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1.
The knowledge of the residence time of formation water is fundamental to understanding the subsurface flow and hydrological setting. To better identify the origin and evolution of coal seam water and its impact on gas storage and production, this study collected coalbed methane co-produced water in the southeast Qinshui Basin and detected chemical and isotopic compositions, especially 36Cl and 129I concentrations. The calculated tracer ages of 129I (5.2–50.6 Ma) and 36Cl (0.13–0.76 Ma) are significantly younger than the age of coal-bearing formation (Pennsylvanian - Cisuralian), indicating freshwater recharge after coal deposition. The model that utilises 129I/I and 36Cl/Cl ratios to constrain the timing of recharge and the proportion of recharge water reveals that over 60% of pre-anthropogenic meteoric water entered coal seams since 10 Ma and mixed with residue initial deposition water, corresponding to the basin inversion in Cenozoic. The spatial distribution of major ion concentrations reveals the primary recharge pathway for meteoric water from coal outcrops at the eastern margin to the basin center. This study demonstrates the occurrence of higher gas production rates from wells that accept water recharge in recent times and suggests the possible potential of the non-stagnant zones for high gas production.  相似文献   
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Variation in the concentrations of iodine-129 (129I, T1/2=15.7 Myr), a low-level radioactive component of nuclear fuel waste, is documented in surface waters and depth profiles collected during 2001 along a transect from the Norwegian Coastal Current to the North Pole. The surface waters near the Norwegian coast are found to have 20 times higher 129I concentration than the surface waters of the Arctic Ocean. The depth profiles of 129I taken in the Arctic Ocean reveal a sharp decline in the concentration to a depth of about 300-500 m followed by a weaker gradient extending down to the bottom. A twofold increase in the 129I concentration is observed in the upper 1000 m since 1996. Based on known estimates of marine transient time from the release sources (the nuclear reprocessing facilities at La Hague, France, and Sellafield, UK), a doubling in the 129I inventory of the top 1000 m of the Arctic Ocean is expected to occur between the years 2001 and 2006. As 129I of polar mixed layer and Atlantic layer of the Arctic Ocean is ventilated by the East Greenland Current into the Nordic Seas and North Atlantic Ocean, further dispersal and increase of the isotope concentration in these regions will be encountered in the near future.  相似文献   
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Previous studies have shown that brines in an Ordovician paleokarst reservoir of the Lunnan oilfield in the Tarim Basin, China, are the product of mixing of paleo-evaporated seawater in the east with paleometeoric waters in the west. In order to put time constraints on the brine and related hydrocarbons in this field, 10 brine samples were collected, for which the iodine concentrations and 129I/I ratios were measured and discussed. The iodine concentration (3.70–31.2 mg/L) and the 129I/I ratio (189–897 × 10−15) show that the iodine in the paleoseawater and meteoric water (MW) had different origins and 129I characteristics. The paleoseawater has a high iodine content (∼31 mg/L), indicating that iodine was introduced into the reservoir along with thermally generated hydrocarbons, possibly in the Cretaceous, from the Caohu Sag in the eastern area. Based on consideration of all possible origins of iodine and 129I in the brines, it is suggested that the meteoric water maintained its initial iodine content (0.01 mg/L) and 129I/I ratio (1500 × 10−15), whereas the iodine-enriched paloseawater (IPSW) exhibited a secular 129I equilibrium (Nsq = 39 atom/μL) as a result of fissiogenic 129I input in the reservoir over a long period of time. The model of brine evolution developed on that basis confirmed that meteoric water entered the reservoir in the Miocene at about 10 Ma, and partially mixed with the iodine-enriched paleoseawater. The movement of meteoric water was facilitated by faults created during the Himalayan orogeny, then became more dense after dissolving Paleogene halite and infiltrated into the reservoir at high pressure. The iodine and 129I concentration in the brine contains information about the path and history of the fluid in the reservoir. This may be useful in oil exploration, since the movement of water was, to some extent, related to hydrocarbon migration.  相似文献   
