and sediment of Taiwan and Japan. This study suggested that the problems concerning BT contamination were neither static nor localized. 相似文献
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Worldwide measures to restrict tributyltin (TBT) in antifouling paints have been legislated for decades, and were upgraded to a total ban on September 2008. With a view to test the response of coastal biota to changing pollution, since 1996 we have determined the concentration of TBT and derivatives di- and mono-butyltin (DBT and MBT) in NW Spain populations of two gastropods of contrasting biology, the rock-snail Nucella lapillus (n = 18) and the mud-snail Nassarius reticulatus (n = 24). TBT pollution in the study area has decreased consistently and considerably over time. In addition, the baseline butyltin (BT) bioaccumulation patterns showed a marked but transient distortion. These field observations are consistent with BT desorption from sediments, a natural phenomenon that is now to be expected in developing countries recently subject to the global TBT ban. 相似文献
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