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Uncertainty analysis of radioactive nuclide transport for one-dimensional single fracture has been studied. First order differential analysis is applied to introduce analytical form of output expectation and variance for contaminant transport equation, by regarding uncertainty of dispersion coefficient and retardation factor. Breakthrough curve of dimensionless concentration is demonstrated by taking I-129 as radioactive nuclide in fracture transport. It is possible to pick up critical ranges in spatial and temporal domain from the output variance. From the viewpoint of preliminary performance assessment for nuclear waste disposal the parameter importance in such system can be substantially measured in the site characterization in future.  相似文献   
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We present multifrequency VLA observations of the two radio galaxies 3C 129 and 3C 129.1 embedded in a luminous X-ray cluster. These radio observations reveal a substantial difference in the Faraday Rotation Measures (RMs) toward 3C 129.1 at the cluster centre and 3C 129 at the cluster periphery. After deriving the density profile from available X-ray data, we find that the RM structure of both radio galaxies can be fitted by a tangled cluster magnetic field with strength 6 μG extending at least 3 core radii (450 kpc) from the cluster centre. The magnetic field makes up a small contribution to the total pressure (5 per cent) in the central regions of the cluster. The radio morphology of 3C 129.1 appears disturbed on the southern side, perhaps by the higher pressure environment. In contrast with earlier claims for the presence of a moderately strong cooling flow in the 3C 129 cluster, our analysis of the X-ray data places a limit on the mass deposition rate from any such flow of < 1.2 M yr−1.  相似文献   
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The concentrations of 129I in seawater samples from two sites (off Sekine and the Toyama Bay) in the Japan Sea were determined by accelerator mass spectrometry. The observed concentrations exceed amounts expected from natural origin and globally distributed fallout due to nuclear weapons testing. Because the fraction of natural origin and global fallout is 2% and 8.9–13.8%, respectively, the residual more than 80% of the concentration must come primarily from nuclear fuel reprocessing plants. This result indicates a rapid distribution of 129I through atmospheric transport on a global scale. The depth distribution of 129I at the Toyama Bay in the Japan Sea shows that the 129I maximum is in the mixed layer and that concentrations decrease with depth. The inventory of 129I in water column is four times higher than that measured in the Gulf of Mexico which has almost the same depth at the Toyama Bay. This higher inventory probably reflects: (1) the rapid water sinking in the Japan Sea, (2) the difference of distance in sampling locations with respect to major 129I releasing plants and (3) the strong increase in emissions from nuclear fuel reprocessing plants after the profile of the Gulf of Mexico was taken.  相似文献   
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^129I的海洋放射年代学及其他应用研究进展   总被引:3,自引:0,他引:3  
刘广山  纪丽红 《台湾海峡》2010,29(1):140-147
应用^129I的海洋学研究可分为3个方面:(1)人工^129I的年代学,利用人工放射性在沉积物岩心中的记录,包括以核试验全球最大沉降年1963年为参考时间和利用切尔诺贝利核电站事故发生的1986年作为参考时间的年代测定.(2)利用宇生^129I的年代学,测年体系主要有地热流体、天然气水合物扣石油地质体系.(3)利用核燃料后处理厂排放的^129I进行的海洋环流与混合研究.核试验和核事故释放的^129I测定的是现代沉积物年代,测年时间尺度为50a.人们提出人类利用原子能之前地球表层初始^129I丰度为1.5×10^-12。,并以该值作为利用宇生^129I估算年代的初始丰度值.半哀期和丰度探测下限水平允许宇生^129I可测年的时间尺度为80Ma.本文综述了以上几方面的研究进展.海洋多金属结核和结壳的生长速率为毫米每兆年量级,一块1~10cm大小的多金属结核和结壳所能涵盖的时间尺度约为10~100Ma,刚好是^129I测年的时间尺度,所以本文提出了多金属结核和结壳可能是合适的^129I测年介质的观点.  相似文献   
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We report results of our optical photometric observations of ten gamma-ray loud blazers, namely: 0219+428 (3C66A), PKS 0420-014 (OA 129), S5 0716+714, 0754+100 (OI 090.4), 0827+243 (OJ248), 1652+398 (Mrk 501), 2200+420 (BL Lacertae), 2230+114 (CTA 102), 2251+158 (3C 454.3) and 2344+514. The observations were carried out in September-October, 2000 using the 70 cm optical telescope at Abstumani Observatory, Georgia. We found intra-day variations in 0420-014, S5 0716+714, BL Lacertae and CTA 102. A variation of 0.3 magnitude over a time scale of about 3 hours was observed in the R passband in BL Lacertae on JD 2451827. We did not detect any variation in 3C 66A, Mrk 501, or 3C 454.3 during our observations. Nor did we detect any clear evidence of variation in 1ES 2344+514 during our two weeks' observing run of the TeV gamma-ray source.  相似文献   
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